Layer-by-layer slot-die coated high-efficiency organic solar cells processed using twin boiling point solvents under ambient condition
Layer-by-layer (LbL) strategy has been developed to form bulk heterojunction (BHJ) structure for processing efficient organic solar cells (OSCs). Herein, LbL slot-die coating with twin boiling point solvents (TBPS) strategy was developed to fabricate highly efficient OSCs, which matches with large-s...
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| Veröffentlicht in: | Nano research 2021-11, Vol.14 (11), p.4236-4242 |
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| creator | Yang, Yu Feng, Erming Li, Hengyue Shen, Zichao Liu, Wanrong Guo, Jingbo Luo, Qun Zhang, Jidong Lu, Guanghao Ma, Changqi Yang, Junliang |
| description | Layer-by-layer (LbL) strategy has been developed to form bulk heterojunction (BHJ) structure for processing efficient organic solar cells (OSCs). Herein, LbL slot-die coating with twin boiling point solvents (TBPS) strategy was developed to fabricate highly efficient OSCs, which matches with large-scale, high throughput roll-to-roll (R2R) industrialized mass process. The TBPS strategy could produce high-quality thin film without any additive, leading to the optimized vertical phase separation with interpenetrating nanostructures, as well as the enhanced charge transport and extraction. Thus, the power conversion efficiency up to 14.42% was achieved for [(2,6-(4,8-bis(5-(2-ethylhexyl-3-fluoro)thiophen-2-yl)-benzo [1,2-b:4,5-b′]dithiophene))-alt-(5,5-(1′,3′-di-2-thienyl-5′,7′-bis(2-ethylhexyl)benzo[1′,2′-c:4′,5′-c′]dithiophene-4,8-dione)]:2,2′-((2Z,2′Z)-((12,13-bis(2-ethylhexyl)-3,9-diundecyl-12,13-dihydro-[1,2,5]thiadiazolo[3,4-e]thieno[2″,3″:4″,5″]thieno[2′,3′:4,5]pyrrolo[3,2-g]thieno[2′,3′:4,5]thieno[3,2-b]indole-2,10-diyl)bis(methanylylidene)) bis(5,6-difluoro-3-oxo-2,3-dihydro-1H-indene-2,1-diylidene))dimalononitrile (PM6:Y6) OSCs fabricated via sequentially LbL slot-die coating using the TBPS strategy under ambient condition. The research provides a potential route for industrialized production of high-efficiency and large-area OSC devices. |
| doi_str_mv | 10.1007/s12274-021-3576-8 |
| format | Article |
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Herein, LbL slot-die coating with twin boiling point solvents (TBPS) strategy was developed to fabricate highly efficient OSCs, which matches with large-scale, high throughput roll-to-roll (R2R) industrialized mass process. The TBPS strategy could produce high-quality thin film without any additive, leading to the optimized vertical phase separation with interpenetrating nanostructures, as well as the enhanced charge transport and extraction. Thus, the power conversion efficiency up to 14.42% was achieved for [(2,6-(4,8-bis(5-(2-ethylhexyl-3-fluoro)thiophen-2-yl)-benzo [1,2-b:4,5-b′]dithiophene))-alt-(5,5-(1′,3′-di-2-thienyl-5′,7′-bis(2-ethylhexyl)benzo[1′,2′-c:4′,5′-c′]dithiophene-4,8-dione)]:2,2′-((2Z,2′Z)-((12,13-bis(2-ethylhexyl)-3,9-diundecyl-12,13-dihydro-[1,2,5]thiadiazolo[3,4-e]thieno[2″,3″:4″,5″]thieno[2′,3′:4,5]pyrrolo[3,2-g]thieno[2′,3′:4,5]thieno[3,2-b]indole-2,10-diyl)bis(methanylylidene)) bis(5,6-difluoro-3-oxo-2,3-dihydro-1H-indene-2,1-diylidene))dimalononitrile (PM6:Y6) OSCs fabricated via sequentially LbL slot-die coating using the TBPS strategy under ambient condition. The research provides a potential route for industrialized production of high-efficiency and large-area OSC devices.