Investigation of spontaneous emission dynamics of dye molecules coupled into transverse Anderson localized cavities in a hyperbolic waveguide
•Spontaneous emission of dye molecules coupled into multimode transverse Anderson localized modes in a hyperbolic waveguide is investigated.•Physics behind the transduction mechanism is explained with the coupling of the emitter emission into transverse Anderson localized modes.•Photonics design of...
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description | •Spontaneous emission of dye molecules coupled into multimode transverse Anderson localized modes in a hyperbolic waveguide is investigated.•Physics behind the transduction mechanism is explained with the coupling of the emitter emission into transverse Anderson localized modes.•Photonics design of the cavity allows generation of multimode Anderson localized modes.•A naturally formed disordered photonic medium in a simple hyperbolic waveguide is demonstrated to enhance light-matter interaction.
Spontaneous emission dynamics of rhodamine 6G molecules coupled into transverse Anderson localized modes in a hyperbolic waveguide is investigated using time-resolved experiments. Four hyperbolic waveguides are simultaneously formed inside a deltoid-shaped fused-silica microtube via the capillary effect. The disordered photonic environment consisting of a rhodamine-doped polymeric material with randomly distributed air inclusions is attributed to localize photons at various resonant wavelengths of the quasi-optical cavities, randomly positioned throughout the guiding medium. The hyperbolic waveguides allow obtaining a single, double, and multimode resonant structures, trapping photons at various frequencies as explored in the form of sharp spectral resonances within the photoluminescence spectrum bandwidth of the dye molecules. Experimental results reveal that the coupling of the fluorescent emitters into multimode localizations in each hyperbolic waveguide corresponds to obtaining quasi-optical cavities at various resonant frequencies, which alter the emission characteristics of the emitters distinctively. The spontaneous emission rate of the dye molecules coupled into the isolated transverse Anderson localized modes is observed to increase by a factor of up to 6.7; thus, the vacuum fluctuations at certain resonant wavelengths are considerably enhanced. |
doi_str_mv | 10.1016/j.photonics.2020.100769 |
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Spontaneous emission dynamics of rhodamine 6G molecules coupled into transverse Anderson localized modes in a hyperbolic waveguide is investigated using time-resolved experiments. Four hyperbolic waveguides are simultaneously formed inside a deltoid-shaped fused-silica microtube via the capillary effect. The disordered photonic environment consisting of a rhodamine-doped polymeric material with randomly distributed air inclusions is attributed to localize photons at various resonant wavelengths of the quasi-optical cavities, randomly positioned throughout the guiding medium. The hyperbolic waveguides allow obtaining a single, double, and multimode resonant structures, trapping photons at various frequencies as explored in the form of sharp spectral resonances within the photoluminescence spectrum bandwidth of the dye molecules. Experimental results reveal that the coupling of the fluorescent emitters into multimode localizations in each hyperbolic waveguide corresponds to obtaining quasi-optical cavities at various resonant frequencies, which alter the emission characteristics of the emitters distinctively. The spontaneous emission rate of the dye molecules coupled into the isolated transverse Anderson localized modes is observed to increase by a factor of up to 6.7; thus, the vacuum fluctuations at certain resonant wavelengths are considerably enhanced.</description><identifier>ISSN: 1569-4410</identifier><identifier>EISSN: 1569-4429</identifier><identifier>DOI: 10.1016/j.photonics.2020.100769</identifier><language>eng</language><publisher>AMSTERDAM: Elsevier B.V</publisher><subject>Capillarity ; Coupling (molecular) ; Dyes ; Emission analysis ; Emitters ; Fluorescence ; Fluorescence lifetime ; Inclusions ; Materials Science ; Materials Science, Multidisciplinary ; Nano-cavity ; Nanoscience & Nanotechnology ; Optical mode ; Optics ; Photoluminescence ; Photons ; Physical Sciences ; Physics ; Physics, Applied ; Resonant frequencies ; Rhodamine 6G ; Science & Technology ; Science & Technology - Other Topics ; Silicon dioxide ; Spontaneous emission ; Technology ; Transverse Anderson localization ; Waveguides ; Wavelengths</subject><ispartof>Photonics and nanostructures, 2020-05, Vol.39, p.100769, Article 100769</ispartof><rights>2020 Elsevier B.V.</rights><rights>Copyright Elsevier Science Ltd. May 2020</rights><woscitedreferencessubscribed>true</woscitedreferencessubscribed><woscitedreferencescount>1</woscitedreferencescount><woscitedreferencesoriginalsourcerecordid>wos000534605600003</woscitedreferencesoriginalsourcerecordid><citedby>FETCH-LOGICAL-c343t-42fed5434057465ea99fac6dc7aa74a080a89c73aa49d340676f14865ecdcccc3</citedby><cites>FETCH-LOGICAL-c343t-42fed5434057465ea99fac6dc7aa74a080a89c73aa49d340676f14865ecdcccc3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.photonics.2020.100769$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>315,782,786,3552,27931,27932,28255,46002</link.rule.ids></links><search><creatorcontrib>Gökbulut, Belkıs</creatorcontrib><creatorcontrib>Inci, Mehmet Naci</creatorcontrib><title>Investigation of spontaneous emission dynamics of dye molecules coupled into transverse Anderson localized cavities in a hyperbolic waveguide</title><title>Photonics and nanostructures</title><addtitle>PHOTONIC NANOSTRUCT</addtitle><description>•Spontaneous emission of dye molecules coupled into multimode transverse Anderson localized modes in a hyperbolic waveguide is investigated.•Physics behind the transduction mechanism is explained with the coupling of the emitter emission into transverse Anderson localized modes.•Photonics design of the cavity allows generation of multimode Anderson localized modes.•A naturally formed disordered photonic medium in a simple hyperbolic waveguide is demonstrated to enhance light-matter interaction.
