Chemical kinetics of solids
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| Format: | Buch |
| Sprache: | English German |
| Veröffentlicht: |
Weinheim [u.a.]
VCH
1995
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| 245 | 1 | 0 | |a Chemical kinetics of solids |c Hermann Schmalzried |
| 264 | 1 | |a Weinheim [u.a.] |b VCH |c 1995 | |
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Datensatz im Suchindex
| DE-BY-TUM_call_number | 0302/CHE 194f 1995 A 3343 |
|---|---|
| DE-BY-TUM_katkey | 652484 |
| DE-BY-TUM_media_number | 040030110435 |
| _version_ | 1816711712319995904 |
| adam_text | HERMANN SCHMALZRIED CHEMICAL KINETICS OF SOLIDS »TRIFJ Y/VP^ WEINHEIM *
NEW YORK TVLL HJ BASEL * CAMBRIDGE * TOKYO TABLE OF CONTENTS PREFACE V
SYMBOLS AND DEFINITIONS XIII 1 INTRODUCTION 1 1.1 SCOPE 1 1.2 HISTORICAL
REMARKS 6 1.3 FOUR BASIC KINETIC SITUATIONS 10 1.3.1 HOMOGENEOUS
REACTIONS: POINT DEFECT RELAXATION 10 1.3.2 STEADY STATE FLUX OF POINT
DEFECTS IN A BINARY COMPOUND 12 1.3.3 THE KINETICS OF AN INTERFACE
REACTION 14 1.3.4 KINETICS OF COMPOUND FORMATION: A + B = AB 16
REFERENCES 18 2 THERMODYNAMICS OF POINT DEFECTS 19 2.1 INTRODUCTION 19
2.2 THERMODYNAMICS OF CRYSTALS 21 2.2.1 PHENOMENOLOGICAL APPROACH 21
2.2.2 REMARKS ON STATISTICAL THERMODYNAMICS OF POINT DEFECTS 27 2.3 SOME
PRACTICAL ASPECTS OF POINT DEFECT THERMODYNAMICS 31 2.4 POINT DEFECTS IN
SOLID SOLUTIONS 38 2.5 CONCLUSIONS 40 REFERENCES 41 3 ONE- AND
TWO-DIMENSIONAL DEFECTS IN CRYSTALS 43 3.1 INTRODUCTION 43 3.2
DISLOCATIONS 43 3.2.1 STRAIN, STRESS, AND ENERGY 43 3.2.2 KINETIC
EFFECTS DUE TO DISLOCATIONS 48 3.3 GRAIN BOUNDARIES 50 3.3.1 STRUCTURE
AND ENERGY OF GRAIN BOUNDARIES 50 3.3.2 PHASE BOUNDARIES IN SOLIDS 54
3.4 MOBILITY OF DISLOCATIONS, GRAIN BOUNDARIES, AND PHASE BOUNDARIES 57
REFERENCES 60 4 BASIC KINETIC CONCEPTS AND SITUATIONS 61 4.1
INTRODUCTION 61 4.1.1 SYSTEMATICS OF SOLID STATE CHEMICAL PROCESSES 61
VIII TABLE OF CONTENTS 4.2 THE CONCEPTS OF IRREVERSIBLE THERMODYNAMICS
63 4.2.1 STRUCTURE ELEMENT FLUXES 66 4.3 DIFFUSION 68 4.3.1 INTRODUCTION
68 4.3.2 FICKIAN TRANSPORT 70 4.3.3 CHEMICAL DIFFUSION 71 4.4 TRANSPORT
IN LONIC SOLIDS 75 4.4.1 INTRODUCTION 75 4.4.2 TRANSPORT IN BINARY LONIC
CRYSTALS AX 78 4.5 TRANSPORT ACROSS PHASE BOUNDARIES 82 4.5.1
INTRODUCTION. EQUILIBRIUM PHASE BOUNDARIES 82 4.5.2 NON-EQUILIBRIUM
PHASE BOUNDARIES 84 4.6 TRANSPORT IN SEMICONDUCTORS; JUNCTIONS 85 4.6.1
INTRODUCTION 85 4.6.2 THE (P-N) JUNCTION 86 4.7 BASIC RATE EQUATIONS FOR
HOMOGENEOUS REACTIONS 88 4.7.1 INTRODUCTION 88 4.7.2 RATE EQUATIONS 89
REFERENCES 93 5 KINETICS AND DYNAMICS. LOCAL EQUILIBRIUM 95 5.1
INTRODUCTION 95 5.1.1 LINEAR RESPONSE 99 5.1.2 TRANSITION STATE 101
5.1.3 BROWNIAN MOTION 103 5.2 KINETIC PARAMETERS AND DYNAMICS 107 5.2.1
