Muon Spin Relaxation Study of Frustrated Tm3Sb3Mg2O14 with Kagomé Lattice
The structure and magnetic properties of rare-earth ions Tm3+Kagomé lattice Tm3Sb3Mg2O14 are studied by x-ray diffraction,magnetic susceptibility and muon spin relaxation(μSR)experiments.The existence of a small amount of Tm/Mg site-mixing disorder is revealed.DC magnetic susceptibility measurement...
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| Veröffentlicht in: | Chinese physics letters 2022-10, Vol.39 (10), p.45-49 |
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| creator | Yang, Yanxing Chen, Kaiwen Ding, Zhaofeng Hillier, Adrian D. Shu, Lei |
| description | The structure and magnetic properties of rare-earth ions Tm3+Kagomé lattice Tm3Sb3Mg2O14 are studied by x-ray diffraction,magnetic susceptibility and muon spin relaxation(μSR)experiments.The existence of a small amount of Tm/Mg site-mixing disorder is revealed.DC magnetic susceptibility measurement shows that Tm3+magnetic moments are antiferromagnetically correlated with a negative Curie-Weiss temperature of-26.3K.Neither long-range magnetic order nor spin-glass transition is observed by DC and AC magnetic susceptibility,and confirmed by μSR experiment down to 0.1 K.However,the emergence of short-range magnetic order is indicated by the zero-field μSR experiments,and the absence of spin dynamics at low temperatures is evidenced by the longitudinal-field μSR technique.Compared with the results of Tm3Sb3Zn2O14,another Tm-based Kagomé lattice with much more site-mixing disorder,the gapless spin liquid like behaviors in Tm3Sb3Zn2O14 can be induced by disorder effect.Samples with perfect geometrical frustration are in urgent demand to establish whether QSL exists in this kind of materials with rare-earth Kagomé lattice. |
| doi_str_mv | 10.1088/0256-307X/39/10/107502 |
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Lett</addtitle><description>The structure and magnetic properties of rare-earth ions Tm3+Kagomé lattice Tm3Sb3Mg2O14 are studied by x-ray diffraction,magnetic susceptibility and muon spin relaxation(μSR)experiments.The existence of a small amount of Tm/Mg site-mixing disorder is revealed.DC magnetic susceptibility measurement shows that Tm3+magnetic moments are antiferromagnetically correlated with a negative Curie-Weiss temperature of-26.3K.Neither long-range magnetic order nor spin-glass transition is observed by DC and AC magnetic susceptibility,and confirmed by μSR experiment down to 0.1 K.However,the emergence of short-range magnetic order is indicated by the zero-field μSR experiments,and the absence of spin dynamics at low temperatures is evidenced by the longitudinal-field μSR technique.Compared with the results of Tm3Sb3Zn2O14,another Tm-based Kagomé lattice with much more site-mixing disorder,the gapless spin liquid like behaviors in Tm3Sb3Zn2O14 can be induced by disorder effect.Samples with perfect geometrical frustration are in urgent demand to establish whether QSL exists in this kind of materials with rare-earth Kagomé lattice.</description><issn>0256-307X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><recordid>eNpFkM1OwzAMgHMAiTF4BZQrhzI7adLmiCbG36ZJbAduUUqS0tG105pqwBvxHLwYrYpAsmzZ_mRLHyEXCFcIaToBJmTEIXmecDVB6CIRwI7I6G9xQk6bZgOAmCKOyMOirSu62hUVfXKleTeh6PvQ2g9aezrbt03Ym-AsXW_5KuOLnC0xpocivNJHk9fb7y86NyEUL-6MHHtTNu78t47Jenaznt5F8-Xt_fR6HhUshRA5yYyzqKRNUdlYMpHYVAlpvUTFEs4ThYozjgIcGulN5sFzIYX1cZf5mFwOZw-m8qbK9aZu91X3UH_mh_It044BYwgAqmPZwBb17p9D0L0s3TvRvRPN1TDsZfEfV5ldQA</recordid><startdate>20221001</startdate><enddate>20221001</enddate><creator>Yang, Yanxing</creator><creator>Chen, Kaiwen</creator><creator>Ding, Zhaofeng</creator><creator>Hillier, Adrian D.