Equilibria and dynamics of gas adsorption on heterogeneous solid surfaces

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Veröffentlicht: Amsterdam Elsevier 1997
Schriftenreihe:Studies in surface science and catalysis 104
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500 |a The fact that the surfaces of real solids are geometrically distorted and chemically non-uniform has long been realized by the scientists investigating various phenomena occurring on solid surfaces. Even in the case when diffraction experiments show a well-organized bulk solid structure, the surface atoms or molecules will usually exhibit a much smaller degree of surface organization. In addition to the results obtained from electron diffraction, this can be seen in the impressive images obtained from STM and AFM microscopies. This geometric and chemical disorder is the source of the energetic heterogeneity for molecules adsorbing on real solid surfaces. Hundreds of papers have been published showing that this heterogeneity is a major factor in determining the behaviour of real adsorption systems. Studies of adsorption on energetically heterogeneous surfaces have proceeded along three somewhat separate paths, with only minor coupling of ideas. One was the study of adsorption equilibria on heterogeneous solid surfaces. The second path was the study of time evolution of adsorption processes such as surface diffusion or adsorption-desorption kinetics on heterogeneous surfaces, and the third was the study of adsorption in porous solids, or more generally, adsorption in systems with limited dimensions. The present monograph is a first attempt to provide a synthesis of the ways that surface geometric and energetic heterogeneities affect both the equilibria and the time evolution of adsorption on real solids. The book contains 17 chapters written by a team of internationally recognized specialists, some of whom have already published books on adsorption 
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spelling Equilibria and dynamics of gas adsorption on heterogeneous solid surfaces editors, W. Rudziński, W.A. Steele, G. Zgrablich
Amsterdam Elsevier 1997
1 Online-Ressource (xviii, 890 p.)
txt rdacontent
c rdamedia
cr rdacarrier
Studies in surface science and catalysis 104
The fact that the surfaces of real solids are geometrically distorted and chemically non-uniform has long been realized by the scientists investigating various phenomena occurring on solid surfaces. Even in the case when diffraction experiments show a well-organized bulk solid structure, the surface atoms or molecules will usually exhibit a much smaller degree of surface organization. In addition to the results obtained from electron diffraction, this can be seen in the impressive images obtained from STM and AFM microscopies. This geometric and chemical disorder is the source of the energetic heterogeneity for molecules adsorbing on real solid surfaces. Hundreds of papers have been published showing that this heterogeneity is a major factor in determining the behaviour of real adsorption systems. Studies of adsorption on energetically heterogeneous surfaces have proceeded along three somewhat separate paths, with only minor coupling of ideas. One was the study of adsorption equilibria on heterogeneous solid surfaces. The second path was the study of time evolution of adsorption processes such as surface diffusion or adsorption-desorption kinetics on heterogeneous surfaces, and the third was the study of adsorption in porous solids, or more generally, adsorption in systems with limited dimensions. The present monograph is a first attempt to provide a synthesis of the ways that surface geometric and energetic heterogeneities affect both the equilibria and the time evolution of adsorption on real solids. The book contains 17 chapters written by a team of internationally recognized specialists, some of whom have already published books on adsorption
Includes bibliographical references and indexes
Adsorption fast
Gas-solid interfaces fast
Surface chemistry fast
Surface chemistry
Adsorption
Gas-solid interfaces
Rudziński, Władysław 1942- Sonstige (DE-588)172340543 oth
Steele, William A. Sonstige oth
Zgrablich, G. Sonstige oth
http://www.sciencedirect.com/science/book/9780444822437 Verlag Volltext
spellingShingle Equilibria and dynamics of gas adsorption on heterogeneous solid surfaces
Adsorption fast
Gas-solid interfaces fast
Surface chemistry fast
Surface chemistry
Adsorption
Gas-solid interfaces
title Equilibria and dynamics of gas adsorption on heterogeneous solid surfaces
title_auth Equilibria and dynamics of gas adsorption on heterogeneous solid surfaces
title_exact_search Equilibria and dynamics of gas adsorption on heterogeneous solid surfaces
title_full Equilibria and dynamics of gas adsorption on heterogeneous solid surfaces editors, W. Rudziński, W.A. Steele, G. Zgrablich
title_fullStr Equilibria and dynamics of gas adsorption on heterogeneous solid surfaces editors, W. Rudziński, W.A. Steele, G. Zgrablich
title_full_unstemmed Equilibria and dynamics of gas adsorption on heterogeneous solid surfaces editors, W. Rudziński, W.A. Steele, G. Zgrablich
title_short Equilibria and dynamics of gas adsorption on heterogeneous solid surfaces
title_sort equilibria and dynamics of gas adsorption on heterogeneous solid surfaces
topic Adsorption fast
Gas-solid interfaces fast
Surface chemistry fast
Surface chemistry
Adsorption
Gas-solid interfaces
topic_facet Adsorption
Gas-solid interfaces
Surface chemistry
url http://www.sciencedirect.com/science/book/9780444822437
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