</description><identifier>ISSN: 1998-0124</identifier><identifier>EISSN: 1998-0000</identifier><identifier>DOI: 10.1007/s12274-021-3576-8</identifier><language>eng</language><publisher>Beijing: Tsinghua University Press</publisher><subject>Atomic/Molecular Structure and Spectra ; Biomedicine ; Biotechnology ; Boiling ; Boiling points ; Charge transport ; Chemistry ; Chemistry and Materials Science ; Chemistry, Physical ; Coatings ; Condensed Matter Physics ; Efficiency ; Energy conversion efficiency ; Heterojunctions ; Indene ; Materials Science ; Materials Science, Multidisciplinary ; Nanoscience & Nanotechnology ; Nanotechnology ; Phase separation ; Photovoltaic cells ; Physical Sciences ; Physics ; Physics, Applied ; Research Article ; Science & Technology ; Science & Technology - Other Topics ; Slot dies ; Solar cells ; Solvents ; Technology ; Thin films ; Vertical separation</subject><ispartof>Nano research, 2021-11, Vol.14 (11), p.4236-4242</ispartof><rights>Tsinghua University Press and Springer-Verlag GmbH Germany, part of Springer Nature 2021</rights><rights>Tsinghua University Press and Springer-Verlag GmbH Germany, part of Springer Nature 2021.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>true</woscitedreferencessubscribed><woscitedreferencescount>37</woscitedreferencescount><woscitedreferencesoriginalsourcerecordid>wos000673055800001</woscitedreferencesoriginalsourcerecordid><citedby>FETCH-LOGICAL-c316t-7728304a03ecd4749b212010d2fc391ad3b8af97d405606648e5f764d9061e3e3</citedby><cites>FETCH-LOGICAL-c316t-7728304a03ecd4749b212010d2fc391ad3b8af97d405606648e5f764d9061e3e3</cites><orcidid>0000-0001-7829-7308</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s12274-021-3576-8$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s12274-021-3576-8$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27923,27924,41487,42556,51318</link.rule.ids></links><search><creatorcontrib>Yang, Yu</creatorcontrib><creatorcontrib>Feng, Erming</creatorcontrib><creatorcontrib>Li, Hengyue</creatorcontrib><creatorcontrib>Shen, Zichao</creatorcontrib><creatorcontrib>Liu, Wanrong</creatorcontrib><creatorcontrib>Guo, Jingbo</creatorcontrib><creatorcontrib>Luo, Qun</creatorcontrib><creatorcontrib>Zhang, Jidong</creatorcontrib><creatorcontrib>Lu, Guanghao</creatorcontrib><creatorcontrib>Ma, Changqi</creatorcontrib><creatorcontrib>Yang, Junliang</creatorcontrib><title>Layer-by-layer slot-die coated high-efficiency organic solar cells processed using twin boiling point solvents under ambient condition</title><title>Nano research</title><addtitle>Nano Res</addtitle><addtitle>NANO RES</addtitle><description>Layer-by-layer (LbL) strategy has been developed to form bulk heterojunction (BHJ) structure for processing efficient organic solar cells (OSCs). Herein, LbL slot-die coating with twin boiling point solvents (TBPS) strategy was developed to fabricate highly efficient OSCs, which matches with large-scale, high throughput roll-to-roll (R2R) industrialized mass process. The TBPS strategy could produce high-quality thin film without any additive, leading to the optimized vertical phase separation with interpenetrating nanostructures, as well as the enhanced charge transport and extraction. Thus, the power conversion efficiency up to 14.42% was achieved for [(2,6-(4,8-bis(5-(2-ethylhexyl-3-fluoro)thiophen-2-yl)-benzo [1,2-b:4,5-b′]dithiophene))-alt-(5,5-(1′,3′-di-2-thienyl-5′,7′-bis(2-ethylhexyl)benzo[1′,2′-c:4′,5′-c′]dithiophene-4,8-dione)]:2,2′-((2Z,2′Z)-((12,13-bis(2-ethylhexyl)-3,9-diundecyl-12,13-dihydro-[1,2,5]thiadiazolo[3,4-e]thieno[2″,3″:4″,5″]thieno[2′,3′:4,5]pyrrolo[3,2-g]thieno[2′,3′:4,5]thieno[3,2-b]indole-2,10-diyl)bis(methanylylidene)) bis(5,6-difluoro-3-oxo-2,3-dihydro-1H-indene-2,1-diylidene))dimalononitrile (PM6:Y6) OSCs fabricated via sequentially LbL slot-die coating using the TBPS strategy under ambient condition. The research provides a potential route for industrialized production of high-efficiency and large-area OSC devices.