Transition metal-dinitrogen complexes preparation and reactivity
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| 084 | |a VH 9600 |0 (DE-625)147383:253 |2 rvk | ||
| 245 | 1 | 0 | |a Transition metal-dinitrogen complexes |b preparation and reactivity |c edited by Yoshiaki Nishibayashi |
| 264 | 1 | |a Weinheim |b Wiley-VCH |c [2019] | |
| 264 | 4 | |c © 2019 | |
| 300 | |a XIII, 481 Seiten |b Illustrationen, Diagramme | ||
| 336 | |b txt |2 rdacontent | ||
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| 653 | |a Biochemie | ||
| 653 | |a Biochemie u. Chemische Biologie | ||
| 653 | |a Catalysis | ||
| 653 | |a Chemie | ||
| 653 | |a Chemistry | ||
| 653 | |a Coordination Chemistry | ||
| 653 | |a Katalyse | ||
| 653 | |a Koordinationschemie | ||
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| 689 | 0 | 1 | |a Stickstofffixierung |0 (DE-588)4183273-5 |D s |
| 689 | 0 | |5 DE-604 | |
| 700 | 1 | |a Nishibayashi, Yoshiaki |d 1968- |0 (DE-588)1158503199 |4 edt | |
| 710 | 2 | |a Wiley-VCH |0 (DE-588)16179388-5 |4 pbl | |
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| adam_text | CONTENTS
PREFACE
XI
ABOUT
THE
EDITOR
XIII
1
OVERVIEWS
OF
THE
PREPARATION
AND
REACTIVITY
OF
TRANSITION
METAL-DINITROGEN
COMPLEXES
1
YOSHIAKI
TANABE
AND
YOSHIAKI
NISHIBAYASHI
1.1
INTRODUCTION
1
1.2
BIOLOGICAL
NITROGEN
FIXATION
4
1.3
HISTORICAL
BACKGROUND
OF
TRANSITION
METAL-DINITROGEN
COMPLEXES
9
1.4
COORDINATION
CHEMISTRY
OF
TRANSITION
METAL-DINITROGEN
COMPLEXES
13
1.4.1
COORDINATION
PATTERNS
OF
DINITROGEN
AND
MONONUCLEAR
TRANSITION
METAL-DINITROGEN
COMPLEXES
13
1.4.2
MULTINUCLEAR
TRANSITION
METAL-DINITROGEN
COMPLEXES
16
1.5
CHEMICAL ACTIVATION
AND
REACTIVITY
OF
DINITROGEN
USING
TRANSITION
METAL
COMPLEXES
21
1.5.1
PROTONATION
OF
TRANSITION
METAL-BOUND
DINITROGEN
21
1.5.2
CLEAVAGE
OF
TRANSITION
METAL-BOUND
DINITROGEN
25
1.5.3
REACTION
OF
TRANSITION METAL-BOUND
DINITROGEN
WITH
DIHYDROGEN
26
1.5.4
FUNCTIONALIZATION
OF
TRANSITION
METAL-BOUND
DINITROGEN
29
1.5.5
ELECTROCHEMICAL
AND
PHOTOCHEMICAL
CONVERSION
OF
DINITROGEN
USING
TRANSITION
METAL
COMPLEXES
31
1.6
CATALYTIC
CONVERSION
OF
DINITROGEN
INTO
AMMONIA
USING
TRANSITION
METAL
COMPLEXES
34
1.6.1
CATALYTIC
FORMATION
OF
AMMONIA
OR
HYDRAZINE
USING
MOLYBDENUM
COMPLEXES
34
1.6.2
CATALYTIC
FORMATION
OF
AMMONIA
OR
HYDRAZINE
USING
TRANSITION
METAL
OTHER
THAN
MOLYBDENUM
(IRON,
RUTHENIUM,
OSMIUM,
COBALT,
AND
VANADIUM)
COMPLEXES
40
1.6.3
CATALYTIC
TRANSFORMATION
OF
HYDRAZINE
INTO
AMMONIA
45
1.6.4
CATALYTIC
FORMATION
OF
SILYLAMINE
47
1.7
CONCLUSION
AND
PERSPECTIVES
50
REFERENCES
51
2
GROUP
4
TRANSITION
METAL-DINITROGEN
COMPLEXES