</creator><creator>Shu, Lei</creator><general>Chinese Physical Society and IOP Publishing Ltd</general><general>State Key Laboratory of Surface Physics,Department of Physics,Fudan University,Shanghai 200438,China%ISIS Facility,STFC Rutherford Appleton Laboratory,Chilton,Didcot,Oxfordshire,OX11 0QX,United Kingdom%State Key Laboratory of Surface Physics,Department of Physics,Fudan University,Shanghai 200438,China</general><general>Collaborative Innovation Center of Advanced Microstructures,Nanjing 210093,China</general><general>Shanghai Research Center for Quantum Sciences,Shanghai 201315,China</general><scope>2B.</scope><scope>4A8</scope><scope>92I</scope><scope>93N</scope><scope>PSX</scope><scope>TCJ</scope></search><sort><creationdate>20221001</creationdate><title>Muon Spin Relaxation Study of Frustrated Tm3Sb3Mg2O14 with Kagomé Lattice</title><author>Yang, Yanxing ; Chen, Kaiwen ; Ding, Zhaofeng ; Hillier, Adrian D. ; Shu, Lei</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-i280t-e62aed196d819d46257d8956df61927337919323150e1a6fabf0f3565df45653</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Yang, Yanxing</creatorcontrib><creatorcontrib>Chen, Kaiwen</creatorcontrib><creatorcontrib>Ding, Zhaofeng</creatorcontrib><creatorcontrib>Hillier, Adrian D.</creatorcontrib><creatorcontrib>Shu, Lei</creatorcontrib><collection>Wanfang Data Journals - Hong Kong</collection><collection>WANFANG Data Centre</collection><collection>Wanfang Data Journals</collection><collection>万方数据期刊 - 香港版</collection><collection>China Online Journals (COJ)</collection><collection>China Online Journals (COJ)</collection><jtitle>Chinese physics letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Yang, Yanxing</au><au>Chen, Kaiwen</au><au>Ding, Zhaofeng</au><au>Hillier, Adrian D.</au><au>Shu, Lei</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Muon Spin Relaxation Study of Frustrated Tm3Sb3Mg2O14 with Kagomé Lattice</atitle><jtitle>Chinese physics letters</jtitle><addtitle>Chinese Phys. Lett</addtitle><date>2022-10-01</date><risdate>2022</risdate><volume>39</volume><issue>10</issue><spage>45</spage><epage>49</epage><pages>45-49</pages><issn>0256-307X</issn><abstract>The structure and magnetic properties of rare-earth ions Tm3+Kagomé lattice Tm3Sb3Mg2O14 are studied by x-ray diffraction,magnetic susceptibility and muon spin relaxation(μSR)experiments.The existence of a small amount of Tm/Mg site-mixing disorder is revealed.DC magnetic susceptibility measurement shows that Tm3+magnetic moments are antiferromagnetically correlated with a negative Curie-Weiss temperature of-26.3K.Neither long-range magnetic order nor spin-glass transition is observed by DC and AC magnetic susceptibility,and confirmed by μSR experiment down to 0.1 K.However,the emergence of short-range magnetic order is indicated by the zero-field μSR experiments,and the absence of spin dynamics at low temperatures is evidenced by the longitudinal-field μSR technique.Compared with the results of Tm3Sb3Zn2O14,another Tm-based Kagomé lattice with much more site-mixing disorder,the gapless spin liquid like behaviors in Tm3Sb3Zn2O14 can be induced by disorder effect.Samples with perfect geometrical frustration are in urgent demand to establish whether QSL exists in this kind of materials with rare-earth Kagomé lattice.</abstract><pub>Chinese Physical Society and IOP Publishing Ltd</pub><doi>10.1088/0256-307X/39/10/107502</doi><tpages>5</tpages><oa>free_for_read</oa></addata></record> |
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| title | Muon Spin Relaxation Study of Frustrated Tm3Sb3Mg2O14 with Kagomé Lattice |
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