</description><subject>Atomic/Molecular Structure and Spectra</subject><subject>Biomedicine</subject><subject>Biotechnology</subject><subject>Boiling</subject><subject>Boiling points</subject><subject>Charge transport</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Chemistry, Physical</subject><subject>Coatings</subject><subject>Condensed Matter Physics</subject><subject>Efficiency</subject><subject>Energy conversion efficiency</subject><subject>Heterojunctions</subject><subject>Indene</subject><subject>Materials Science</subject><subject>Materials Science, Multidisciplinary</subject><subject>Nanoscience & Nanotechnology</subject><subject>Nanotechnology</subject><subject>Phase separation</subject><subject>Photovoltaic cells</subject><subject>Physical Sciences</subject><subject>Physics</subject><subject>Physics, Applied</subject><subject>Research Article</subject><subject>Science & Technology</subject><subject>Science & Technology - Other Topics</subject><subject>Slot dies</subject><subject>Solar cells</subject><subject>Solvents</subject><subject>Technology</subject><subject>Thin films</subject><subject>Vertical separation</subject><issn>1998-0124</issn><issn>1998-0000</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><sourceid>HGBXW</sourceid><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNqNkU1vFSEUhiemJrbVH-COxGWD5WuAWTY32prcpBtdEwbO3NJM4QqMzf0D_m4Zx4-ViWfDIXne8x5euu4tJe8pIeq6UMaUwIRRzHslsX7RndNh0Ji0OvvdUyZedRelPBIiGRX6vPu-tyfIeDzheW1QmVPFPgByyVbw6CEcHjBMU3ABojuhlA82BodKmm1GDua5oGNODkpp9FJCPKD6HCIaU5jXyzGFWFf8G8Ra0BJ9c7FPYxtXm0n0oYYUX3cvJzsXePPrvOy-fPzweXeH9_e3n3Y3e-w4lRUrxTQnwhIOzgslhpFRRijxbHJ8oNbzUdtpUF6QXhIphYZ-UlL4gUgKHPhl926b23b-ukCp5jEtOTZLw3pNdJMJ3Si6US6nUjJM5pjDk80nQ4lZ4zZb3KbFbda4zaq52jTPMKap_IwL_ujaJ0jFSd88WtFG6_-nd6HaNaRdWmJtUrZJS8PjAfLfJ_x7ux_PmqT3</recordid><startdate>20211101</startdate><enddate>20211101</enddate><creator>Yang, Yu</creator><creator>Feng, Erming</creator><creator>Li, Hengyue</creator><creator>Shen, Zichao</creator><creator>Liu, Wanrong</creator><creator>Guo, Jingbo</creator><creator>Luo, Qun</creator><creator>Zhang, Jidong</creator><creator>Lu, Guanghao</creator><creator>Ma, Changqi</creator><creator>Yang, Junliang</creator><general>Tsinghua University Press</general><general>Tsinghua Univ Press</general><general>Springer Nature B.V</general><scope>BLEPL</scope><scope>DTL</scope><scope>HGBXW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7QF</scope><scope>7QO</scope><scope>7QQ</scope><scope>7SE</scope><scope>7SR</scope><scope>7U5</scope><scope>7X7</scope><scope>7XB</scope><scope>8AO</scope><scope>8BQ</scope><scope>8FD</scope><scope>8FE</scope><scope>8FG</scope><scope>8FH</scope><scope>8FI</scope><scope>8FJ</scope><scope>8FK</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AEUYN</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BBNVY</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>BHPHI</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>FR3</scope><scope>FYUFA</scope><scope>GHDGH</scope><scope>GNUQQ</scope><scope>H8G</scope><scope>HCIFZ</scope><scope>JG9</scope><scope>K9.</scope><scope>KB.