79
HIDETAKE
SEINO
AND
YUJI
KAJITA
2.1
2.2
INTRODUCTION
79
PREPARATION OF
GROUP
4
TRANSITION
METAL-DINITROGEN
COMPLEXES
80
2.2.1
DINITROGEN
COMPLEXES
OF
BIS(CYCLOPENTADIENYL)TITANIUM
DERIVATIVES
80
2.2.2
DINITROGEN
COMPLEXES
OF
BIS(CYCLOPENTADIENYL)ZIRCONIUM
AND
BIS(CYCLOPENTADIENYL)HAFNIUM
DERIVATIVES
89
2.2.3
OTHER
DINITROGEN
COMPLEXES
BASED
ON
CYCLOPENTADIENYL
LIGANDS
98
2.2.4
2.2.5
2.3
2.3.1
2.3.2
2.3.3
2.3.4
2.3.5
2.3.6
2.3.7
2.3.8
2.3.9
2.4
2.5
DINITROGEN
COMPLEXES
SUPPORTED
BY
O-DONOR
LIGANDS
100
HETEROBIMETALLIC
DINITROGEN
COMPLEXES
109
REACTIONS
OF
GROUP
4
TRANSITION
METAL-DINITROGEN
COMPLEXES
112
PROTONATION
112
REDUCTION
115
REACTIONS
WITH
HYDROGEN
120
REACTIONS
WITH
SI
*
H
AND
B
*
H
BONDS
129
REACTIONS
WITH
ALKYL
HALIDES
AND
THEIR
EQUIVALENTS
131
REACTIONS
WITH
ALKYNES
136
REACTIONS
WITH CARBON
DIOXIDE
AND
CUMULENES
138
REACTIONS
WITH
CARBON
MONOXIDE
142
DINITROGEN
LIGAND
SUBSTITUTION
148
CONCLUSION
AND
PERSPECTIVES
151
ADDITION
AFTER
ACCEPTANCE
OF
THIS
MANUSCRIPT
151
REFERENCES
152
3
GROUP
5
TRANSITION
METAL-DINITROGEN
COMPLEXES
159
LEILA
M.
DUMAN
AND
LAWRENCE
R.
SITA
3.1
3.2
3.2.1
3.2.2
3.2.3
3.3
3.3.1
3.3.2
3.3.3
3.4
INTRODUCTION
159
PREPARATION
OF
GROUP
5
METAL
N
2
COMPLEXES
160
VANADIUM
160
NIOBIUM
174
TANTALUM
178
N=N
BOND
CLEAVAGE
WITHIN
GROUP
5
METAL
N
2
COMPLEXES
187
VANADIUM
188
NIOBIUM
192
TANTALUM
197
NITROGEN
FIXATION
MEDIATED
BY
GROUP
5
TRANSITION-METAL
N
2
COMPLEXES
201
3.4.1
3.4.2
3.4.3
3.5
3.6
VANADIUM
202
NIOBIUM
204
TANTALUM
206
CPAM
GROUP
5
BIMETALLIC
(P-QLQI-N
2
)
COMPLEXES
206
CONCLUSIONS
AND
PERSPECTIVES
212
REFERENCES
214
4
GROUP
6
TRANSITION
METAL-DINITROGEN
COMPLEXES
221
NICOLAS
MEZAILLES
4.1
4.2
4.2.1
4.2.1.1
4.2.1.2
4.2.1.3
4.2.2
INTRODUCTION
221
PREPARATION
OF
GROUP
6
TRANSITION
METAL-DINITROGEN
COMPLEXES
222
END-ON
DINITROGEN
COMPLEXES
FROM
N
2
222
ARENE
AND
PHOSPHINE
LIGANDS
222
THIOETHER
LIGANDS
226
NITROGEN
AND
CP
LIGANDS
226
END-ON
BRIDGING
DINITROGEN
COMPLEXES
FROM
N
2
:
SYNTHESIS
AND
N
2
SPLITTING
228
4.3
STOICHIOMETRIC
REACTIONS
OF
GROUP
6
TRANSITION
METAL-DINITROGEN
AND
METAL-NITRIDO
COMPLEXES
234
4.3.1
4.3.2
4.3.3
4.4
N
*
H
BOND
FORMATION
234
N
*
C
BOND
FORMATION
238
N-ELEMENT
BOND
FORMATION
241
CATALYTIC
REACTIONS
OF
GROUP
6
TRANSITION
METAL-DINITROGEN
COMPLEXES
247
4.4.1
CATALYTIC
FORMATION OF
N
2
H
4
/NH
3
FROM
NONISOLATED
M-N
2
COMPLEXES
247
4.4.2
4.4.3
4.5
4.6
CATALYTIC
FORMATION OF
N(SIME
3
)
3
247
CATALYTIC
FORMATION
OF
NH
3
251
CHEMISTRY
OF
CR
COMPLEXES
259
CONCLUSION
AND
PERSPECTIVES
261
REFERENCES
263
5
TOWARD
N
*
N
BOND
CLEAVAGE:
SYNTHESIS
AND
REACTIVITY
OF
GROUP
7
DINITROGEN
COMPLEXES
271
ELON
A.
