Synthesis of zero-valent iron/biochar by carbothermal reduction from wood waste and iron mud for removing rhodamine B
This study proposes a new process to synthesize zero-valent iron/biochar (Fe 0 -BC) by carbothermal reduction using wood waste and iron mud as raw materials under different temperature. The characterization results showed that the Fe 0 -BC synthesized at 1200 °C (Fe 0 -BC-1200) possessed favorable a...
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| Veröffentlicht in: | Environmental science and pollution research international 2021-09, Vol.28 (35), p.48556-48568 |
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| creator | Chen, Chao Liu, Jianguo Gen, Chao Liu, Qin Zhu, Xuetao Qi, Wenzhi Wang, Fan |
| description | This study proposes a new process to synthesize zero-valent iron/biochar (Fe
0
-BC) by carbothermal reduction using wood waste and iron mud as raw materials under different temperature. The characterization results showed that the Fe
0
-BC synthesized at 1200 °C (Fe
0
-BC-1200) possessed favorable adsorption capacity with the specific surface area of 103.18 m
2
/g and that the zero-valent iron (Fe
0
) particles were uniformly dispersed on the biochar surface. The removal efficiency of rhodamine B (RB) was determined to evaluate the performance of the prepared Fe
0
-BC. Fe
0
-BC-1200 presented the best performance on RB removal, which mainly ascribes to that more Fe
0
particles generated at higher temperature. The equilibrium adsorption capacity reached 49.93 mg/g when the initial RB concentration and the Fe
0
-BC-1200 dosage were 100 mg/L and 2 g/L, respectively, and the pseudo-second-order model was suitable to fit the removal experimental data. LCMC and XRD analyses revealed that the removal mechanism included the physical adsorption of biochar and the redox reaction of Fe
0
. Moreover, copper existing in the iron mud was also reduced to Cu
0
, which was beneficial to catalyze the oxidation of iron; the degradation of RB was promoted at the same time.
Graphical abstract |
| doi_str_mv | 10.1007/s11356-021-13962-y |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_webof</sourceid><recordid>TN_cdi_webofscience_primary_000645190100010</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2519312452</sourcerecordid><originalsourceid>FETCH-LOGICAL-c419t-364b7e1e17201f7861582a18607c73c67b55bca9d7da6c74d482480479d2f88b3</originalsourceid><addsrcrecordid>eNqN0U2L1TAUBuAginMd_QMuJOBGkDo5SZo0S734BQMu1HVIk3RuhjYZk3Yu9debmY4juBAXJYU-7-E0L0LPgbwBQuRZAWCtaAiFBpgStFkfoB0I4I3kSj1EO6I4r584P0FPSrkkhBJF5WN0wpiqb1zt0PJ1jfPBl1BwGvBPn1NzbUYfZxxyimd9SPZgMu5XbE3uU6V5MiPO3i12DiniIacJH1Ny-GjK7LGJ7jaKp8XhIeVKp3Qd4gXOh-TMFKLH756iR4MZi392d56i7x_ef9t_as6_fPy8f3veWA5qbpjgvfTgQVICg-wEtB010AkirWRWyL5te2uUk84IK7njHeUd4VI5OnRdz07Rq23uVU4_Fl9mPYVi_Tia6NNSNG1BMaC8pZW-_ItepiXHul1VogMiWAtV0U3ZnErJftBXOUwmrxqIvilFb6XoWoq-LUWvNfTibvTST97dR363UEG3gaPv01Bs8NH6e0YIEbwuSur8-uzDbG5ufp-WONfo6_-PVs02XaqIFz7_-cl_7P8LqK-4qw</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2568106351</pqid></control><display><type>article</type><title>Synthesis of zero-valent iron/biochar by carbothermal reduction from wood waste and iron mud for removing rhodamine B</title><source>SpringerNature Journals</source><source>Web of Science - Science Citation Index Expanded - 2021<img src="https://exlibris-pub.s3.amazonaws.com/fromwos-v2.jpg" /></source><creator>Chen, Chao ; Liu, Jianguo ; Gen, Chao ; Liu, Qin ; Zhu, Xuetao ; Qi, Wenzhi ; Wang, Fan</creator><creatorcontrib>Chen, Chao ; Liu, Jianguo ; Gen, Chao ; Liu, Qin ; Zhu, Xuetao ; Qi, Wenzhi ; Wang, Fan</creatorcontrib><description>This study proposes a new process to synthesize zero-valent iron/biochar (Fe
0
-BC) by carbothermal reduction using wood waste and iron mud as raw materials under different temperature. The characterization results showed that the Fe
0
-BC synthesized at 1200 °C (Fe
0
-BC-1200) possessed favorable adsorption capacity with the specific surface area of 103.18 m
2
/g and that the zero-valent iron (Fe
0
) particles were uniformly dispersed on the biochar surface. The removal efficiency of rhodamine B (RB) was determined to evaluate the performance of the prepared Fe
0
-BC. Fe
0