PHENOMENOLOGICAL COEFFICIENTS AND KINETIC THEORY 107 5.2.2 CORRELATION
OF ATOMIC JUMPS 109 5.2.3 CONDUCTIVITY OF LONIC CRYSTALS: FREQUENCY
DEPENDENCE 112 5.2.4 DIFFUSIVE MOTION AND PHONONS 116 5.3 RELAXATION OF
IRREGULAER STRUCTURE ELEMENTS 117 5.3.1 INTRODUCTION 117 5.3.2 RELAXATION
OF STRUCTURE ELEMENTS IN NONSTOICHIOMETRIC COMPOUNDS A^O 118 5.3.3
RELAXATION OF INTRINSIC DISORDER 119 5.4 DEFECT EQUILIBRATION DURING
INTERDIFFUSION 123 5.4.1 THE ATOMISTICS OF INTERDIFFUSION 123 5.4.2 THE
KIRKENDALL EFFECT 125 5.4.3 LOCAL DEFECT EQUILIBRATION DURING
INTERDIFFUSION 127 5.4.4 INTERDIFFUSION OF HETEROVALENT COMPOUNDS 133
REFERENCES 135 6 HETEROGENEOUS SOLID STATE REACTIONS 137 6.1
INTRODUCTION 137 TABLE OF CONTENTS IX 6.2 NUCLEATION AND INITIAL GROWTH
138 6.2.1 INTRODUCTORY REMARKS 138 6.2.2 NUCLEATION KINETICS 140 6.2.3
EARLY GROWTH 143 6.3 COMPOUND FORMATION 146 6.3.1 FORMATION KINETICS OF
DOUBLE SALTS 146 6.3.2 FORMATION OF MULTIPHASE PRODUCTS 153 6.4
DISPLACEMENT REACTIONS 155 6.5 POWDER REACTIONS 157 6.5.1 GENERAL 157
6.5.2 SELF-PROPAGATING EXOTHERMIC POWDER REACTIONS 158 6.6 INTERFACE
RATE CONTROL 160 6.7 THERMAL DECOMPOSITION OF SOLIDS 162 REFERENCES 163
7 OXIDATION OF METALS 165 7.1 INTRODUCTION 165 7.2 WAGNER S THEORY OF
METAL OXIDATION 166 7.3 NON-PARABOLIC RATE LAWS 171 7.4 ALLOY OXIDATION
175 7.4.1 THE MORPHOLOGICAL STABILITY OF BOUNDARIES DURING METAL
OXIDATION 176 7.5 SOME PRACTICAL ASPECTS OF HIGH TEMPERATURE CORROSION
179 REFERENCES 181 8 SOLIDS IN THERMODYNAMIC POTENTIAL GRADIENTS 183 8.1
INTRODUCTION 183 8.2 MULTICOMPONENT SOLIDS IN CHEMICAL POTENTIAL
GRADIENTS 184 8.3 KINETIC DECOMPOSITION OF COMPOUNDS IN CHEMICAL
POTENTIAL GRADIENTS 189 8.4 CROSS EFFECTS 191 8.5 DEMIXING UNDER
NON-HYDROSTATIC STRESS 198 8.6 DEMIXING IN TEMPERATURE GRADIENTS
(LUDWIG-SORET EFFECT) 200 8.7 DEMIXING IN MULTIPHASE SYSTEMS 202 8.8
MULTIPHASE SYSTEMS IN ELECTRIC FIELDS 204 REFERENCES 207 9 INTERNAL
REACTIONS 209 9.1 INTRODUCTION 209 9.2 INTERNAL OXIDATION OF METALS 211
9.3 INTERNAL REACTIONS IN NONMETALLIC SYSTEMS 213 9.3.1 INTERNAL
OXIDATION IN NONMETALLIC SOLID SOLUTIONS 213 9.3.2 INTERNAL REDUCTION IN
NONMETALLIC SOLUTIONS 217 X TABLE OF CONTENTS 9.4 INTERNAL REACTIONS
DRIVEN BY OTHER THAN CHEMICAL POTENTIAL GRADIENTS 220 9.4.1 INTERNAL
REACTIONS IN HETEROPHASE ASSEMBLAGES 221 9.4.2 INTERNAL REACTIONS IN
INHOMOGENEOUS SYSTEMS WITH VARYING DISORDER TYPES 222 9.4.3 FORMAL
TREATMENT OF ELECTROCHEMICAL INTERNAL REACTIONS 226 9.5 INTERNAL
REACTIONS A + B = AB IN CRYSTAL C AS SOLVENT 229 9.5.1 THE INTERNAL
REACTION AO + B0 2 = AB0 3 229 9.6 INTERNAL REACTIONS DURING
INTERDIFFUSION 231 REFERENCES 233 10 REACTIONS AT AND ACROSS INTERFACES
235 10.1 INTRODUCTION 235 10.2 SOME FUNDAMENTAL ASPECTS OF INTERFACE
THERMODYNAMICS 236 10.3 STATIC INTERFACES 244 10.4 MOVING INTERFACES 250
