Thermal transport and phonon hydrodynamics in strontium titanate

We present a study of thermal conductivity, \(\kappa\), in undoped and doped strontium titanate in a wide temperature range (2-400 K) and detecting different regimes of heat flow. In undoped SrTiO\(_{3}\), \(\kappa\) evolves faster than cubic with temperature below its peak and in a narrow temperatu...

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Veröffentlicht in:arXiv.org 2018-03
Hauptverfasser: Martelli, Valentina, Julio Larrea Jiménez, Continentino, Mucio, Baggio-Saitovitch, Elisa, Behnia, Kamran
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Sprache:eng
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Zusammenfassung:We present a study of thermal conductivity, \(\kappa\), in undoped and doped strontium titanate in a wide temperature range (2-400 K) and detecting different regimes of heat flow. In undoped SrTiO\(_{3}\), \(\kappa\) evolves faster than cubic with temperature below its peak and in a narrow temperature window. Such a behavior, previously observed in a handful of solids, has been attributed to a Poiseuille flow of phonons, expected to arise when momentum-conserving scattering events outweigh momentum-degrading ones. The effect disappears in presence of dopants. In SrTi\(_{1-x}\)Nb\(_{x}\)O\(_{3}\), a significant reduction in lattice thermal conductivity starts below the temperature at which the average interdopant distance and the thermal wavelength of acoustic phonons become comparable. In the high-temperature regime, thermal diffusivity becomes proportional to the inverse of temperature, with a prefactor set by sound velocity and Planckian time (\(\tau_{p}=\frac{\hbar}{k_{B}T}\)).
ISSN:2331-8422
DOI:10.48550/arxiv.1802.05868