From non-covalent assemblies to molecular machines
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| 245 | 1 | 0 | |a From non-covalent assemblies to molecular machines |c ed. by Jean-Pierre Sauvage ... |
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CONTENTS
PREFACE XIII LIST OF CONTRIBUTORS XV DESCRIPTION XIX OPENING SESSION XX
THE INTERNATIONAL SOLVAY INSTITUTES XXIII SOLVAY SCIENTIFIC COMMITTEE
FOR CHEMISTRY XXV 21ST SOLVAY CONFERENCE ON CHEMISTRY XXVI
PART ONE NONCOVALENT ASSEMBLIES: DESIGN AND SYNTHESIS I
1 INTRODUCTION AND DEFINITION OF NONCOVALENT ASSEMBLIES 3 JULIUS REBEKJR
REFERENCES 6
2 NONCOVALENT ASSEMBLIES: DESIGN AND SYNTHESIS 7 MAKOTO FUJITA AND
TAKASHI MURASE 2.1 INTRODUCTION 7
2.2 LANDMARKS IN SELF-ASSEMBLY FIELDS 8 2.3 HYDROGEN-BONDED ASSEMBLIES
15 2.4 COORDINATION ASSEMBLIES 17
2.5 FUNCTION THROUGH ARCHITECTURE 21 2.6 CONCLUSIONS 27
REFERENCES 27
3 DISCUSSION 1.A 31
CHAIRMAN:JULIUS REBEKJR
4 NONCOVALENT SYNTHESIS OF MOLECULAR RECEPTORS 35 DAVID N. REINHOUDT 4.1
INTRODUCTION 35
4.2 NONCOVALENT SYNTHESIS 35
4.3 SUPRAMOLECULAR CHIRALITY 38
BIBLIOGRAFISCHE INFORMATIONEN HTTP://D-NB.INFO/1002408156
DIGITALISIERT DURCH
IMAGE 2
VI CONTENTS
4.4 OPTICAL AMPLIFICATION IN DYNAMIC SUPRAMOLECULAR SYSTEMS 40
ACKNOWLEDGMENTS 41 REFERENCES 42
5 CUCURBITURILS: NEW PLAYERS IN NONCOVALENT ASSEMBLY 43 KIMOON KIM
ACKNOWLEDGMENTS 48 REFERENCES 48
6 COMMENT ON THE POSSIBLE PRESENCE OF BUBBLES INSIDE SELF-ASSEMBLED
MOLECULAR CAGES 51 JOSEF M ICH I REFERENCES 56
7 DISCUSSION L.B 57
CHAIRMAN: JULIUS REBEKJR
PART TWO TEMPLATE SYNTHESIS OF CATENANES AND ROTAXANES 65
8 A SHORT HISTORY OF THE MECHANICAL BOND 67 JOHN-CARL OLSEN, KIRSTEN E.
GRIFFITHS, ANDJ. FRASER STODDART 8.1 INTRODUCTION 67
8.1.1 HISTORICAL PERSPECTIVE 69 8.2 DONOR/ACCEPTOR TEMPLATED SYSTEMS 72
8.3 CHARGED HYDROGEN BOND-TEMPLATED SYSTEMS 80 8.3.1 REVERSE RECOGNITION
IN ROTAXANE SYNTHESIS 82 8.3.2 THREADING-FOLLOWED-BY-STOPPERING
PROTOCOLS 83 8.3.3 CLIPPING PROTOCOL 84 8.3.4 SLIPPAGE 86 8.3.5 RING
SHRINKAGE 87 8.3.6 THREADING ACCOMPANIED BY SWELLING 87 8.3.7 OTHER
MECHANICALLY INTERLOCKED MOLECULES 88 8.3.8 MOLECULAR SWITCHES 89 8.4
