Pulse-area theorem for precision control of the rotational motions of a single molecule in a cavity
Journal of Physics A: Mathematical and Theoretical, 2023 We perform a combined analytical and numerical investigation to explore how an analytically designed pulse can precisely control the rotational motions of a single-molecular polariton formed by the strong coupling of two low-lying rotational s...
Gespeichert in:
| Hauptverfasser: | , |
|---|---|
| Format: | Artikel |
| Sprache: | eng |
| Schlagworte: | |
| Online-Zugang: | Volltext bestellen |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | |
|---|---|
| container_issue | |
| container_start_page | |
| container_title | |
| container_volume | |
| creator | Fan, Li-Bao Shu, Chuan-Cun |
| description | Journal of Physics A: Mathematical and Theoretical, 2023 We perform a combined analytical and numerical investigation to explore how
an analytically designed pulse can precisely control the rotational motions of
a single-molecular polariton formed by the strong coupling of two low-lying
rotational states with a single-mode cavity. To this end, we derive a
pulse-area theorem that gives amplitude and phase conditions of the pulses in
the frequency domain for driving the polariton from a given initial state to an
arbitrary coherent state. The pulse-area theorem is examined for generating the
maximum degree of orientation using a pair of pulses. We show that the phase
condition can be satisfied by setting the initial phases of the two identically
overlapped pulses or by controlling the time delay between pulses for practical
applications. |
| doi_str_mv | 10.48550/arxiv.2308.01567 |
| format | Article |
| fullrecord | <record><control><sourceid>arxiv_GOX</sourceid><recordid>TN_cdi_arxiv_primary_2308_01567</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2308_01567</sourcerecordid><originalsourceid>FETCH-LOGICAL-a677-1e73bce8d36e7185732426a9022c4b48e4fd01c45b692b8379ffa5624727489f3</originalsourceid><addsrcrecordid>eNotj8tqwzAQRbXpoqT9gK6qH7Crt-RlCH1BoFlkb8bKqBHYVpCV0Px97bSruZw7zHAIeeKsVk5r9gL5J15qIZmrGdfG3hO_O_cTVpARaDliyjjQkDI9ZfRximmkPo0lp56msCzQnAqUmUNPh7SEaWmATnH87nFmPfrzHOI4Qw-XWK4P5C7A_OXxf67I_u11v_motl_vn5v1tgJjbcXRys6jO0iDljttpVDCQMOE8KpTDlU4MO6V7kwjOidtEwJoI5QVVrkmyBV5_jt7s2xPOQ6Qr-1i295s5S8NE1AB</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype></control><display><type>article</type><title>Pulse-area theorem for precision control of the rotational motions of a single molecule in a cavity</title><source>arXiv.org</source><creator>Fan, Li-Bao ; Shu, Chuan-Cun</creator><creatorcontrib>Fan, Li-Bao ; Shu, Chuan-Cun</creatorcontrib><description>Journal of Physics A: Mathematical and Theoretical, 2023 We perform a combined analytical and numerical investigation to explore how
an analytically designed pulse can precisely control the rotational motions of
a single-molecular polariton formed by the strong coupling of two low-lying
rotational states with a single-mode cavity. To this end, we derive a
pulse-area theorem that gives amplitude and phase conditions of the pulses in
the frequency domain for driving the polariton from a given initial state to an
arbitrary coherent state. The pulse-area theorem is examined for generating the
maximum degree of orientation using a pair of pulses. We show that the phase
condition can be satisfied by setting the initial phases of the two identically
overlapped pulses or by controlling the time delay between pulses for practical
applications.</description><identifier>DOI: 10.48550/arxiv.2308.01567</identifier><language>eng</language><subject>Physics - Quantum Physics</subject><creationdate>2023-08</creationdate><rights>http://creativecommons.org/licenses/by/4.0</rights><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>228,230,781,886</link.rule.ids><linktorsrc>$$Uhttps://arxiv.org/abs/2308.01567$$EView_record_in_Cornell_University$$FView_record_in_$$GCornell_University$$Hfree_for_read</linktorsrc><backlink>$$Uhttps://doi.org/10.48550/arXiv.2308.01567$$DView paper in arXiv$$Hfree_for_read</backlink></links><search><creatorcontrib>Fan, Li-Bao</creatorcontrib><creatorcontrib>Shu, Chuan-Cun</creatorcontrib><title>Pulse-area theorem for precision control of the rotational motions of a single molecule in a cavity</title><description>Journal of Physics A: Mathematical and Theoretical, 2023 We perform a combined analytical and numerical investigation to explore how
