Low-temperature electroluminescence excitation mapping of excitons and trions in short channel monochiral carbon nanotube device
Single walled carbon nanotubes as emerging quantum-light sources may fill a technological gap in silicon photonics due to their potential use as near infrared, electrically driven, classical or non-classical emitters. Unlike in photoluminescence, where nanotubes are excited with light, electrical ex...
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Zusammenfassung: | Single walled carbon nanotubes as emerging quantum-light sources may fill a
technological gap in silicon photonics due to their potential use as near
infrared, electrically driven, classical or non-classical emitters. Unlike in
photoluminescence, where nanotubes are excited with light, electrical
excitation of single tubes is challenging and heavily influenced by device
fabrication, architecture and biasing conditions. Here we present
electroluminescence spectroscopy data of ultra short channel devices made from
(9,8) carbon nanotubes emitting in the telecom band. Emissions are stable under
current biasing and no quenching is observed down to 10 nm gap size.
Low-temperature electroluminescence spectroscopy data also reported exhibits
cold emission and linewidths down to 2 meV at 4 K. Electroluminescence
excitation maps give evidence that carrier recombination is the mechanism for
light generation in short channels. Excitonic and trionic emissions can be
switched on and off by gate voltage and corresponding emission efficiency maps
were compiled. Insights are gained into the influence of acoustic phonons on
the linewidth, absence of intensity saturation and exciton exciton
annihilation, environmental effects like dielectric screening and strain on the
emission wavelength, and conditions to suppress hysteresis and establish
optimum operation conditions. |
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DOI: | 10.48550/arxiv.1909.05126 |