ANION-TEMPLATED SYNTHESIS 90 8.5 NEUTRAL HYDROGEN BOND-TEMPLATED SYSTEMS
93 8.5.1 CATENANES 94 8.5.2 ROTAXANES 99 8.5.3 NOVEL CATENANE AND
ROTAXANE ARCHITECTURES 103 8.6 METAL-CONTAINING CATENANES AND ROTAXANES
106 8.7 SOLVOPHOBICALLY DRIVEN TEMPLATION 115 8.8 APPLICATIONS 122
8.9 CONCLUSIONS 127
REFERENCES 128
IMAGE 3
CONTENTS VII
9 DISCUSSION 2.A 141
CHAIRMAN: FRITZ VOGLIE
10 DYNAMIC COMBINATORIAL APPROACHES TO CATENANES 147 JEREMY K. M.
SANDERS NOTES ADDED AFTER THE CONFERENCE 149
REFERENCES 249
11 DISCUSSION 2.B 151
CHAIRMAN: FRITZ VOEGTLE
PART THREE MOLECULAR MACHINES BASED ON CATENANES AND ROTAXANES 157
12 MOLECULAR MACHINES BASED ON ROTAXANES AND CATENANES 159 VINCENZO
BALZANI, ALBERTO CREDI, AND MARGHERITA VENTURI 12.1 INTRODUCTION 159
12.2 MOLECULAR MACHINES: HISTORY AND OVERVIEW 260 12.2.1 GENERAL
CONCEPTS 260 12.2.2 NATURAL DEVICES AND MACHINES 161 12.2.3 ARTIFICIAL
MOLECULAR DEVICES AND MACHINES 162
12.2.4 MECHANICAL MOTION IN ARTIFICIAL MOLECULAR-S CALE SYSTEMS 263
12.2.5 ENERGY SUPPLY 265 12.2.5.1 CHEMICAL ENERGY 165 12.2.5.2 LIGHT
ENERGY 265
12.2.5.3 ELECTRICAL ENERGY 166 12.3 MOLECULAR MACHINES BASED ON
ROTAXANES 266 12.3.1 INTRODUCTION I66 12.3.2 CHEMICALLY DRIVEN MOVEMENTS
169 12.3.2.1 ROTAXANES BASED ON MACROCYCLIC CROWN ETHERS 169 12.3.2.2
ROTAXANES BASED ON METAL COMPLEXES 172 12.3.2.3 ROTAXANES BASED ON
CUCURBITURIL AND CYCLODEXTRIN 172 12.3.2.4 OTHER SYSTEMS 274 12.3.3
ELECTROCHEMICALLY DRIVEN MOVEMENTS 175 12.3.3.1 ROTAXANES BASED ON
TETRACATIONIC CYCLOPHANES 275 12.3.3.2 ROTAXANES BASED ON METAL
COMPLEXES 176 12.3.4 PHOTOCHEMICALLY DRIVEN MOVEMENTS 178 12.3.4.1
SYSTEMS BASED ON PHOTOINDUCED ELECTRON TRANSFER 178 12.3.4.2 SYSTEMS
BASED ON PHOTOISOMERIZATION REACTIONS 182 12.3.5 ALLOWING/PREVENTING
RING MOTION 283 12.4 MOLECULAR MACHINES BASED ON CATENANES 187 12.4.1
INTRODUCTION 187
12.4.2 CHEMICALLY DRIVEN PROCESSES 288 12.4.3 ELECTROCHEMICALLY DRIVEN
PROCESSES 189
IMAGE 4
VILI CONTENTS
12.4.4 PHOTOCHEMICALLY DRIVEN PROCESSES 190
12.4.5 UNIDIRECTIONAL RING ROTATION IN CATENANES 292 12.5 PERFORMING
FUNCTIONS WITH MOLECULAR MACHINES 296 12.5.1 BEYOND THE SOLUTION PHASE:
