Application of GETFLOWS Coupled with Chemical Reactions to Arsenic Removal through Ferrihydrite Coprecipitation in an Artificial Wetland of a Japanese Closed Mine
Passive systems that utilize a natural power such as a pond, plant, or microorganisms, is expected to be a cost-effective method for acid mine drainage (AMD) treatment. The Ningyo-toge mine, a non-operational uranium mine located in Okayama Prefecture, Japan, generates AMD containing arsenic and iro...
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| Veröffentlicht in: | Minerals (Basel) 2020-05, Vol.10 (5), p.475, Article 475 |
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| creator | Kato, Tatsuya Kawasaki, Yohei Kadokura, Masakazu Suzuki, Kohei Tawara, Yasuhiro Ohara, Yoshiyuki Tokoro, Chiharu |
| description | Passive systems that utilize a natural power such as a pond, plant, or microorganisms, is expected to be a cost-effective method for acid mine drainage (AMD) treatment. The Ningyo-toge mine, a non-operational uranium mine located in Okayama Prefecture, Japan, generates AMD containing arsenic and iron. To quantitatively study arsenic and iron ion removal in an artificial wetland and pond, chemical reactions were modeled and incorporated into the GETFLOWS (general-purpose terrestrial fluid-flow simulator) software. The chemical reaction models consisted of arsenite and ferrous oxidation equations and arsenic adsorption on ferrihydrite. The X-ray diffraction analysis of sediment samples showed ferrihydrite patterns. These results were consistent with the model for arsenite/ferrous oxidation and arsenic adsorption on ferrihydrite. Geofluid simulation was conducted to simulate mass transfer with the utilized topographic model, inlet flow rate, precipitation, and evaporation. The measured arsenic and iron ions concentrations in solution samples from the wetland and pond, fitted well with the model. This indicated that the main removal mechanism was the oxidation of arsenite/ferrous ions and that arsenic was removed by adsorption rather than dilution. |
| doi_str_mv | 10.3390/min10050475 |
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The Ningyo-toge mine, a non-operational uranium mine located in Okayama Prefecture, Japan, generates AMD containing arsenic and iron. To quantitatively study arsenic and iron ion removal in an artificial wetland and pond, chemical reactions were modeled and incorporated into the GETFLOWS (general-purpose terrestrial fluid-flow simulator) software. The chemical reaction models consisted of arsenite and ferrous oxidation equations and arsenic adsorption on ferrihydrite. The X-ray diffraction analysis of sediment samples showed ferrihydrite patterns. These results were consistent with the model for arsenite/ferrous oxidation and arsenic adsorption on ferrihydrite. Geofluid simulation was conducted to simulate mass transfer with the utilized topographic model, inlet flow rate, precipitation, and evaporation. The measured arsenic and iron ions concentrations in solution samples from the wetland and pond, fitted well with the model. This indicated that the main removal mechanism was the oxidation of arsenite/ferrous ions and that arsenic was removed by adsorption rather than dilution.</description><identifier>ISSN: 2075-163X</identifier><identifier>EISSN: 2075-163X</identifier><identifier>DOI: 10.3390/min10050475</identifier><language>eng</language><publisher>BASEL: Mdpi</publisher><subject>Acid mine drainage ; Adsorption ; Aluminum ; Arsenic ; Arsenic removal ; Arsenite ; Artificial wetlands ; Chemical precipitation ; Chemical reactions ; Computational fluid dynamics ; Computer simulation ; Coprecipitation ; Diffraction patterns ; Dilution ; Evaporation ; Evaporation rate ; Ferrous ions ; Flow rates ; Flow velocity ; Fluid flow ; Geochemistry & Geophysics ; GETFLOWS ; Inlet flow ; Inlets (waterways) ; Ions ; Iron ; Mass transfer ; Microorganisms ; Mine drainage ; Mineralogy ; Mines ; Mining & Mineral Processing ; Oxidation ; Physical Sciences ; Pollutant removal ; Ponds ; Precipitation ; quantitative modeling ; Removal ; Science & Technology ; Sediment samplers ; Sediment samples ; Simulation ; Simulators ; Studies ; surface complexation ; Surface water ; the three-dimensional topographic model ; Uranium ; Water pollution ; Wetlands ; X-ray diffraction ; X-ray diffraction analysis</subject><ispartof>Minerals (Basel), 2020-05, Vol.10 (5), p.475, Article 475</ispartof><rights>2020. 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Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>true</woscitedreferencessubscribed><woscitedreferencescount>6</woscitedreferencescount><woscitedreferencesoriginalsourcerecordid>wos000548343700090</woscitedreferencesoriginalsourcerecordid><citedby>FETCH-LOGICAL-c364t-cf5bc7995017af5168b282f76ee941b293d3d12bddf6e186a7419632c115140d3</citedby><cites>FETCH-LOGICAL-c364t-cf5bc7995017af5168b282f76ee941b293d3d12bddf6e186a7419632c115140d3</cites><orcidid>0000-0001-6214-0402</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>315,781,785,27928,27929,28252</link.rule.ids></links><search><creatorcontrib>Kato, Tatsuya</creatorcontrib><creatorcontrib>Kawasaki, Yohei</creatorcontrib><creatorcontrib>Kadokura, Masakazu</creatorcontrib><creatorcontrib>Suzuki, Kohei</creatorcontrib><creatorcontrib>Tawara, Yasuhiro</creatorcontrib><creatorcontrib>Ohara, Yoshiyuki</creatorcontrib><creatorcontrib>Tokoro, Chiharu</creatorcontrib><title>Application