Multi-year analysis of aerosol optical properties at various timescales using AERONET data in tropical West Africa

The optical properties of aerosols are investigated using multi-year analysis from the Ilorin AERONET site (8.320° N, 4.340° E) in Nigeria, in tropical West Africa. Characterization at five wavelengths (440, 550, 675, 870 and 1020 nm) were carried out to investigate the absorption and scattering ten...

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Veröffentlicht in:Journal of aerosol science 2021-01, Vol.151, p.105625, Article 105625
Hauptverfasser: Yusuf, Najib, Said S, Rabia, Tilmes, Simone, Gbobaniyi, Emiola
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Sprache:eng
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Zusammenfassung:The optical properties of aerosols are investigated using multi-year analysis from the Ilorin AERONET site (8.320° N, 4.340° E) in Nigeria, in tropical West Africa. Characterization at five wavelengths (440, 550, 675, 870 and 1020 nm) were carried out to investigate the absorption and scattering tendencies of aerosol properties at multi-timescale. Results show large aerosol optical thickness (AOT) at 550 nm in a mixed aerosol load with 74% coarse mode dominance and 24% fine mode particles densely distributed in the dry-cold/Harmattan season (DJF) and sparsely distributed in the wet season (June–Oct). The volume size distribution (VSD) pattern shows higher variations and dominance for the coarse mode in the dry season than for the accumulation mode. The Ångström exponent (AE) α and τ550 show regular variations, with seasonal averaged maximum α > 1 and τ550 peak at ~ 1.0. Values of α > 1 were observed in wet seasons; ~1.1 (Aug), 1.04 (Sep). Averaged single scattering albedo (SSA) is confined to values between 0.83 and 0.97, with the highest values in October and lowest values in DJF due to biomass burning (BB) emissions mixed with transported desert dust that are composed of iron oxides (hematite) absorbing mineral. Seasonal ϖ0 increases with increasing wavelength and absorption was found to be the highest at 440 nm, with a total absorption of 0.16. The asymmetry parameter g shows minor interannual variations. The highest value of >0.70 was found at the shortest wavelength (440 nm), and was found to decrease as wavelengths increased. The real part of the refractive index (RR) ranges between 1.17 and 1.44 depending on seasons, and the imaginary part of the refractive index (RI) shows higher absorption for dry season (0.009). •Optical properties of aerosols are investigated using ground-based data multi-year analysis in the tropic.•Large AOT is observed with 74% coarse mode aerosols as dominance and 24% fine mode particles.•Values of α > 1 are observed even in wet seasons, though dominant in DJF.•Total absorption of 0.16 is found across wavelengths studied and absorption is highest at 440 nm.•Volume size distribution pattern shows higher variations and dominance in the coarse mode in the dry season.
ISSN:0021-8502
1879-1964
DOI:10.1016/j.jaerosci.2020.105625