Many-body recombination in insulating cuprates
We study the pump-probe response of three insulating cuprates and develop a model for its recombination kinetics. The dependence on time, fluence, and both pump and probe photon energies imply many-body recombination on femtosecond timescales, characterized by anomalously large trapping and Auger co...
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Veröffentlicht in: | arXiv.org 2019-12 |
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Hauptverfasser: | , , , , , , |
Format: | Artikel |
Sprache: | eng |
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Zusammenfassung: | We study the pump-probe response of three insulating cuprates and develop a model for its recombination kinetics. The dependence on time, fluence, and both pump and probe photon energies imply many-body recombination on femtosecond timescales, characterized by anomalously large trapping and Auger coefficients. The fluence dependence follows a universal form that includes a characteristic volume scale, which we associate with the holon-doublon excitation efficiency. This volume varies strongly with pump photon energy and peaks near twice the charge-transfer energy, suggesting that the variation is caused by carrier multiplication through impact ionization. |
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ISSN: | 2331-8422 |
DOI: | 10.48550/arxiv.1912.01604 |