10.4.1 GENERAL REMARKS 250 10.4.2 INTERFACE MOTION DURING PHASE
TRANSFORMATION 252 10.4.3 INTERFACE MOVEMENT DURING THE HETEROGENEOUS
REACTION A + B = AB 257 10.4.4 THE DRAGGED BOUNDARY (GENERALIZED SOLUTE
DRAG) 258 10.4.5 DIFFUSION INDUCED GRAIN BOUNDARY MOTION 260 10.5
MORPHOLOGICAL QUESTIONS 261 10.6 THE ATOMIC STRUCTURE OF MOVING
INTERFACES 262 REFERENCES 264 11 MORPHOLOGY 265 11.1 INTRODUCTION 265
11.2 INTERFACE STABILITY 267 11.2.1 QUALITATIVE DISCUSSION 267 11.2.2
EXAMPLES OF UNSTABLE MOVING INTERFACES 273 11.2.3 FORMAL STABILITY
ANALYSIS 277 11.2.4 STABILIZING FACTORS 282 11.2.5 STABILITY AND THE
REACTION PATH 282 11.3 MOVING BOUNDARIES IN OTHER THAN CHEMICAL FIELDS
285 11.4 NON-MONOTONOUS BEHAVIOR IN TIME 288 REFERENCES 290 12 PHASE
TRANSFORMATIONS 291 12.1 INTRODUCTION 291 12.2 NONDIFFUSIVE
TRANSFORMATIONS 296 12.2.1 MARTENSITIC TRANSFORMATIONS 296 12.2.2
SECOND-ORDER TRANSFORMATIONS 298 TABLE OF CONTENTS 12.3 DIFFUSIVE
TRANSFORMATIONS 304 12.3.1 FIRST-ORDER TRANSFORMATION WITH SMALL
COMPOSITION CHANGES 305 12.3.2 SPINODAL DECOMPOSITION 308 REFERENCES 312
13 REACTIONS IN SOLIDS UNDER IRRADIATION 315 13.1 INTRODUCTION 315 13.2
PARTICLE IRRADIATION 317 13.2.1 BASIC CONCEPTS 317 13.2.2 RADIATION
EFFECTS IN HALIDES (RADIOLYSIS) 320 13.2.3 RADIATION EFFECTS IN METALS
321 13.3 PHOTON IRRADIATION 324 13.3.1 BASIC CONCEPTS 324 13.3.2
RADIATION EFFECTS IN HALIDES (PHOTOLYSIS) 326 13.3.3 AG BASED
PHOTOGRAPHY 327 REFERENCES 328 14 INFLUENCE OF MECHANICAL STRESS 331
14.1 INTRODUCTION 331 14.2 THERMODYNAMIC CONSIDERATIONS 332 14.2.1
THERMODYNAMICS OF STRESSED SOLIDS 332 14.2.2 THERMODYNAMICS OF STRESSED
SOLIDS WITH ONLY IMMOBILE COMPONENTS 335 14.3 TRANSPORT IN STRESSED
SOLIDS 336 14.3.1 INTRODUCTORY REMARKS 336 14.3.2 THE INFLUENCE OF
STRESS ON HETEROGENEOUS REACTIONS A + B = AB 14.3.3 TRANSPORT IN
INHOMOGENEOUSLY STRESSED CRYSTALS 338 14.4 CREEP AND FRACTURE 342 14.4.1
INTRODUCTORY REMARKS 342 14.4.2 CREEP 342 14.4.3 FRACTURE 347 14.4.4
TOUGHENING OF CRYSTALS BY PHASE TRANSFORMATIONS 349 14.5 TRIBOCHEMISTRY
351 REFERENCES 353 15 TRANSPORT AND REACTIONS IN SPECIAL SYSTEMS 355
15.1 INTRODUCTION 355 15.2 SILICATES 356 15.2.1 INTRODUCTORY REMARKS 356
15.2.2 TRANSPORT IN SILICATES 357 15.2.3 ORDER-DISORDER REACTIONS 363
15.2.4 THE ROLE OF HYDROGEN IN SILICATES 364 15.2.5 SILICATE GLASSES 365
XII TABLE OF CONTENTS 15.3 FAST ION CONDUCTORS 368 15.3.1 INTRODUCTORY
REMARKS 368 15.3.2 HALIDES 370 15.3.3 AG 2 S (AG 2 SE, AG 2 TE) 372
15.3.4 OXIDES: STABILIZED ZIRCONIA 374 15.3.5 SS-ALUMINA 377 15.3.6
PROTON CONDUCTORS 379 15.4 HYDRIDES 380 15.4.1 INTRODUCTORY REMARKS 380
15.4.2 PHASE EQUILIBRIA 382 15.4.3 KINETICS OF HYDRIDE FORMATION AND
DECOMPOSITION 383 15.5 MOLECULAR (ORGANIC) CRYSTALS 386 15.5.1
INTRODUCTORY REMARKS 386 15.5.2 DIFFUSION IN MOLECULAR CRYSTALS 388