</scope><scope>L7M</scope><scope>LK8</scope><scope>M0S</scope><scope>M7P</scope><scope>P64</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><orcidid>https://orcid.org/0000-0001-7829-7308</orcidid></search><sort><creationdate>20211101</creationdate><title>Layer-by-layer slot-die coated high-efficiency organic solar cells processed using twin boiling point solvents under ambient condition</title><author>Yang, Yu ; Feng, Erming ; Li, Hengyue ; Shen, Zichao ; Liu, Wanrong ; Guo, Jingbo ; Luo, Qun ; Zhang, Jidong ; Lu, Guanghao ; Ma, Changqi ; Yang, Junliang</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c316t-7728304a03ecd4749b212010d2fc391ad3b8af97d405606648e5f764d9061e3e3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>Atomic/Molecular Structure and Spectra</topic><topic>Biomedicine</topic><topic>Biotechnology</topic><topic>Boiling</topic><topic>Boiling points</topic><topic>Charge transport</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Chemistry, Physical</topic><topic>Coatings</topic><topic>Condensed Matter Physics</topic><topic>Efficiency</topic><topic>Energy conversion efficiency</topic><topic>Heterojunctions</topic><topic>Indene</topic><topic>Materials Science</topic><topic>Materials Science, Multidisciplinary</topic><topic>Nanoscience & Nanotechnology</topic><topic>Nanotechnology</topic><topic>Phase separation</topic><topic>Photovoltaic cells</topic><topic>Physical Sciences</topic><topic>Physics</topic><topic>Physics, Applied</topic><topic>Research Article</topic><topic>Science & Technology</topic><topic>Science & Technology - Other Topics</topic><topic>Slot dies</topic><topic>Solar cells</topic><topic>Solvents</topic><topic>Technology</topic><topic>Thin films</topic><topic>Vertical separation</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Yang, Yu</creatorcontrib><creatorcontrib>Feng, Erming</creatorcontrib><creatorcontrib>Li, Hengyue</creatorcontrib><creatorcontrib>Shen, Zichao</creatorcontrib><creatorcontrib>Liu, Wanrong</creatorcontrib><creatorcontrib>Guo, Jingbo</creatorcontrib><creatorcontrib>Luo, Qun</creatorcontrib><creatorcontrib>Zhang, Jidong</creatorcontrib><creatorcontrib>Lu, Guanghao</creatorcontrib><creatorcontrib>Ma, Changqi</creatorcontrib><creatorcontrib>Yang, Junliang</creatorcontrib><collection>Web of Science Core Collection</collection><collection>Science Citation Index Expanded</collection><collection>Web of Science - Science Citation Index Expanded - 2021</collection><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>Aluminium Industry Abstracts</collection><collection>Biotechnology Research Abstracts</collection><collection>Ceramic Abstracts</collection><collection>Corrosion Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Health & Medical Collection</collection><collection>ProQuest Central (purchase pre-March 2016)</collection><collection>ProQuest Pharma Collection</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>ProQuest Natural Science Collection</collection><collection>Hospital Premium Collection</collection><collection>Hospital Premium Collection (Alumni Edition)</collection><collection>ProQuest Central (Alumni) (purchase pre-March 2016)</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central (Alumni Edition)</collection><collection>ProQuest One Sustainability</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central Essentials</collection><collection>Biological Science Collection</collection><collection>ProQuest Central</collection><collection>Technology Collection (ProQuest)</collection><collection>Natural Science Collection (ProQuest)</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>Engineering Research Database</collection><collection>Health Research Premium Collection</collection><collection>Health Research Premium Collection (Alumni)</collection><collection>ProQuest Central Student</collection><collection>Copper Technical Reference Library</collection><collection>SciTech Premium Collection</collection><collection>Materials Research Database</collection><collection>ProQuest Health & Medical Complete (Alumni)</collection><collection>Materials Science Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>ProQuest