an analytically designed pulse can precisely control the rotational motions of
a single-molecular polariton formed by the strong coupling of two low-lying
rotational states with a single-mode cavity. To this end, we derive a
pulse-area theorem that gives amplitude and phase conditions of the pulses in
the frequency domain for driving the polariton from a given initial state to an
arbitrary coherent state. The pulse-area theorem is examined for generating the
maximum degree of orientation using a pair of pulses. We show that the phase
condition can be satisfied by setting the initial phases of the two identically
overlapped pulses or by controlling the time delay between pulses for practical
applications.</description><subject>Physics - Quantum Physics</subject><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><sourceid>GOX</sourceid><recordid>eNotj8tqwzAQRbXpoqT9gK6qH7Crt-RlCH1BoFlkb8bKqBHYVpCV0Px97bSruZw7zHAIeeKsVk5r9gL5J15qIZmrGdfG3hO_O_cTVpARaDliyjjQkDI9ZfRximmkPo0lp56msCzQnAqUmUNPh7SEaWmATnH87nFmPfrzHOI4Qw-XWK4P5C7A_OXxf67I_u11v_motl_vn5v1tgJjbcXRys6jO0iDljttpVDCQMOE8KpTDlU4MO6V7kwjOidtEwJoI5QVVrkmyBV5_jt7s2xPOQ6Qr-1i295s5S8NE1AB</recordid><startdate>20230803</startdate><enddate>20230803</enddate><creator>Fan, Li-Bao</creator><creator>Shu, Chuan-Cun</creator><scope>GOX</scope></search><sort><creationdate>20230803</creationdate><title>Pulse-area theorem for precision control of the rotational motions of a single molecule in a cavity</title><author>Fan, Li-Bao ; Shu, Chuan-Cun</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a677-1e73bce8d36e7185732426a9022c4b48e4fd01c45b692b8379ffa5624727489f3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Physics - Quantum Physics</topic><toplevel>online_resources</toplevel><creatorcontrib>Fan, Li-Bao</creatorcontrib><creatorcontrib>Shu, Chuan-Cun</creatorcontrib><collection>arXiv.org</collection></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext_linktorsrc</fulltext></delivery><addata><au>Fan, Li-Bao</au><au>Shu, Chuan-Cun</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Pulse-area theorem for precision control of the rotational motions of a single molecule in a cavity</atitle><date>2023-08-03</date><risdate>2023</risdate><abstract>Journal of Physics A: Mathematical and Theoretical, 2023 We perform a combined analytical and numerical investigation to explore how
an analytically designed pulse can precisely control the rotational motions of
a single-molecular polariton formed by the strong coupling of two low-lying
rotational states with a single-mode cavity. To this end, we derive a
pulse-area theorem that gives amplitude and phase conditions of the pulses in
the frequency domain for driving the polariton from a given initial state to an
arbitrary coherent state. The pulse-area theorem is examined for generating the
maximum degree of orientation using a pair of pulses. We show that the phase
condition can be satisfied by setting the initial phases of the two identically
overlapped pulses or by controlling the time delay between pulses for practical
applications.</abstract><doi>10.48550/arxiv.2308.01567</doi><oa>free_for_read</oa></addata></record> |
| fulltext | fulltext_linktorsrc |
| identifier | DOI: 10.48550/arxiv.2308.01567 |
| ispartof | |
| issn | |
| language | eng |
| recordid | cdi_arxiv_primary_2308_01567 |
| source | arXiv.org |
| subjects | Physics - Quantum Physics |
| title | Pulse-area theorem for precision control of the rotational motions of a single molecule in a cavity |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2024-12-15T14%3A47%3A52IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-arxiv_GOX&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Pulse-area%20theorem%20for%20precision%20control%20of%20the%20rotational%20motions%20of%20a%20single%20molecule%20in%20a%20cavity&rft.au=Fan,%20Li-Bao&rft.date=2023-08-03&rft_id=info:doi/10.48550/arxiv.2308.01567&rft_dat=%3Carxiv_GOX%3E2308_01567%3C/arxiv_GOX%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_id=info:pmid/&rfr_iscdi=true |