ISON
5.1
5.1.1
5.1.2
5.1.2.1
5.1.2.2
5.2
5.2.1
5.2.2
5.3
SYNTHESIS
OF
GROUP
VII
N
2
COMPLEXES
271
SYNTHESES
OF
TERMINAL
N
2
COMPLEXES
271
REACTIVITY
OF
TERMINAL
N
2
COMPLEXES
275
SYNTHESIS
OF
BRIDGED
N
2
COMPLEXES
BY
REACTION
WITH
LEWIS
ACIDS
276
ALTERNATIVE
SYNTHESES
OF
BRIDGED
N
2
COMPLEXES
279
CLEAVAGE
AND
FUNCTIONALIZATION
OF
N
2
BONDS
280
GENERATION
OF
DIAZOMETHANE
FROM
CPMN(CO)
2
N
2
280
CLEAVAGE
OF
N
2
IN
THE
COORDINATION
SPHERE
OF
RHENIUM
281
CONCLUSIONS
AND
FUTURE
OUTLOOK
281
REFERENCES
282
6
GROUP
8
TRANSITION
METAL-DINITROGEN
COMPLEXES
285
ADAM
D.
PIASCIK
AND
ANDREW
E.
ASHLEY
6.1
6.2
6.2.1
6.2.2
6.2.3
INTRODUCTION
285
PREPARATION
OF
GROUP
8
TRANSITION
METAL-DINITROGEN
COMPLEXES
288
LIGAND
SUBSTITUTION
288
PRECURSOR
REDUCTION
292
OTHER
METHODS
296
6.3
STOICHIOMETRIC
REACTIONS
OF
GROUP
8
TRANSITION
METAL-DINITROGEN
COMPLEXES
297
6.3.1
SUBSTITUTION
REACTIONS
AND
LABILITY
OF
BOUND
N
2
297
6.3.2
CLEAVAGE
AND
FUNCTIONALIZATION
OF
COORDINATED
N
2
301
6.3.3
OTHER
STOICHIOMETRIC
REACTIVITY
309
6.4
CATALYTIC
REACTIONS
OF
GROUP
8
TRANSITION
METAL-DINITROGEN
COMPLEXES
311
6.4.1
EARLY
RESULTS
AND
FE
BIS(DIPHOSPHINE)
SYSTEMS
FOR
CATALYTIC
N
2
FIXATION
311
6.4.2
CATALYTIC
NH
3
PRODUCTION
BY
EP
R
3
-SUPPORTED
SYSTEMS
313
6.4.3
CATALYTIC
N
2
FIXATION
BY
OTHER
SYSTEMS
317
6.4.4
OTHER
CATALYTIC
REACTIONS
OF
GROUP
8
M-N
2
COMPLEXES
31
9
6.5
CONCLUSION
AND
PERSPECTIVES
327
REFERENCES
328
7
GROUP
9
TRANSITION
METAL-DINITROGEN
COMPLEXES
337
CONNIE
C.
