Waste cotton fabric derived porous carbon containing Fe3O4/NiS nanoparticles for electrocatalytic oxygen evolution

Developing low-cost, active and durable electrocatalysts for oxygen evolution reaction (OER) is an urgent task for the applications such as water splitting and rechargeable metal-air battery. Herein, this work reports the fabrication of a metal and hetero atom co-doped fibrous carbon structure deriv...

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Veröffentlicht in:Journal of materials science & technology 2020-12, Vol.59, p.92-99
Hauptverfasser: Jiang, Shan, Shao, Hao, Cao, Genyang, Li, Han, Xu, Weilin, Li, Jingliang, Fang, Jian, Wang, Xungai
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container_end_page 99
container_issue
container_start_page 92
container_title Journal of materials science & technology
container_volume 59
creator Jiang, Shan
Shao, Hao
Cao, Genyang
Li, Han
Xu, Weilin
Li, Jingliang
Fang, Jian
Wang, Xungai
description Developing low-cost, active and durable electrocatalysts for oxygen evolution reaction (OER) is an urgent task for the applications such as water splitting and rechargeable metal-air battery. Herein, this work reports the fabrication of a metal and hetero atom co-doped fibrous carbon structure derived from cotton textile wastes and its use as an efficient OER catalyst. The free-standing fibrous carbon structure, fabricated with a simple two-step carbonization process, has a high specific surface area of 1796 m2/g and a uniform distribution of Fe3O4/NiS nanoparticles (Fe3O4/NiS@CC). The composite exhibits excellent OER performance with an onset potential of 1.44 V and a low overpotential of 310 mV at the current density of 10 mA/cm2 in a 1.0 M KOH solution, which even surpass commercial RuO2 catalyst. Additionally, this ternary catalyst shows remarkable long-term stability without current density loss after continuous operation for 26 h. It can be believed that the outstanding OER performance is attributed to the synergistic effect between the iron oxides and nickel sulphides, as well as the micro-meso porous carbon structure. This study demonstrates a new strategy to use conventional textile materials to prepare highly efficient electrocatalysts; it also provides a simple approach to turn textile waste into valuable products.
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source ScienceDirect Journals (5 years ago - present); Alma/SFX Local Collection
subjects Iron oxides
Nickel sulphides
OER electrocatalyst
Porous carbon
Waste cotton
title Waste cotton fabric derived porous carbon containing Fe3O4/NiS nanoparticles for electrocatalytic oxygen evolution
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