Effect of electron beam irradiation on EIS and photoelectrochemical performance of electrodeposited nanocrystalline Bi2Te3 thin films
In this research work, we have synthesized nanocrystalline Bi 2 Te 3 thin films for photoelectrochemical (PEC) solar cell application by potentiostatic electrodeposition method on stainless steel substrates. Subsequently films were irradiated with electron beam irradiation (EBI) of energy 4.5 MeV at...
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| Veröffentlicht in: | Journal of materials science. Materials in electronics 2021-08, Vol.32 (15), p.20031-20046 |
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| creator | Thorat, Jayavant B. Harale, Namdev S. Dhole, Indrajeet A. Shinde, S. K. Rath, M. C. Shinde, Tukaram J. Shinde, Nitin S. Fulari, Vijay J. |
| description | In this research work, we have synthesized nanocrystalline Bi
2
Te
3
thin films for photoelectrochemical (PEC) solar cell application by potentiostatic electrodeposition method on stainless steel substrates. Subsequently films were irradiated with electron beam irradiation (EBI) of energy 4.5 MeV at various doses of irradiation ranging from 10 to 50 kGy. The experimental results showed that synthesized Bi
2
Te
3
thin films having polycrystalline nature and rhombohedral crystal structure with momentous morphological digression through various doses of irradiation. The electrochemical active surface area (ECSA) and photoelectrochemical (PEC) performance of Bi
2
Te
3
thin films were improved well at irradiation dose of 40 kGy. The calculated values of photoconversion efficiency and fill factor for Bi
2
Te
3
thin film were found to be 0.1837% and 0.5383, respectively. The values of photoconversion efficiency and fill factor of same electrode before irradiation have values 0.0987% and 0.3979, respectively. The enhancement in efficiency and fill factor due to EBI were found 53% and 74%, respectively. The enhancement in PEC properties is due to increased active surface area of the Bi
2
Te
3
films after irradiation dose. The results showed that, EBI are capable to strengthen the quality of electrode for PEC solar cell application. |
| doi_str_mv | 10.1007/s10854-021-06290-x |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_webof</sourceid><recordid>TN_cdi_webofscience_primary_000675367700004</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2556905405</sourcerecordid><originalsourceid>FETCH-LOGICAL-c270t-a217bb5258e2ae6703fdac462d4bbb9d650db9080bb11d50fbbdf726d6f12fa33</originalsourceid><addsrcrecordid>eNqNkc9qFTEUh4MoeK2-gKuASxk9yUySmaVebrVQcGEFdyF_vSkzyZjkYvsAvrdpp6grEQI5hO93TvIFoZcE3hAA8bYQGNnQASUdcDpBd_MI7QgTfTeM9OtjtIOJiW5glD5Fz0q5BgA-9OMO_Tx470zFyWM3tyKniLVTCw45KxtUDe2grcPFZ6yixesx1fRAmqNbglEzXl32KS8qGvdXI-vWVEJ1FkcVk8m3pap5DtHh94FeuR7XY4jYh3kpz9ETr-biXjzsZ-jL-eFq_7G7_PThYv_usjNUQO0UJUJrRtnoqHJcQO-tMgOndtBaT5YzsHqCEbQmxDLwWlsvKLfcE-pV35-hV1vfNafvJ1eqvE6nHNtISRnjE7ABWKPoRpmcSsnOyzWHReVbSUDe6Zabbtl0y3vd8qaFXm-hH04nX0xwzcbv4J1vwXouRKtgaPT4__Q-1Pt_2KdTrC3ab9HS8PjN5T9v-Mf1fgHQdqdS</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2556905405</pqid></control><display><type>article</type><title>Effect of electron beam irradiation on EIS and photoelectrochemical performance of electrodeposited nanocrystalline Bi2Te3 thin films</title><source>Web of Science - Science Citation Index Expanded - 2021<img src="https://exlibris-pub.s3.amazonaws.com/fromwos-v2.jpg" /></source><source>SpringerLink Journals - AutoHoldings</source><creator>Thorat, Jayavant B. ; Harale, Namdev S. ; Dhole, Indrajeet A. ; Shinde, S. K. ; Rath, M. C. ; Shinde, Tukaram J. ; Shinde, Nitin S. ; Fulari, Vijay J.</creator><creatorcontrib>Thorat, Jayavant B. ; Harale, Namdev S. ; Dhole, Indrajeet A. ; Shinde, S. K. ; Rath, M. C. ; Shinde, Tukaram J. ; Shinde, Nitin S. ; Fulari, Vijay J.</creatorcontrib><description>In this research work, we have synthesized nanocrystalline Bi
2
Te
3
thin films for photoelectrochemical (PEC) solar cell application by potentiostatic electrodeposition method on stainless steel substrates. Subsequently films were irradiated with electron beam irradiation (EBI) of energy 4.5 MeV at various doses of irradiation ranging from 10 to 50 kGy. The experimental results showed that synthesized Bi
2
Te
3
thin films having polycrystalline nature and rhombohedral crystal structure with momentous morphological digression through various doses of irradiation. The electrochemical active surface area (ECSA) and photoelectrochemical (PEC) performance of Bi