LU
AND
STEVEN
D.
PRINSLOW
7.1
COBALT-DINITROGEN
COMPLEXES
337
7.1.1
MONODENTATE
PHOSPHINE
DONORS
338
7.1.1.1
C
O
H(N
2
)(PR
3
)
3
AND
RELATED
CO(I)
COMPLEXES
338
7.1.1.2
COBALTATE
COMPLEXES:
[CO(N
2
)(PR
3
)
3
]~
342
7.1.2
TRIPODAL
POLYPHOSPHINE
LIGANDS
34S
7.1.2.1
TRIS(PHOSPHINE)
LIGANDS
34S
7.1.2.2
TRIS(PHOSPHINO)BORATE
LIGANDS
346
7.1.2.3
TRISPHOSPHINE
SYSTEMS
WITH
AN
APICAL
MAIN
GROUP
DONOR
347
7.1.2.4
TRISPHOSPHINE
SYSTEMS
WITH
AN
APICAL
TRANSITION
METALLOLIGAND
DONOR
350
7.1.3
LIGANDS
WITH
EXCLUSIVELY
NITROGEN
DONORS
355
7.1.3.1
TRIS(PYRAZOYL)BORATE
(TP)
LIGANDS
355
7.1.3.2
P-DIKETIMINATE
LIGANDS
356
7.1.3.3
BIS(A-IMINO)PYRIDINE
LIGANDS
358
7.1.4
TV-HETEROCYCLIC
CARBENE
LIGANDS
359
7.1.5
PINCER
LIGANDS
360
7.1.5.1
MONOANIONIC
PNP-TYPE
AND
PBP-TYPE
LIGANDS
361
7.1.5.2
PINCER
LIGANDS
WITH
N/P
DONORS
363
7.1.5.3
TV-HETEROCYCLIC
CARBENE-BASED
PINCER
LIGANDS
365
7.1.6
OTHER
ASSORTED
LIGANDS
367
7.1.7
ANALYSIS
AND
SUMMARY
OF
COBALT-DINITROGEN
COMPLEXES
369
7.2
RHODIUM-DINITROGEN
COMPLEXES
370
7.2.1
EARLY
RH-N
2
COMPLEXES
370
7.2.2
PHOSPHINE
LIGANDS
372
7.2.3
LIGANDS
WITH
EXCLUSIVELY
NITROGEN
DONORS
374
7.2.3.1
BIS(A-IMINO)PYRIDINE
LIGANDS
374
7.2.3.2
P-DIKETIMINATE
LIGANDS
375
7.2.4
PINCER
LIGANDS
375
7.2.4.1
PCP
PINCER
LIGANDS
376
7.2.4.2
PNP
PINCER
LIGANDS
378
7.2.4.3
OTHER
PINCER
LIGANDS
380
7.2.5
TV-HETEROCYCLIC
CARBENE
LIGANDS
380
7.2.6
SUMMARY
OF
RHODIUM-DINITROGEN
COMPLEXES
381
7.3
IRIDIUM-DINITROGEN
COMPLEXES
381
7.3.1
EARLY
IR-N
2
COMPLEXES
382
7.3.2
PHOSPHINE
LIGANDS
383
7.3.3
LIGANDS
WITH
EXCLUSIVELY
NITROGEN
DONORS
385
7.3.3.1
TRIS(PYRAZOYL)BORATE
(TP)
LIGANDS
385
7.3.3.2
P-DIKETIMINATE
LIGANDS
386
7.3.4
PINCER
LIGANDS
386
7.3.4.1
PNP-TYPE
PINCER
LIGANDS
386
7.3.4.2
PCP-
AND
PSIP-TYPE
PINCER
LIGANDS
388
7.3.5
TV-HETEROCYCLIC
CARBENE
LIGANDS
390
7.3.6
MISCELLANEOUS
391
7.3.7
SUMMARY
OF
IRIDIUM-DINITROGEN
COMPLEXES
391
7.4
GROUP
9
CATALYSTS
FOR
N
2
FUNCTIONALIZATION
392
7.4.1
COBALT-BASED
CATALYSTS
392
7.4.1.1
DINITROGEN
SILYLATION
393
7.4.1.2
DINITROGEN
FIXATION
395
7.4.2
OUTLOOK
FOR
RHODIUM
AND
IRIDIUM
CATALYSTS
396
ACKNOWLEDGMENTS
396
REFERENCES
396
8
GROUP
10
AND
11
TRANSITION
METAL-DINITROGEN
COMPLEXES
403
RICARDO
B.