of GETFLOWS Coupled with Chemical Reactions to Arsenic Removal through Ferrihydrite Coprecipitation in an Artificial Wetland of a Japanese Closed Mine</title><title>Minerals (Basel)</title><addtitle>MINERALS-BASEL</addtitle><description>Passive systems that utilize a natural power such as a pond, plant, or microorganisms, is expected to be a cost-effective method for acid mine drainage (AMD) treatment. The Ningyo-toge mine, a non-operational uranium mine located in Okayama Prefecture, Japan, generates AMD containing arsenic and iron. To quantitatively study arsenic and iron ion removal in an artificial wetland and pond, chemical reactions were modeled and incorporated into the GETFLOWS (general-purpose terrestrial fluid-flow simulator) software. The chemical reaction models consisted of arsenite and ferrous oxidation equations and arsenic adsorption on ferrihydrite. The X-ray diffraction analysis of sediment samples showed ferrihydrite patterns. These results were consistent with the model for arsenite/ferrous oxidation and arsenic adsorption on ferrihydrite. Geofluid simulation was conducted to simulate mass transfer with the utilized topographic model, inlet flow rate, precipitation, and evaporation. The measured arsenic and iron ions concentrations in solution samples from the wetland and pond, fitted well with the model. This indicated that the main removal mechanism was the oxidation of arsenite/ferrous ions and that arsenic was removed by adsorption rather than dilution.</description><subject>Acid mine drainage</subject><subject>Adsorption</subject><subject>Aluminum</subject><subject>Arsenic</subject><subject>Arsenic removal</subject><subject>Arsenite</subject><subject>Artificial wetlands</subject><subject>Chemical precipitation</subject><subject>Chemical reactions</subject><subject>Computational fluid dynamics</subject><subject>Computer simulation</subject><subject>Coprecipitation</subject><subject>Diffraction patterns</subject><subject>Dilution</subject><subject>Evaporation</subject><subject>Evaporation rate</subject><subject>Ferrous ions</subject><subject>Flow rates</subject><subject>Flow velocity</subject><subject>Fluid flow</subject><subject>Geochemistry & Geophysics</subject><subject>GETFLOWS</subject><subject>Inlet flow</subject><subject>Inlets 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Yoshiyuki</au><au>Tokoro, Chiharu</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Application of GETFLOWS Coupled with Chemical Reactions to Arsenic Removal through Ferrihydrite Coprecipitation in an Artificial Wetland of a Japanese Closed Mine</atitle><jtitle>Minerals (Basel)</jtitle><stitle>MINERALS-BASEL</stitle><date>2020-05-01</date><risdate>2020</risdate><volume>10</volume><issue>5</issue><spage>475</spage><pages>475-</pages><artnum>475</artnum><issn>2075-163X</issn><eissn>2075-163X</eissn><abstract>Passive systems that utilize a natural power such as a pond, plant, or microorganisms, is expected to be a cost-effective method for acid mine drainage (AMD) treatment. The Ningyo-toge mine, a non-operational uranium mine located in Okayama Prefecture, Japan, generates AMD containing arsenic and iron. To quantitatively study arsenic and iron ion removal in an artificial wetland and pond, chemical reactions were modeled and incorporated into the GETFLOWS (general-purpose terrestrial fluid-flow simulator) software. The chemical reaction models consisted of arsenite and ferrous oxidation equations and arsenic adsorption on ferrihydrite. The X-ray diffraction analysis of sediment samples showed ferrihydrite patterns. These results were consistent with the model for arsenite/ferrous oxidation and arsenic adsorption on ferrihydrite. Geofluid simulation was conducted to simulate mass transfer with the utilized topographic model, inlet flow rate, precipitation, and evaporation. The measured arsenic and iron ions concentrations in solution samples from the wetland and pond, fitted well with the model. This indicated that the main removal mechanism was the oxidation of arsenite/ferrous ions and that arsenic was removed by adsorption rather than dilution.</abstract><cop>BASEL</cop><pub>Mdpi</pub><doi>10.3390/min10050475</doi><tpages>16</tpages><orcidid>https://orcid.org/0000-0001-6214-0402</orcidid><oa>free_for_read</oa></addata></record> |
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| subjects | Acid mine drainage Adsorption Aluminum Arsenic Arsenic removal Arsenite Artificial wetlands Chemical precipitation Chemical reactions Computational fluid dynamics Computer simulation Coprecipitation Diffraction patterns Dilution Evaporation Evaporation rate Ferrous ions Flow rates Flow velocity Fluid flow Geochemistry & Geophysics GETFLOWS Inlet flow Inlets (waterways) Ions Iron Mass transfer Microorganisms Mine drainage Mineralogy Mines Mining & Mineral Processing Oxidation Physical Sciences Pollutant removal Ponds Precipitation quantitative modeling Removal Science & Technology Sediment samplers Sediment samples Simulation Simulators Studies surface complexation Surface water the three-dimensional topographic model Uranium Water pollution Wetlands X-ray diffraction X-ray diffraction analysis |
| title | Application of GETFLOWS Coupled with Chemical Reactions to Arsenic Removal through Ferrihydrite Coprecipitation in an Artificial Wetland of a Japanese Closed Mine |
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