-BC-1200 presented the best performance on RB removal, which mainly ascribes to that more Fe
0
particles generated at higher temperature. The equilibrium adsorption capacity reached 49.93 mg/g when the initial RB concentration and the Fe
0
-BC-1200 dosage were 100 mg/L and 2 g/L, respectively, and the pseudo-second-order model was suitable to fit the removal experimental data. LCMC and XRD analyses revealed that the removal mechanism included the physical adsorption of biochar and the redox reaction of Fe
0
. Moreover, copper existing in the iron mud was also reduced to Cu
0
, which was beneficial to catalyze the oxidation of iron; the degradation of RB was promoted at the same time.
Graphical abstract</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-021-13962-y</identifier><identifier>PMID: 33909249</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Adsorption ; Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; Charcoal ; Earth and Environmental Science ; Ecotoxicology ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; Environmental Sciences ; Environmental Sciences & Ecology ; High temperature ; Iron ; Life Sciences & Biomedicine ; Mud ; Oxidation ; Performance evaluation ; Raw materials ; Redox reactions ; Reduction ; Research Article ; Rhodamine ; Science & Technology ; Surface chemistry ; Synthesis ; Waste Water Technology ; Water Management ; Water Pollution Control ; Wood waste</subject><ispartof>Environmental science and pollution research international, 2021-09, Vol.28 (35), p.48556-48568</ispartof><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2021</rights><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2021.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>true</woscitedreferencessubscribed><woscitedreferencescount>10</woscitedreferencescount><woscitedreferencesoriginalsourcerecordid>wos000645190100010</woscitedreferencesoriginalsourcerecordid><citedby>FETCH-LOGICAL-c419t-364b7e1e17201f7861582a18607c73c67b55bca9d7da6c74d482480479d2f88b3</citedby><cites>FETCH-LOGICAL-c419t-364b7e1e17201f7861582a18607c73c67b55bca9d7da6c74d482480479d2f88b3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-021-13962-y$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-021-13962-y$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>315,781,785,27929,27930,39263,41493,42562,51324</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/33909249$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Chen, Chao</creatorcontrib><creatorcontrib>Liu, Jianguo</creatorcontrib><creatorcontrib>Gen, Chao</creatorcontrib><creatorcontrib>Liu, Qin</creatorcontrib><creatorcontrib>Zhu, Xuetao</creatorcontrib><creatorcontrib>Qi, Wenzhi</creatorcontrib><creatorcontrib>Wang, Fan</creatorcontrib><title>Synthesis of zero-valent iron/biochar by carbothermal reduction from wood waste and iron mud for removing rhodamine B</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>ENVIRON SCI POLLUT R</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>This study proposes a new process to synthesize zero-valent iron/biochar (Fe
0
-BC) by carbothermal reduction using wood waste and iron mud as raw materials under different temperature. The characterization results showed that the Fe
0
-BC synthesized at 1200 °C (Fe
0
-BC-1200) possessed favorable adsorption capacity with the specific surface area of 103.18 m
2
/g and that the zero-valent iron (Fe
0
) particles were uniformly dispersed on the biochar surface. The removal efficiency of rhodamine B (RB) was determined to evaluate the performance of the prepared Fe
0
-BC. Fe
0
-BC-1200 presented the best performance on RB removal, which mainly ascribes to that more Fe
0
particles generated at higher temperature. The equilibrium adsorption capacity reached 49.93 mg/g when the initial RB concentration and the Fe
0
-BC-1200 dosage were 100 mg/L and 2 g/L, respectively, and the pseudo-second-order model was suitable to fit the removal experimental data. LCMC and XRD analyses revealed that the removal mechanism included the physical adsorption of biochar and the redox reaction of Fe
0
. Moreover, copper existing in the iron mud was also reduced to Cu
0
, which was beneficial to catalyze the oxidation of iron; the degradation of RB was promoted at the same time.