Spontaneous emission dynamics of rhodamine 6G molecules coupled into transverse Anderson localized modes in a hyperbolic waveguide is investigated using time-resolved experiments. Four hyperbolic waveguides are simultaneously formed inside a deltoid-shaped fused-silica microtube via the capillary effect. The disordered photonic environment consisting of a rhodamine-doped polymeric material with randomly distributed air inclusions is attributed to localize photons at various resonant wavelengths of the quasi-optical cavities, randomly positioned throughout the guiding medium. The hyperbolic waveguides allow obtaining a single, double, and multimode resonant structures, trapping photons at various frequencies as explored in the form of sharp spectral resonances within the photoluminescence spectrum bandwidth of the dye molecules. Experimental results reveal that the coupling of the fluorescent emitters into multimode localizations in each hyperbolic waveguide corresponds to obtaining quasi-optical cavities at various resonant frequencies, which alter the emission characteristics of the emitters distinctively. The spontaneous emission rate of the dye molecules coupled into the isolated transverse Anderson localized modes is observed to increase by a factor of up to 6.7; thus, the vacuum fluctuations at certain resonant wavelengths are considerably enhanced.</description><subject>Capillarity</subject><subject>Coupling (molecular)</subject><subject>Dyes</subject><subject>Emission analysis</subject><subject>Emitters</subject><subject>Fluorescence</subject><subject>Fluorescence lifetime</subject><subject>Inclusions</subject><subject>Materials Science</subject><subject>Materials Science, Multidisciplinary</subject><subject>Nano-cavity</subject><subject>Nanoscience & Nanotechnology</subject><subject>Optical mode</subject><subject>Optics</subject><subject>Photoluminescence</subject><subject>Photons</subject><subject>Physical Sciences</subject><subject>Physics</subject><subject>Physics, Applied</subject><subject>Resonant frequencies</subject><subject>Rhodamine 6G</subject><subject>Science & Technology</subject><subject>Science & Technology - Other Topics</subject><subject>Silicon dioxide</subject><subject>Spontaneous emission</subject><subject>Technology</subject><subject>Transverse Anderson localization</subject><subject>Waveguides</subject><subject>Wavelengths</subject><issn>1569-4410</issn><issn>1569-4429</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><sourceid>AOWDO</sourceid><recordid>eNqNkMFq3DAQhk1poUnaZ6igx7Ib2ZLl9XFZmjQQyCU9i4k0TrR4Na4kO2zeIe9cuQ57TXWZYfg-jfQXxbeSr0teqsv9eniiRN6ZuK54NU95o9oPxVlZq3YlZdV-PPUl_1ycx7jnXAhVqrPi9cZPGJN7hOTIM-pYHMgn8EhjZHhwMc5ze_RwyBtmwB6RHahHM_YYmaFx6NEy5xOxFMDHCUNEtvU216z2ZKB3LxkxMLnksuM8A_Z0HDA8UO8Me4YJH0dn8UvxqYM-4te3elH8vvp5v_u1ur27vtltb1dGSJFWsurQ1lJIXjdS1Qht24FR1jQAjQS-4bBpTSMAZGszpRrVlXKTSWNNPuKi-L7cOwT6M-b_6z2NweeVupoDU7Jum0w1C2UCxRiw00NwBwhHXXI9Z6_3-pS9nrPXS_bZ3CzmMz5QF41Db_Bkc85rIRWvVe642Ln0L_wdjT5l9cf_q5neLjTmtCaHQb8Z1gU0SVty7z72L0fZttU</recordid><startdate>202005</startdate><enddate>202005</enddate><creator>Gökbulut, Belkıs</creator><creator>Inci, Mehmet Naci</creator><general>Elsevier B.V</general><general>Elsevier</general><general>Elsevier Science Ltd</general><scope>AOWDO</scope><scope>BLEPL</scope><scope>DTL</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7U5</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope></search><sort><creationdate>202005</creationdate><title>Investigation of spontaneous emission dynamics of dye molecules coupled into transverse Anderson localized cavities in a hyperbolic waveguide</title><author>Gökbulut, Belkıs ; Inci, Mehmet Naci</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c343t-42fed5434057465ea99fac6dc7aa74a080a89c73aa49d340676f14865ecdcccc3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>Capillarity</topic><topic>Coupling (molecular)</topic><topic>Dyes</topic><topic>Emission analysis</topic><topic>Emitters</topic><topic>Fluorescence</topic><topic>Fluorescence lifetime</topic><topic>Inclusions</topic><topic>Materials Science</topic><topic>Materials Science, Multidisciplinary</topic><topic>Nano-cavity</topic><topic>Nanoscience & Nanotechnology</topic><topic>Optical