2
Te
3
thin films were improved well at irradiation dose of 40 kGy. The calculated values of photoconversion efficiency and fill factor for Bi
2
Te
3
thin film were found to be 0.1837% and 0.5383, respectively. The values of photoconversion efficiency and fill factor of same electrode before irradiation have values 0.0987% and 0.3979, respectively. The enhancement in efficiency and fill factor due to EBI were found 53% and 74%, respectively. The enhancement in PEC properties is due to increased active surface area of the Bi
2
Te
3
films after irradiation dose. The results showed that, EBI are capable to strengthen the quality of electrode for PEC solar cell application.</description><identifier>ISSN: 0957-4522</identifier><identifier>EISSN: 1573-482X</identifier><identifier>DOI: 10.1007/s10854-021-06290-x</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Bismuth tellurides ; Characterization and Evaluation of Materials ; Chemistry and Materials Science ; Crystal structure ; Efficiency ; Electron beams ; Electron irradiation ; Engineering ; Engineering, Electrical & Electronic ; Food irradiation ; Materials Science ; Materials Science, Multidisciplinary ; Nanocrystals ; Optical and Electronic Materials ; Photovoltaic cells ; Physical Sciences ; Physics ; Physics, Applied ; Physics, Condensed Matter ; Quantum efficiency ; Radiation dosage ; Science & Technology ; Solar cells ; Stainless steels ; Substrates ; Surface area ; Synthesis ; Technology ; Thin films</subject><ispartof>Journal of materials science. Materials in electronics, 2021-08, Vol.32 (15), p.20031-20046</ispartof><rights>The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2021</rights><rights>The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2021.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>true</woscitedreferencessubscribed><woscitedreferencescount>0</woscitedreferencescount><woscitedreferencesoriginalsourcerecordid>wos000675367700004</woscitedreferencesoriginalsourcerecordid><cites>FETCH-LOGICAL-c270t-a217bb5258e2ae6703fdac462d4bbb9d650db9080bb11d50fbbdf726d6f12fa33</cites><orcidid>0000-0002-3829-3879</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10854-021-06290-x$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10854-021-06290-x$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>315,781,785,27929,27930,39263,41493,42562,51324</link.rule.ids></links><search><creatorcontrib>Thorat, Jayavant B.</creatorcontrib><creatorcontrib>Harale, Namdev S.</creatorcontrib><creatorcontrib>Dhole, Indrajeet A.</creatorcontrib><creatorcontrib>Shinde, S. K.</creatorcontrib><creatorcontrib>Rath, M. C.</creatorcontrib><creatorcontrib>Shinde, Tukaram J.</creatorcontrib><creatorcontrib>Shinde, Nitin S.</creatorcontrib><creatorcontrib>Fulari, Vijay J.</creatorcontrib><title>Effect of electron beam irradiation on EIS and photoelectrochemical performance of electrodeposited nanocrystalline Bi2Te3 thin films</title><title>Journal of materials science. Materials in electronics</title><addtitle>J Mater Sci: Mater Electron</addtitle><addtitle>J MATER SCI-MATER EL</addtitle><description>In this research work, we have synthesized nanocrystalline Bi
2
Te
3
thin films for photoelectrochemical (PEC) solar cell application by potentiostatic electrodeposition method on stainless steel substrates. Subsequently films were irradiated with electron beam irradiation (EBI) of energy 4.5 MeV at various doses of irradiation ranging from 10 to 50 kGy. The experimental results showed that synthesized Bi
2
Te
3
thin films having polycrystalline nature and rhombohedral crystal structure with momentous morphological digression through various doses of irradiation. The electrochemical active surface area (ECSA) and photoelectrochemical (PEC) performance of Bi
2
Te
3
thin films were improved well at irradiation dose of 40 kGy. The calculated values of photoconversion efficiency and fill factor for Bi
2
Te
3
thin film were found to be 0.1837% and 0.5383, respectively. The values of photoconversion efficiency and fill factor of same electrode before irradiation have values 0.0987% and 0.3979, respectively. The enhancement in efficiency and fill factor due to EBI were found 53% and 74%, respectively. The enhancement in PEC properties is due to increased active surface area of the Bi