Graphical abstract</description><subject>Adsorption</subject><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Charcoal</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Environmental Sciences</subject><subject>Environmental Sciences & Ecology</subject><subject>High temperature</subject><subject>Iron</subject><subject>Life Sciences & Biomedicine</subject><subject>Mud</subject><subject>Oxidation</subject><subject>Performance evaluation</subject><subject>Raw materials</subject><subject>Redox reactions</subject><subject>Reduction</subject><subject>Research Article</subject><subject>Rhodamine</subject><subject>Science & Technology</subject><subject>Surface chemistry</subject><subject>Synthesis</subject><subject>Waste Water Technology</subject><subject>Water Management</subject><subject>Water Pollution Control</subject><subject>Wood waste</subject><issn>0944-1344</issn><issn>1614-7499</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><sourceid>HGBXW</sourceid><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNqN0U2L1TAUBuAginMd_QMuJOBGkDo5SZo0S734BQMu1HVIk3RuhjYZk3Yu9debmY4juBAXJYU-7-E0L0LPgbwBQuRZAWCtaAiFBpgStFkfoB0I4I3kSj1EO6I4r584P0FPSrkkhBJF5WN0wpiqb1zt0PJ1jfPBl1BwGvBPn1NzbUYfZxxyimd9SPZgMu5XbE3uU6V5MiPO3i12DiniIacJH1Ny-GjK7LGJ7jaKp8XhIeVKp3Qd4gXOh-TMFKLH756iR4MZi392d56i7x_ef9t_as6_fPy8f3veWA5qbpjgvfTgQVICg-wEtB010AkirWRWyL5te2uUk84IK7njHeUd4VI5OnRdz07Rq23uVU4_Fl9mPYVi_Tia6NNSNG1BMaC8pZW-_ItepiXHul1VogMiWAtV0U3ZnErJftBXOUwmrxqIvilFb6XoWoq-LUWvNfTibvTST97dR363UEG3gaPv01Bs8NH6e0YIEbwuSur8-uzDbG5ufp-WONfo6_-PVs02XaqIFz7_-cl_7P8LqK-4qw</recordid><startdate>20210901</startdate><enddate>20210901</enddate><creator>Chen, 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of zero-valent iron/biochar by carbothermal reduction from wood waste and iron mud for removing rhodamine B</title><author>Chen, Chao ; Liu, Jianguo ; Gen, Chao ; Liu, Qin ; Zhu, Xuetao ; Qi, Wenzhi ; Wang, Fan</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c419t-364b7e1e17201f7861582a18607c73c67b55bca9d7da6c74d482480479d2f88b3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>Adsorption</topic><topic>Aquatic Pollution</topic><topic>Atmospheric Protection/Air Quality Control/Air Pollution</topic><topic>Charcoal</topic><topic>Earth and Environmental Science</topic><topic>Ecotoxicology</topic><topic>Environment</topic><topic>Environmental Chemistry</topic><topic>Environmental Health</topic><topic>Environmental science</topic><topic>Environmental Sciences</topic><topic>Environmental Sciences & Ecology</topic><topic>High temperature</topic><topic>Iron</topic><topic>Life Sciences & Biomedicine</topic><topic>Mud</topic><topic>Oxidation</topic><topic>Performance evaluation</topic><topic>Raw materials</topic><topic>Redox reactions</topic><topic>Reduction</topic><topic>Research Article</topic><topic>Rhodamine</topic><topic>Science & Technology</topic><topic>Surface chemistry</topic><topic>Synthesis</topic><topic>Waste Water Technology</topic><topic>Water Management</topic><topic>Water Pollution Control</topic><topic>Wood waste</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Chen, Chao</creatorcontrib><creatorcontrib>Liu, Jianguo</creatorcontrib><creatorcontrib>Gen, Chao</creatorcontrib><creatorcontrib>Liu, Qin</creatorcontrib><creatorcontrib>Zhu, Xuetao</creatorcontrib><creatorcontrib>Qi, Wenzhi</creatorcontrib><creatorcontrib>Wang, Fan</creatorcontrib><collection>Web of Science Core Collection</collection><collection>Science Citation