mode</topic><topic>Optics</topic><topic>Photoluminescence</topic><topic>Photons</topic><topic>Physical Sciences</topic><topic>Physics</topic><topic>Physics, Applied</topic><topic>Resonant frequencies</topic><topic>Rhodamine 6G</topic><topic>Science & Technology</topic><topic>Science & Technology - Other Topics</topic><topic>Silicon dioxide</topic><topic>Spontaneous emission</topic><topic>Technology</topic><topic>Transverse Anderson localization</topic><topic>Waveguides</topic><topic>Wavelengths</topic><toplevel>online_resources</toplevel><creatorcontrib>Gökbulut, Belkıs</creatorcontrib><creatorcontrib>Inci, Mehmet Naci</creatorcontrib><collection>Web of Science - Science Citation Index Expanded - 2020</collection><collection>Web of Science Core Collection</collection><collection>Science Citation Index Expanded</collection><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Photonics and nanostructures</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Gökbulut, Belkıs</au><au>Inci, Mehmet Naci</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Investigation of spontaneous emission dynamics of dye molecules coupled into transverse Anderson localized cavities in a hyperbolic waveguide</atitle><jtitle>Photonics and nanostructures</jtitle><stitle>PHOTONIC NANOSTRUCT</stitle><date>2020-05</date><risdate>2020</risdate><volume>39</volume><spage>100769</spage><pages>100769-</pages><artnum>100769</artnum><issn>1569-4410</issn><eissn>1569-4429</eissn><abstract>•Spontaneous emission of dye molecules coupled into multimode transverse Anderson localized modes in a hyperbolic waveguide is investigated.•Physics behind the transduction mechanism is explained with the coupling of the emitter emission into transverse Anderson localized modes.•Photonics design of the cavity allows generation of multimode Anderson localized modes.•A naturally formed disordered photonic medium in a simple hyperbolic waveguide is demonstrated to enhance light-matter interaction.
Spontaneous emission dynamics of rhodamine 6G molecules coupled into transverse Anderson localized modes in a hyperbolic waveguide is investigated using time-resolved experiments. Four hyperbolic waveguides are simultaneously formed inside a deltoid-shaped fused-silica microtube via the capillary effect. The disordered photonic environment consisting of a rhodamine-doped polymeric material with randomly distributed air inclusions is attributed to localize photons at various resonant wavelengths of the quasi-optical cavities, randomly positioned throughout the guiding medium. The hyperbolic waveguides allow obtaining a single, double, and multimode resonant structures, trapping photons at various frequencies as explored in the form of sharp spectral resonances within the photoluminescence spectrum bandwidth of the dye molecules. Experimental results reveal that the coupling of the fluorescent emitters into multimode localizations in each hyperbolic waveguide corresponds to obtaining quasi-optical cavities at various resonant frequencies, which alter the emission characteristics of the emitters distinctively. The spontaneous emission rate of the dye molecules coupled into the isolated transverse Anderson localized modes is observed to increase by a factor of up to 6.7; thus, the vacuum fluctuations at certain resonant wavelengths are considerably enhanced.</abstract><cop>AMSTERDAM</cop><pub>Elsevier B.V</pub><doi>10.1016/j.photonics.2020.100769</doi><tpages>10</tpages></addata></record> |
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subjects | Capillarity Coupling (molecular) Dyes Emission analysis Emitters Fluorescence Fluorescence lifetime Inclusions Materials Science Materials Science, Multidisciplinary Nano-cavity Nanoscience & Nanotechnology Optical mode Optics Photoluminescence Photons Physical Sciences Physics Physics, Applied Resonant frequencies Rhodamine 6G Science & Technology Science & Technology - Other Topics Silicon dioxide Spontaneous emission Technology Transverse Anderson localization Waveguides Wavelengths |
title | Investigation of spontaneous emission dynamics of dye molecules coupled into transverse Anderson localized cavities in a hyperbolic waveguide |
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