FERREIRA
AND
LESLIE
J.
MURRAY
8.1
INTRODUCTION
403
8.2
GROUP
10
TRANSITION
METAL-DINITROGEN
COMPLEXES
405
8.2.1
NICKEL
405
8.2.1.1
INTERACTION
OF
DINITROGEN
WITH
NICKEL
SURFACES
406
8.2.1.2
MATRIX-ASSISTED
ISOLATION
OF
BINARY
OR
TERNARY
COMPOUNDS
406
8.2.1.3
COORDINATION
COMPOUNDS
408
8.2.1.4
STRUCTURAL
RELATIONSHIPS
AND
COMPARISONS
420
8.2.2
PALLADIUM
AND
PLATINUM
422
8.3
GROUP
11
TRANSITION
METAL-DINITROGEN
COMPLEXES
423
8.3.1
COPPER
423
8.3.1.1
MATRIX-ASSISTED
ISOLATION
OF
BINARY
OR
TERNARY
COMPOUNDS
423
8.3.1.2
COORDINATION
COMPOUNDS
425
8.3.1.3
STRUCTURAL
RELATIONSHIPS
AND
COMPARISONS
427
8.3.2
SILVER
AND
GOLD
429
8.4
CONCLUSION
AND
PERSPECTIVES
430
REFERENCES
431
9
GROUP
3
TRANSITION
METAL,
LANTHANIDE,
AND
ACTINIDE-DINITROGEN
COMPLEXES
441
YOSHIAKI
TANABE
9.1
INTRODUCTION
441
9.2
PREPARATION
AND
CHARACTERIZATION OF
GROUP
3
TRANSITION
METAL,
LANTHANIDE,
AND
ACTINIDE-DINITROGEN
COMPLEXES
443
9.2.1
OVERVIEWS
OF
PREPARATION,
STRUCTURES,
AND
CHARACTERIZATION
OF
GROUP
3
TRANSITION
METAL,
LANTHANIDE,
AND
ACTINIDE-DINITROGEN
COMPLEXES
443
9.2.2
PREPARATION
AND
STRUCTURES
OF
SIDE-ON-BOUND
{(N
2
)
2
}-BRIDGED
DINUCLEAR
GROUP
3
TRANSITION
METAL,
LANTHANIDE,
AND
ACTINIDE-DINITROGEN
COMPLEXES
443
9.2.3
PREPARATION
AND
STRUCTURES
OF
SIDE-ON-BOUND
{(N
2
)
3
*
{-BRIDGED
DINUCLEAR
GROUP
3
TRANSITION METAL
AND
LANTHANIDE
COMPLEXES
456
9.2.4
PREPARATION
AND
STRUCTURES
OF
{(N
2
)
4
*
}-BRIDGED
DINUCLEAR,
TRINUCLEAR,
AND
TETRANUCLEAR
LANTHANIDE
AND
ACTINIDE-DINITROGEN
COMPLEXES
457
9.2.5
PREPARATION
AND
STRUCTURES
OF
END-ON-BOUND
GROUP
3
TRANSITION
METAL,
LANTHANIDE,
AND
ACTINIDE-DINITROGEN
COMPLEXES
460
9.3
REACTIVITY
AND
PROPERTY
OF
GROUP
3
TRANSITION
METAL,
LANTHANIDE,
AND
ACTINIDE-DINITROGEN
COMPLEXES
462
9.3.1
CLEAVAGE,
PROTONATION,
AND
FUNCTIONALIZATION
OF
DINITROGEN
UPON
GROUP
3
TRANSITION
METAL,
LANTHANIDE,
AND
ACTINIDE-DINITROGEN
COMPLEXES
462
9.3.2
GROUP
3
TRANSITION
METAL-DINITROGEN
COMPLEXES
AS
MEDIATORS
FOR
THE
TRANSFORMATION
OF
SMALL
MOLECULES
466
9.3.3
{(N
2
)
3
}-BRIDGED
DINUCLEAR
GROUP
3
TRANSITION
METAL
AND
LANTHANIDE
COMPLEXES
AS
SINGLE-MOLECULE
MAGNETS
468
9.4
CONCLUSION
AND
PERSPECTIVES
469
REFERENCES
470
INDEX
475
|
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| author2 | Nishibayashi, Yoshiaki 1968- |
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| ctrlnum | (OCoLC)1091654673 (DE-599)DNB1165248611 |
| discipline | Chemie / Pharmazie |
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| genre_facet | Aufsatzsammlung |
| id | DE-604.BV045503315 |
| illustrated | Illustrated |
| indexdate | 2024-07-10T08:19:54Z |
| institution | BVB |
| institution_GND | (DE-588)16179388-5 |
| isbn | 9783527344253 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-030887980 |
| oclc_num | 1091654673 |