Index Expanded</collection><collection>Web of Science - Science Citation 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(Alumni)</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>Environmental Science Collection</collection><collection>ProQuest Central Basic</collection><collection>MEDLINE - Academic</collection><jtitle>Environmental science and pollution research international</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Chen, Chao</au><au>Liu, Jianguo</au><au>Gen, Chao</au><au>Liu, Qin</au><au>Zhu, Xuetao</au><au>Qi, Wenzhi</au><au>Wang, Fan</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Synthesis of zero-valent iron/biochar by carbothermal reduction from wood waste and iron mud for removing rhodamine B</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><stitle>ENVIRON SCI POLLUT R</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2021-09-01</date><risdate>2021</risdate><volume>28</volume><issue>35</issue><spage>48556</spage><epage>48568</epage><pages>48556-48568</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>This study proposes a new process to synthesize zero-valent iron/biochar (Fe
0
-BC) by carbothermal reduction using wood waste and iron mud as raw materials under different temperature. The characterization results showed that the Fe
0
-BC synthesized at 1200 °C (Fe
0
-BC-1200) possessed favorable adsorption capacity with the specific surface area of 103.18 m
2
/g and that the zero-valent iron (Fe
0
) particles were uniformly dispersed on the biochar surface. The removal efficiency of rhodamine B (RB) was determined to evaluate the performance of the prepared Fe
0
-BC. Fe
0
-BC-1200 presented the best performance on RB removal, which mainly ascribes to that more Fe
0
particles generated at higher temperature. The equilibrium adsorption capacity reached 49.93 mg/g when the initial RB concentration and the Fe
0
-BC-1200 dosage were 100 mg/L and 2 g/L, respectively, and the pseudo-second-order model was suitable to fit the removal experimental data. LCMC and XRD analyses revealed that the removal mechanism included the physical adsorption of biochar and the redox reaction of Fe
0
. Moreover, copper existing in the iron mud was also reduced to Cu
0
, which was beneficial to catalyze the oxidation of iron; the degradation of RB was promoted at the same time.
Graphical abstract</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>33909249</pmid><doi>10.1007/s11356-021-13962-y</doi><tpages>13</tpages><oa>free_for_read</oa></addata></record> |
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| source | SpringerNature Journals; Web of Science - Science Citation Index Expanded - 2021<img src="https://exlibris-pub.s3.amazonaws.com/fromwos-v2.jpg" /> |
| subjects | Adsorption Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Charcoal Earth and Environmental Science Ecotoxicology Environment Environmental Chemistry Environmental Health Environmental science Environmental Sciences Environmental Sciences & Ecology High temperature Iron Life Sciences & Biomedicine Mud Oxidation Performance evaluation Raw materials Redox reactions Reduction Research Article Rhodamine Science & Technology Surface chemistry Synthesis Waste Water Technology Water Management Water Pollution Control Wood waste |
| title | Synthesis of zero-valent iron/biochar by carbothermal reduction from wood waste and iron mud for removing rhodamine B |
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