ORDERING AND ADDRESSING 296 12.5.2 MOLECULAR VALVES 197 12.5.3 MOLECULAR
MUSCLES 298
12.5.4 PHOTOINDUCED TRANSPORT OF LIQUID DROPLETS 199 12.5.5 INTERLOCKED
COMPOUNDS IN SOLID-STATE ELECTRONIC DEVICES 200 12.6 PERSPECTIVES 204
ACKNOWLEDGMENTS 205 REFERENCES 206
13 DISCUSSION 3.A 213
CHAIRMAN: DAVID A. LEIGH
14 REARRANGEMENT OF A SURFACE-DEPOSITED [2]CATENANE BY COORDINATION TO
COPPER(L) AT THE SINGLE-MOLECULE LEVEL 219 JEAN-PIERRE SAUVAGE
CONCLUSIONS 222
REFERENCES 222
15 A TOROIDAL OXIDATION CATALYST 225 ALAN E. ROWAN, JOHANNES A.A.W.
ELEMANS, AND ROELANDJ.M . NOLTE REFERENCES 230
16 DISCUSSION 3.B 231
CHAIRMAN: DAVID A. LEIGH
PART FOUR MOLECULAR MACHINES BASED ON NON-INTERLOCKING MOLECULES 242
17 SYNTHETIC MOLECULAR MACHINES BASED ON NON-INTERLOCKED SYSTEMS:
FROM CONCEPT TO APPLICATIONS 243 WESLEY R. BROWNE, DIRK PIJPER, MICHAEL
M. POLLARD, AND BEN L. FERINGA 17.1 INTRODUCTION 243
17.2 DESIGN CONCEPTS 244
17.3 SYNTHETIC MOLECULAR ROTORS 246 17.3.1 METAL COMPLEXES AS ROTORS 246
17.3.2 CORRELATED ROTATION THROUGH STERIC INTERACTIONS 250 17.3.3
MOLECULAR GYROSCOPE IN THE SOLID STATE 253 17.3.4 ROTARY MOTION
CONTROLLED BY AN EXTERNAL INPUT 254 17.3.5 ELECTRICALLY DRIVEN ROTORS
AND MACHINES 256 17.3.6 MOLECULAR ROTATION ON SURFACES 258 17.4
SYNTHETIC MOLECULAR MOTORS AND MACHINES 263 17.4.1 BIASED BROWNIAN
MOTION 264
IMAGE 5
CONTENTS IX
17.4.2 CHEMICALLY DRIVEN MOLECULAR MOTORS 265
17.4.3 LIGHT-DRIVEN MOLECULAR MACHINES BASED ON AZOBENZENES 268 17.4.4
LIGHT-DRIVEN MOLECULAR ROTARY MOTORS 269 17.4.5 SECOND-GENERATION
LIGHT-DRIVEN MOLECULAR MOTORS 272 17.5 MOLECULAR MACHINES: PUTTING
MOTORS TO WORK 274 17.5.1 LIGHT-DRIVEN MACHINES 274
17.5.2 PHOTOCHEMICALLY DRIVEN MECHANICAL CHANGES IN CRYSTALS AND
POLYMERS 276 17.5.3 MOLECULAR MOTORS OPERATING ON SURFACES 279 17.6
MOLECULAR MOTORS AT WORK 282 17.7 CONCLUSIONS AND OUTLOOK 283
REFERENCES 285
18 DISCUSSION 4.A 292
CHAIRMAN: TAKUZO AIDA
19 COMMENT ON MOLECULAR MACHINES BASED ON NON-INTERLOCKING MOLECULES
(OTHER THAN CATENANES AND ROTAXANES) 297 JOSEF MICHL REFERENCES 300
20 A FEW HINTS TOWARDS ARTIFICIAL ACTIVE MACROSCOPIC SYSTEMS 301 JACQUES
PROST 20.1 ACTIVE MOLECULES 301 20.2 ACTIVE GELS 302
20.3 EXPECTED PROPERTIES 304 ACKNOWLEDGMENTS 304 REFERENCES 305
21 FLUCTUATION THEOREM, NONEQUILIBRIUM WORK, AND MOLECULAR MACHINES 307
PIERRE GASPARD
21.1 INTRODUCTION 307
21.2 FLUCTUATION THEOREM 308 21.3 NONEQUILIBRIUM WORK RELATIONS 308 21.4
APPLICATION TO THE F,-ATPASE MOLECULAR MOTOR 309 21.5 PERSPECTIVES 320
21.6 NOTE ADDED AFTER THE CONFERENCE 310 ACKNOWLEDGMENTS 322 REFERENCES
311
22 DISCUSSION 4.B 323