| open_access_boolean | |
| owner | DE-29T DE-11 |
| owner_facet | DE-29T DE-11 |
| physical | XIII, 481 Seiten Illustrationen, Diagramme |
| publishDate | 2019 |
| publishDateSearch | 2019 |
| publishDateSort | 2019 |
| publisher | Wiley-VCH |
| record_format | marc |
| spelling | Transition metal-dinitrogen complexes preparation and reactivity edited by Yoshiaki Nishibayashi Weinheim Wiley-VCH [2019] © 2019 XIII, 481 Seiten Illustrationen, Diagramme txt rdacontent n rdamedia nc rdacarrier Stickstofffixierung (DE-588)4183273-5 gnd rswk-swf Übergangsmetallkomplexe (DE-588)4131837-7 gnd rswk-swf Biochemie Biochemie u. Chemische Biologie Catalysis Chemie Chemistry Coordination Chemistry Katalyse Koordinationschemie (DE-588)4143413-4 Aufsatzsammlung gnd-content Übergangsmetallkomplexe (DE-588)4131837-7 s Stickstofffixierung (DE-588)4183273-5 s DE-604 Nishibayashi, Yoshiaki 1968- (DE-588)1158503199 edt Wiley-VCH (DE-588)16179388-5 pbl Erscheint auch als Online-Ausgabe, ePDF 978-3-527-34429-1 Erscheint auch als Online-Ausgabe, ePub 978-3-527-34427-7 Erscheint auch als Online-Ausgabe, oBook 978-3-527-34426-0 X:MVB http://www.wiley-vch.de/publish/dt/books/ISBN978-3-527-34425-3/ DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030887980&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Transition metal-dinitrogen complexes preparation and reactivity Stickstofffixierung (DE-588)4183273-5 gnd Übergangsmetallkomplexe (DE-588)4131837-7 gnd |
| subject_GND | (DE-588)4183273-5 (DE-588)4131837-7 (DE-588)4143413-4 |
| title | Transition metal-dinitrogen complexes preparation and reactivity |
| title_auth | Transition metal-dinitrogen complexes preparation and reactivity |
| title_exact_search | Transition metal-dinitrogen complexes preparation and reactivity |
| title_full | Transition metal-dinitrogen complexes preparation and reactivity edited by Yoshiaki Nishibayashi |
| title_fullStr | Transition metal-dinitrogen complexes preparation and reactivity edited by Yoshiaki Nishibayashi |
| title_full_unstemmed | Transition metal-dinitrogen complexes preparation and reactivity edited by Yoshiaki Nishibayashi |
| title_short | Transition metal-dinitrogen complexes |
| title_sort | transition metal dinitrogen complexes preparation and reactivity |
| title_sub | preparation and reactivity |
| topic | Stickstofffixierung (DE-588)4183273-5 gnd Übergangsmetallkomplexe (DE-588)4131837-7 gnd |
| topic_facet | Stickstofffixierung Übergangsmetallkomplexe Aufsatzsammlung |
| url | http://www.wiley-vch.de/publish/dt/books/ISBN978-3-527-34425-3/ http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030887980&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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