A set-up for Hard X-ray Time-resolved Resonant Inelastic X-ray Scattering at SwissFEL

We present a new set up for resonant inelastic hard X-ray scattering at the Bernina beamline of SwissFEL with energy, momentum, and temporal resolution. The compact R=0.5 m Johann-type spectrometer can be equipped with up to 3 crystal analysers and allows efficient collection of RIXS spectra. Optica...

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Veröffentlicht in:arXiv.org 2023-12
Hauptverfasser: Hui-Yuan, Chen, Versteeg, Rolf B, Puppin, Michele, Leroy, Ludmila, Mankowsky, Roman, Bohler, Pirmin, Deng, Yunpei, Kerkhoff, Linda, Mozzanica, Aldo, Oggenfuss, Roland Alexander, Pradervand, Claude, Sander, Mathias, Smolentsev, Grigory, Vetter, Seraphin, Zamofing, Thierry, Lemke, Henrik T, Chergui, Majed, Mancini, Giulia F
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Sprache:eng
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Zusammenfassung:We present a new set up for resonant inelastic hard X-ray scattering at the Bernina beamline of SwissFEL with energy, momentum, and temporal resolution. The compact R=0.5 m Johann-type spectrometer can be equipped with up to 3 crystal analysers and allows efficient collection of RIXS spectra. Optical pumping for time-resolved studies can be realized with a broad span of optical wavelengths. We demonstrate the performance of the set-up at overall ~180 meV resolution in a study of ground-state and photoexcited (at 400 nm) honeycomb 5d iridate \(\alpha\)-\(\mathrm{Li_2IrO_3}\). Steady-state RIXS spectra at the Iridium \({L_3}\)-edge (11.214 keV) have been collected and are in very good agreement with data collected at synchrotrons. The time-resolved RIXS transients (pumped minus unpumped spectra) exhibit changes in the energy-loss region
ISSN:2331-8422
DOI:10.48550/arxiv.2312.10133