Unveiling a Hidden Order Transition at the Interface of an Exchange-Spring-Coupled Ferromagnet/Antiferromagnet Bilayer

Study of the exchange bias (H ex) switching in a ferromagnet (FM)/antiferromagnet (AFM) bilayer driven by spin–orbit torque (SOT) has currently been an explicit research field for various SOT applications, but a complete understanding of AFM and its interaction with SOT at an FM/AFM interface remain...

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Veröffentlicht in:ACS applied electronic materials 2024-12, Vol.6 (12), p.9053-9060
Hauptverfasser: Yang, Chao-Yao, Tseng, Chih-Hsiang, Chen, Sheng-Huai, Cheng, Chih-Wei, Lai, Chih-Huang
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Sprache:eng
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Zusammenfassung:Study of the exchange bias (H ex) switching in a ferromagnet (FM)/antiferromagnet (AFM) bilayer driven by spin–orbit torque (SOT) has currently been an explicit research field for various SOT applications, but a complete understanding of AFM and its interaction with SOT at an FM/AFM interface remains elusive. This study reports an SOT-driven hidden order transition behind the H ex in a heavy metal (Pt)/FM (Co)/AFM (IrMn) trilayer along with the interaction between Co magnetization (with perpendicular anisotropy) and IrMn spins. The exchange coupling across the Co/IrMn interface facilitates a long-range spin order in the form of an exchange-spring configuration, resulting in two distinct orders in IrMn: a canting-induced FM order ( m ⇀ ) responsible for hosting H ex and a hidden Néel order ( n ⇀ ) representing the AFM nature. The SOT generated in Pt appeared to disturb the order in IrMn when it was first applied to the device, leading to the reduction in m ⇀ along the perpendicular direction and an increase in the component of n ⇀ along the current axis; therefore, a diminished H ex along with a developed planar anisotropic magnetoresistance (MR) can be observed. The coupled transitions of m ⇀ and n ⇀ appear to be irreversibly driven by SOT and independent of current polarity at the first SOT measurement. Subsequent SOT measurements reveal a reversible switching of m ⇀ , manifested by the reversible H ex switching while n ⇀ remains unaltered along the current axis, as indicated by the unchanged anisotropic MR. This work unveils a hidden Néel order transition at a fully dynamic FM/AFM interface.
ISSN:2637-6113
2637-6113
DOI:10.1021/acsaelm.4c01698