CHAIRMAN: TAKUZO AIDA
IMAGE 6
X CONTENTS
PART FIVE TOWARDS MOLECULAR LOGICS AND ARTIFICIAL PHOTOSYNTHESIS 327
23 CHAIRMAN S COMMENTS 319 A. PRASANNA DE SILVA REFERENCES 320
24 TOWARDS MOLECULAR LOGIC AND ARTIFICIAL PHOTOSYNTHESIS 321 DEVENS
GUST, THOMAS A. MOORE, AND ANA L. MOORE 24.1 INTRODUCTION 321
24.2 ARTIFICIAL PHOTOSYNTHESIS 321 24.2.1 NATURAL PHOTOSYNTHESIS 322
24.2.2 REALIZING ARTIFICIAL PHOTOSYNTHESIS 324 24.2.2.1 MIMICKING THE
REACTION CENTER 324
24.2.2.2 ARTIFICIAL ANTENNA SYSTEMS 333 24.2.2.3 USING THE STORED ENERGY
336 24.3 MOLECULAR LOGIC 337
24.3.1 WHAT IS MOLECULAR LOGIC? 337 24.3.2 SIMPLE SWITCHES 338 24.3.3
CHEMICALLY OPERATED LOGIC GATES 339 24.3.4 PHOTOCHEMICAL LOGIC GATES AND
RELATED DEVICES 340
24.3.5 COMBINATIONS OF LOGIC GATES 343 24.3.6 RECONFIGURABLE MOLECULAR
LOGIC DEVICES 344 24.3.7 ULTRAFAST SWITCHING 346 24.3.8 COMMUNICATION
AMONG MOLECULAR SWITCHES 347
24.3.9 ARE THERE APPLICATIONS FOR MOLECULAR LOGIC? 348 24.4 FINAL
COMMENTS 350
REFERENCES 350
25 DISCUSSION 5.A 355
CHAIRMAN: A. PRASANNA DE SILVA
26 ARTIFICIAL PHOTOSYNTHESIS: OXYGEN EVOLUTION FROM PHOTOCHEMICAL WATER
SPLITTING 361 VINCENZO BALZANI 26.1 INTRODUCTION 361
26.2 OXYGEN EVOLUTION 362 26.3 LESSONS FROM NATURE 363
26.4 PROTON-COUPLED ELECTRON TRANSFER 364 REFERENCES 364
27 POTENTIAL APPLICATIONS OF MOLECULAR LOGIC 367 ALBERTO CREDI 27.1
INTRODUCTION 367
27.2 DISCUSSION 368
ACKNOWLEDGMENTS 373 REFERENCES 374
IMAGE 7
CONTENTS XI
28 DISCUSSION 5.B 377
CHAIRMAN: A. PRASANNA DE SILVA
PART SIX FROM SINGLE MOLECULES TO PRACTICAL DEVICES 379
29 FROM SINGLE MOLECULES TO PRACTICAL DEVICES 382 JEAN-PIERRE LAUNAY
29.1 INTRODUCTION 382
29.2 DEVICES BASED ON MECHANICAL EFFECTS 382 29.2.1 MOLECULES AS TOOLS
ON SURFACES 382 29.2.2 TRANSPORT BY MOLECULES ON SURFACES 382 29.2.3
ROTORS AND MOTORS ON SURFACES 385 29.2.4 GEARS 389
29.2.5 RACKS AND PINIONS ON SURFACES 390 29.2.6 THE CHALLENGE OF
UNIDIRECTIONAL ROTATION (MOSTLY IN SOLUTION) 391 29.2.7 VEHICLES ON
SURFACES 393 29.3 DEVICES BASED ON ELECTRONIC EFFECTS 397
29.3.1 PRELIMINARY: HOW TO CONNECT WIRES TO A SINGLE MOLECULE 398 29.3.2
OVERVIEW OF THE DIFFERENT TRANSPORT REGIMES 400 29.3.3 WIRES 405
29.3.4 CONNECTING ELEMENTS TO METAL ELECTRODES: IMPORTANCE OF THE ATOMIC
PRECISION 408 29.3.5 RECTIFICATION 409 29.3.6 SINGLE ELECTRON STORAGE
411
29.3.7 NEGATIVE DIFFERENTIAL RESISTANCE DEVICES 412 29.3.8
SINGLE-MOLECULE TRANSISTORS 414 29.4 DEVICES BASED ON A COMBINATION OF
MECHANICAL AND ELECTRONIC EFFECTS 426
29.4.1 SWITCHES 426 29.4.2 AMPLIFIER WITH C 60 428 29.4.3 MOLECULAR
AMMETER 429
29.4.4 MORSE MANIPULATOR 421 29.4.5 QUANTUM LOGICAL GATE 422 29.5