15.5.3 CONDUCTING POLYMERS 389 REFERENCES 391 16 APPENDIX: EXPERIMENTAL
METHODS FOR IN-SITU INVESTIGATIONS 16.1 INTRODUCTION 393 16.2
THERMOGRAVIMETRY, -MANOMETRY, -VOLUMETRY, -ANALYSIS 395 16.2.1
THERMOGRAVIMETRY 395 16.2.2 THERMOMANOMETRY, THERMOVOLUMETRY 396 16.2.3
THERMAL ANALYSIS 397 16.3 ELECTROCHEMICAL MEASUREMENTS 398 16.3.1
INTRODUCTORY REMARKS 398 16.3.2 CHEMICAL POTENTIAL SENSORS 399 16.4
SPECTROSCOPIC METHODS: NUCLEAR SPECTROSCOPY 402 16.4.1 INTRODUCTION 402
16.4.2 PHYSICAL BACKGROUND 404 16.4.3 IN-SITU APPLICATION, EXAMPLES 408
16.5 SPECTROSCOPIC METHODS: ELECTROMAGNETIC SPECTROSCOPY (IR, VIS, UV,
X-RAY) 412 16.5.1 INTRODUCTION 412 16.5.2 PHYSICAL BACKGROUND 412 16.5.3
IN-SITU APPLICATION, EXAMPLES 413 16.6 PARTICLE SPECTROSCOPY 415 16.6.1
INTRODUCTION 415 16.6.2 PHYSICAL BACKGROUND 416 16.6.3 EXAMPLES 417
REFERENCES 419 EPILOGUE 421 SUBJECT INDEX 423 AUTHOR INDEX 431
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| id | DE-604.BV010162441 |
| illustrated | Illustrated |
| indexdate | 2024-11-25T17:14:19Z |
| institution | BVB |
| isbn | 352729094X |
| language | English German |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-006748848 |
| oclc_num | 31661771 |
| open_access_boolean | |
| owner | DE-355 DE-BY-UBR DE-29T DE-703 DE-384 DE-91G DE-BY-TUM DE-20 DE-634 DE-19 DE-BY-UBM DE-83 DE-11 DE-188 |
| owner_facet | DE-355 DE-BY-UBR DE-29T DE-703 DE-384 DE-91G DE-BY-TUM DE-20 DE-634 DE-19 DE-BY-UBM DE-83 DE-11 DE-188 |
| physical | XVI, 433 S. Ill., zahlr. graph. Darst. |
| publishDate | 1995 |
| publishDateSearch | 1995 |
| publishDateSort | 1995 |
| publisher | VCH |
| record_format | marc |
| spellingShingle | Schmalzried, Hermann 1932- Chemical kinetics of solids Dynamica gtt Vaste stoffen gtt Chemical kinetics Solid state chemistry Festkörper (DE-588)4016918-2 gnd Reaktionskinetik (DE-588)4048655-2 gnd |
| subject_GND | (DE-588)4016918-2 (DE-588)4048655-2 |
| title | Chemical kinetics of solids |
| title_auth | Chemical kinetics of solids |
| title_exact_search | Chemical kinetics of solids |
| title_full | Chemical kinetics of solids Hermann Schmalzried |
| title_fullStr | Chemical kinetics of solids Hermann Schmalzried |
| title_full_unstemmed | Chemical kinetics of solids Hermann Schmalzried |
| title_short | Chemical kinetics of solids |
| title_sort | chemical kinetics of solids |
| topic | Dynamica gtt Vaste stoffen gtt Chemical kinetics Solid state chemistry Festkörper (DE-588)4016918-2 gnd Reaktionskinetik (DE-588)4048655-2 gnd |
| topic_facet | Dynamica Vaste stoffen Chemical kinetics Solid state chemistry Festkörper Reaktionskinetik |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=006748848&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT schmalzriedhermann chemicalkineticsofsolids |