Spatial patterns in Sr-87/Sr-86 ratios in modern human dental enamel and tap water from the Netherlands: Implications for forensic provenancing

The analysis of strontium isotope ratios in human dental enamel has become important in the fields of archaeological and forensic science for determining provenance and hence mobility. The prerequisite for the approach relies on a correlation between dietary Sr intake and the underlying local geolog...

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Veröffentlicht in:The Science of the total environment 2020-08, Vol.729, Article 138992
Hauptverfasser: Kootker, Lisette M., Plomp, Esther, Ammer, Saskia T. M., Hoogland, Vera, Davies, Gareth R.
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Sprache:eng
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Zusammenfassung:The analysis of strontium isotope ratios in human dental enamel has become important in the fields of archaeological and forensic science for determining provenance and hence mobility. The prerequisite for the approach relies on a correlation between dietary Sr intake and the underlying local geology. This premise is brought into question for anthropological forensic investigations by the increasing globalisation of food supply, the establishment of nation-wide or international supermarket chains, and increasing urbanisation. To better understand the processes that cause spatial variation of Sr isotope ratios in the modern environment, this study determines the range of Sr-87/Sr-86 ratios in the modern Dutch environment based on 296 modern human dental enamel and tap water samples. Tap water Sr-87/Sr-86 from the Netherlands range from 0.70837 to 0.71278 (Delta Srmax-min = 0.0044) and modern human enamel from 0.70847 to 0.70995 (Delta Srmax-min = 0.0015). The Sr-87/Sr-86 ratios of tap water are predominantly determined by the underlying bedrock geology at the sampling point. In contrast, the human enamel data record an insignificant, weak correlation with water supply or local geology. Hence, the main principle behind the application of Sr-87/Sr-86 as a proxy for mobility appears invalid in the modern globalised Dutch context. The range of Sr-87/Sr-86 in modern Dutch humans that can be used for anthropological forensic investigations is between 0.7085 and 0.7100 (n = 153), with 98.0% of individuals between 0.7088 and 0.7099. (c) 2020 The Authors. Published by Elsevier B.V. This is an open access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/).
ISSN:0048-9697
1879-1026
DOI:10.1016/j.scitotenv.2020.138992