CONCLUSIONS 424
ACKNOWLEDGMENT 426 REFERENCES 426
30 DISCUSSION 6.A 429
CHAIRMAN: ENRICO DALCANALE
31 A SPRING-LOADED DEVICE 435 DARIUSH AJAMI AND JULIUS REBEKJR NOTES
AFTER THE CONFERENCE 440 ACKNOWLEDGMENTS 442
REFERENCES 442
IMAGE 8
XII CONTENTS
32 FROM ELECTROCHEMICALLY-DRIVEN CONFORMATIONAL POLYMERIC STATES TO
MACROSCOPIC SENSING AND TACTILE MUSCLES 443 TORIBIO F. OTERO REFERENCES
452
33 CONTROLLING SELF-ASSEMBLY IN SPACE AND TIME 453 BEN L. FERINGA 33.1
INTRODUCTION 453
33.2 LOW-MOLECULAR-WEIGHT GELATORS 453 33.3 DYNAMIC CONTROL OF GELATION
455 33.4 CONCLUDING REMARKS 460 REFERENCES 460
34 DISCUSSION 6.B 463
CHAIRMAN: ENRICO DALCANALE
INDEX 467
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| id | DE-604.BV036805930 |
| illustrated | Illustrated |
| indexdate | 2024-12-24T00:14:17Z |
| institution | BVB |
| isbn | 9783527322770 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-020722013 |
| oclc_num | 694876303 |
| open_access_boolean | |
| owner | DE-19 DE-BY-UBM DE-11 |
| owner_facet | DE-19 DE-BY-UBM DE-11 |
| physical | XXVIII, 478 S. Ill., graph. Darst. |
| publishDate | 2011 |
| publishDateSearch | 2011 |
| publishDateSort | 2011 |
| publisher | Wiley-VCH |
| record_format | marc |
| spellingShingle | From non-covalent assemblies to molecular machines Molekulare Maschine (DE-588)7515135-2 gnd Catenane (DE-588)4147390-5 gnd Rotaxane (DE-588)4178513-7 gnd |
| subject_GND | (DE-588)7515135-2 (DE-588)4147390-5 (DE-588)4178513-7 |
| title | From non-covalent assemblies to molecular machines |
| title_auth | From non-covalent assemblies to molecular machines |
| title_exact_search | From non-covalent assemblies to molecular machines |
| title_full | From non-covalent assemblies to molecular machines ed. by Jean-Pierre Sauvage ... |
| title_fullStr | From non-covalent assemblies to molecular machines ed. by Jean-Pierre Sauvage ... |
| title_full_unstemmed | From non-covalent assemblies to molecular machines ed. by Jean-Pierre Sauvage ... |
| title_short | From non-covalent assemblies to molecular machines |
| title_sort | from non covalent assemblies to molecular machines |
| topic | Molekulare Maschine (DE-588)7515135-2 gnd Catenane (DE-588)4147390-5 gnd Rotaxane (DE-588)4178513-7 gnd |
| topic_facet | Molekulare Maschine Catenane Rotaxane |
| url | http://deposit.dnb.de/cgi-bin/dokserv?id=3474324&prov=M&dok_var=1&dok_ext=htm http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=020722013&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT sauvagejeanpierre fromnoncovalentassembliestomolecularmachines |