Lattice effect on the superexchange interaction in antiferromagnetic Bi$_2$Sr$_2$CaCu$_2$O$_8
The in-plane superexchange interaction $J$ of cuprate superconductors has long been suggested to be an important parameter for exploring their high-temperature superconductivity. The bilayer Bi$_2$Sr$_2$CaCu$_2$O$_{8+\delta}$ is the most studied system with high-quality single crystals in the wide d...
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Zusammenfassung: | The in-plane superexchange interaction $J$ of cuprate superconductors has
long been suggested to be an important parameter for exploring their
high-temperature superconductivity. The bilayer
Bi$_2$Sr$_2$CaCu$_2$O$_{8+\delta}$ is the most studied system with high-quality
single crystals in the wide doping range with the the same structure and phase.
So far, the lattice parameter dependence of $J$ in its antiferromagnetic parent
compound Bi$_2$Sr$_2$CaCu$_2$O$_{8}$ has not been established. By combining
Raman scattering and x-ray diffraction techniques on the same sample in the
same pressure environment, we obtain the evolution of both the two-magnon
spectrum and the structural parameters with pressure up to nearly 30 GPa, The
relationship between pressure or the in-plane lattice parameter and $J$ is thus
established for Bi$_2$Sr$_2$CaCu$_2$O$_{8}$. Over the studied pressure range,
superconductivity does not appear in this parent compound based on a sensitive
magnetic measurement technique. The effects of pressure and chemical doping on
the superexchange interaction and structure and their implications for
superconductivity are discussed from the comparison of the obtained
experimental data with the existing experiments. The results and findings
provide valuable information for the understanding of superconductivity and the
future theory developments for superconductivity in cuprates. |
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DOI: | 10.48550/arxiv.2304.11311 |