2
Te
3
films after irradiation dose. The results showed that, EBI are capable to strengthen the quality of electrode for PEC solar cell application.</description><subject>Bismuth tellurides</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry and Materials Science</subject><subject>Crystal structure</subject><subject>Efficiency</subject><subject>Electron beams</subject><subject>Electron irradiation</subject><subject>Engineering</subject><subject>Engineering, Electrical & Electronic</subject><subject>Food irradiation</subject><subject>Materials Science</subject><subject>Materials Science, Multidisciplinary</subject><subject>Nanocrystals</subject><subject>Optical and Electronic Materials</subject><subject>Photovoltaic cells</subject><subject>Physical Sciences</subject><subject>Physics</subject><subject>Physics, Applied</subject><subject>Physics, Condensed Matter</subject><subject>Quantum efficiency</subject><subject>Radiation dosage</subject><subject>Science & Technology</subject><subject>Solar cells</subject><subject>Stainless steels</subject><subject>Substrates</subject><subject>Surface area</subject><subject>Synthesis</subject><subject>Technology</subject><subject>Thin films</subject><issn>0957-4522</issn><issn>1573-482X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><sourceid>HGBXW</sourceid><sourceid>AFKRA</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNqNkc9qFTEUh4MoeK2-gKuASxk9yUySmaVebrVQcGEFdyF_vSkzyZjkYvsAvrdpp6grEQI5hO93TvIFoZcE3hAA8bYQGNnQASUdcDpBd_MI7QgTfTeM9OtjtIOJiW5glD5Fz0q5BgA-9OMO_Tx470zFyWM3tyKniLVTCw45KxtUDe2grcPFZ6yixesx1fRAmqNbglEzXl32KS8qGvdXI-vWVEJ1FkcVk8m3pap5DtHh94FeuR7XY4jYh3kpz9ETr-biXjzsZ-jL-eFq_7G7_PThYv_usjNUQO0UJUJrRtnoqHJcQO-tMgOndtBaT5YzsHqCEbQmxDLwWlsvKLfcE-pV35-hV1vfNafvJ1eqvE6nHNtISRnjE7ABWKPoRpmcSsnOyzWHReVbSUDe6Zabbtl0y3vd8qaFXm-hH04nX0xwzcbv4J1vwXouRKtgaPT4__Q-1Pt_2KdTrC3ab9HS8PjN5T9v-Mf1fgHQdqdS</recordid><startdate>20210801</startdate><enddate>20210801</enddate><creator>Thorat, Jayavant B.</creator><creator>Harale, Namdev S.</creator><creator>Dhole, Indrajeet A.</creator><creator>Shinde, S. K.</creator><creator>Rath, M. C.</creator><creator>Shinde, Tukaram J.</creator><creator>Shinde, Nitin S.</creator><creator>Fulari, Vijay J.</creator><general>Springer US</general><general>Springer Nature</general><general>Springer Nature B.V</general><scope>BLEPL</scope><scope>DTL</scope><scope>HGBXW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7SR</scope><scope>8BQ</scope><scope>8FD</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>ARAPS</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>F28</scope><scope>FR3</scope><scope>HCIFZ</scope><scope>JG9</scope><scope>KB.</scope><scope>L7M</scope><scope>P5Z</scope><scope>P62</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>S0W</scope><orcidid>https://orcid.org/0000-0002-3829-3879</orcidid></search><sort><creationdate>20210801</creationdate><title>Effect of electron beam irradiation on EIS and photoelectrochemical performance of electrodeposited nanocrystalline Bi2Te3 thin films</title><author>Thorat, Jayavant B. ; Harale, Namdev S. ; Dhole, Indrajeet A. ; Shinde, S. K. ; Rath, M. C. ; Shinde, Tukaram J. ; Shinde, Nitin S. ; Fulari, Vijay J.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c270t-a217bb5258e2ae6703fdac462d4bbb9d650db9080bb11d50fbbdf726d6f12fa33</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>Bismuth tellurides</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry and Materials Science</topic><topic>Crystal structure</topic><topic>Efficiency</topic><topic>Electron beams</topic><topic>Electron irradiation</topic><topic>Engineering</topic><topic>Engineering, Electrical & Electronic</topic><topic>Food irradiation</topic><topic>Materials Science</topic><topic>Materials Science, Multidisciplinary</topic><topic>Nanocrystals</topic><topic>Optical and Electronic Materials</topic><topic>Photovoltaic cells</topic><topic>Physical Sciences</topic><topic>Physics</topic><topic>Physics, Applied</topic><topic>Physics, Condensed Matter</topic><topic>Quantum efficiency</topic><topic>Radiation dosage</topic><topic>Science & Technology</topic><topic>Solar cells</topic><topic>Stainless steels</topic><topic>Substrates</topic><topic>Surface area</topic><topic>Synthesis</topic><topic>Technology</topic><topic>Thin films</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Thorat, Jayavant B.</creatorcontrib><creatorcontrib>Harale, Namdev S.