Biological Science Collection</collection><collection>Health & Medical Collection (Alumni Edition)</collection><collection>Biological Science Database</collection><collection>Biotechnology and BioEngineering Abstracts</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><jtitle>Nano research</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Yang, Yu</au><au>Feng, Erming</au><au>Li, Hengyue</au><au>Shen, Zichao</au><au>Liu, Wanrong</au><au>Guo, Jingbo</au><au>Luo, Qun</au><au>Zhang, Jidong</au><au>Lu, Guanghao</au><au>Ma, Changqi</au><au>Yang, Junliang</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Layer-by-layer slot-die coated high-efficiency organic solar cells processed using twin boiling point solvents under ambient condition</atitle><jtitle>Nano research</jtitle><stitle>Nano Res</stitle><stitle>NANO RES</stitle><date>2021-11-01</date><risdate>2021</risdate><volume>14</volume><issue>11</issue><spage>4236</spage><epage>4242</epage><pages>4236-4242</pages><issn>1998-0124</issn><eissn>1998-0000</eissn><abstract>Layer-by-layer (LbL) strategy has been developed to form bulk heterojunction (BHJ) structure for processing efficient organic solar cells (OSCs). Herein, LbL slot-die coating with twin boiling point solvents (TBPS) strategy was developed to fabricate highly efficient OSCs, which matches with large-scale, high throughput roll-to-roll (R2R) industrialized mass process. The TBPS strategy could produce high-quality thin film without any additive, leading to the optimized vertical phase separation with interpenetrating nanostructures, as well as the enhanced charge transport and extraction. Thus, the power conversion efficiency up to 14.42% was achieved for [(2,6-(4,8-bis(5-(2-ethylhexyl-3-fluoro)thiophen-2-yl)-benzo [1,2-b:4,5-b′]dithiophene))-alt-(5,5-(1′,3′-di-2-thienyl-5′,7′-bis(2-ethylhexyl)benzo[1′,2′-c:4′,5′-c′]dithiophene-4,8-dione)]:2,2′-((2Z,2′Z)-((12,13-bis(2-ethylhexyl)-3,9-diundecyl-12,13-dihydro-[1,2,5]thiadiazolo[3,4-e]thieno[2″,3″:4″,5″]thieno[2′,3′:4,5]pyrrolo[3,2-g]thieno[2′,3′:4,5]thieno[3,2-b]indole-2,10-diyl)bis(methanylylidene)) bis(5,6-difluoro-3-oxo-2,3-dihydro-1H-indene-2,1-diylidene))dimalononitrile (PM6:Y6) OSCs fabricated via sequentially LbL slot-die coating using the TBPS strategy under ambient condition. The research provides a potential route for industrialized production of high-efficiency and large-area OSC devices.</abstract><cop>Beijing</cop><pub>Tsinghua University Press</pub><doi>10.1007/s12274-021-3576-8</doi><tpages>7</tpages><orcidid>https://orcid.org/0000-0001-7829-7308</orcidid></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 1998-0124 |
| ispartof | Nano research, 2021-11, Vol.14 (11), p.4236-4242 |
| issn | 1998-0124 1998-0000 |
| language | eng |
| recordid | cdi_webofscience_primary_000673055800001 |
| source | SpringerLink Journals - AutoHoldings |
| subjects | Atomic/Molecular Structure and Spectra Biomedicine Biotechnology Boiling Boiling points Charge transport Chemistry Chemistry and Materials Science Chemistry, Physical Coatings Condensed Matter Physics Efficiency Energy conversion efficiency Heterojunctions Indene Materials Science Materials Science, Multidisciplinary Nanoscience & Nanotechnology Nanotechnology Phase separation Photovoltaic cells Physical Sciences Physics Physics, Applied Research Article Science & Technology Science & Technology - Other Topics Slot dies Solar cells Solvents Technology Thin films Vertical separation |
| title | Layer-by-layer slot-die coated high-efficiency organic solar cells processed using twin boiling point solvents under ambient condition |
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