Many-body recombination in insulating cuprates

We study the pump-probe response of three insulating cuprates and develop a model for its recombination kinetics. The dependence on time, fluence, and both pump and probe photon energies imply many-body recombination on femtosecond timescales, characterized by anomalously large trapping and Auger co...

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Veröffentlicht in:arXiv.org 2019-12
Hauptverfasser: Sahota, Derek G, Liang, Ruixing, Dion, M, Fournier, Patrick, Dąbkowska, Hanna A, Luke, Graeme M, Dodge, J Steven
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Sprache:eng
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Zusammenfassung:We study the pump-probe response of three insulating cuprates and develop a model for its recombination kinetics. The dependence on time, fluence, and both pump and probe photon energies imply many-body recombination on femtosecond timescales, characterized by anomalously large trapping and Auger coefficients. The fluence dependence follows a universal form that includes a characteristic volume scale, which we associate with the holon-doublon excitation efficiency. This volume varies strongly with pump photon energy and peaks near twice the charge-transfer energy, suggesting that the variation is caused by carrier multiplication through impact ionization.
ISSN:2331-8422
DOI:10.48550/arxiv.1912.01604