</creatorcontrib><creatorcontrib>Dhole, Indrajeet A.</creatorcontrib><creatorcontrib>Shinde, S. K.</creatorcontrib><creatorcontrib>Rath, M. C.</creatorcontrib><creatorcontrib>Shinde, Tukaram J.</creatorcontrib><creatorcontrib>Shinde, Nitin S.</creatorcontrib><creatorcontrib>Fulari, Vijay J.</creatorcontrib><collection>Web of Science Core Collection</collection><collection>Science Citation Index Expanded</collection><collection>Web of Science - Science Citation Index Expanded - 2021</collection><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>Advanced Technologies & Aerospace Collection</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>ANTE: Abstracts in New Technology & Engineering</collection><collection>Engineering Research Database</collection><collection>SciTech Premium Collection</collection><collection>Materials Research Database</collection><collection>Materials Science Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Advanced Technologies & Aerospace Database</collection><collection>ProQuest Advanced Technologies & Aerospace Collection</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>DELNET Engineering & Technology Collection</collection><jtitle>Journal of materials science. Materials in electronics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Thorat, Jayavant B.</au><au>Harale, Namdev S.</au><au>Dhole, Indrajeet A.</au><au>Shinde, S. K.</au><au>Rath, M. C.</au><au>Shinde, Tukaram J.</au><au>Shinde, Nitin S.</au><au>Fulari, Vijay J.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Effect of electron beam irradiation on EIS and photoelectrochemical performance of electrodeposited nanocrystalline Bi2Te3 thin films</atitle><jtitle>Journal of materials science. Materials in electronics</jtitle><stitle>J Mater Sci: Mater Electron</stitle><stitle>J MATER SCI-MATER EL</stitle><date>2021-08-01</date><risdate>2021</risdate><volume>32</volume><issue>15</issue><spage>20031</spage><epage>20046</epage><pages>20031-20046</pages><issn>0957-4522</issn><eissn>1573-482X</eissn><abstract>In this research work, we have synthesized nanocrystalline Bi
2
Te
3
thin films for photoelectrochemical (PEC) solar cell application by potentiostatic electrodeposition method on stainless steel substrates. Subsequently films were irradiated with electron beam irradiation (EBI) of energy 4.5 MeV at various doses of irradiation ranging from 10 to 50 kGy. The experimental results showed that synthesized Bi
2
Te
3
thin films having polycrystalline nature and rhombohedral crystal structure with momentous morphological digression through various doses of irradiation. The electrochemical active surface area (ECSA) and photoelectrochemical (PEC) performance of Bi
2
Te
3
thin films were improved well at irradiation dose of 40 kGy. The calculated values of photoconversion efficiency and fill factor for Bi
2
Te
3
thin film were found to be 0.1837% and 0.5383, respectively. The values of photoconversion efficiency and fill factor of same electrode before irradiation have values 0.0987% and 0.3979, respectively. The enhancement in efficiency and fill factor due to EBI were found 53% and 74%, respectively. The enhancement in PEC properties is due to increased active surface area of the Bi
2
Te
3
films after irradiation dose. The results showed that, EBI are capable to strengthen the quality of electrode for PEC solar cell application.</abstract><cop>New York</cop><pub>Springer US</pub><doi>10.1007/s10854-021-06290-x</doi><tpages>16</tpages><orcidid>https://orcid.org/0000-0002-3829-3879</orcidid></addata></record> |
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| subjects | Bismuth tellurides Characterization and Evaluation of Materials Chemistry and Materials Science Crystal structure Efficiency Electron beams Electron irradiation Engineering Engineering, Electrical & Electronic Food irradiation Materials Science Materials Science, Multidisciplinary Nanocrystals Optical and Electronic Materials Photovoltaic cells Physical Sciences Physics Physics, Applied Physics, Condensed Matter Quantum efficiency Radiation dosage Science & Technology Solar cells Stainless steels Substrates Surface area Synthesis Technology Thin films |
| title | Effect of electron beam irradiation on EIS and photoelectrochemical performance of electrodeposited nanocrystalline Bi2Te3 thin films |
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