Experimental Protection of the Spin Coherence of a Molecular Qubit Exceeding a Millisecond

Molecular qubits are promising as they can benefit from tailoring and versatile design of chemistry. It is essential to reduce the decoherence of molecular qubits caused by their interactions with the environment. Herein the dynamical decoupling (DD) technique is utilized to combat such decoherence....

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Veröffentlicht in:Chinese physics letters 2021-03, Vol.38 (3), p.30303-中插10, Article 030303
Hauptverfasser: Dai, Yingqiu, Fu, Yue, Shi, Zhifu, Qin, Xi, Mu, Shiwei, Wu, Yang, Su, Ji-Hu, Deng, Yi-Fei, Qin, Lei, Zhai, Yuan-Qi, Zheng, Yan-Zhen, Rong, Xing, Du, Jiangfeng
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container_end_page 中插10
container_issue 3
container_start_page 30303
container_title Chinese physics letters
container_volume 38
creator Dai, Yingqiu
Fu, Yue
Shi, Zhifu
Qin, Xi
Mu, Shiwei
Wu, Yang
Su, Ji-Hu
Deng, Yi-Fei
Qin, Lei
Zhai, Yuan-Qi
Zheng, Yan-Zhen
Rong, Xing
Du, Jiangfeng
description Molecular qubits are promising as they can benefit from tailoring and versatile design of chemistry. It is essential to reduce the decoherence of molecular qubits caused by their interactions with the environment. Herein the dynamical decoupling (DD) technique is utilized to combat such decoherence. The coherence time for a transition-metal complex (PPh4)(2)[Cu(mnt)(2)] is prolonged from 6.8 mu s to 1.4 ms. The ratio of the coherence time and the length of pi/2 pulse, defined as the single qubit figure of merit (Q(M)), reaches 1.4 x 10(5), which is 40 times greater than what previously reported for this molecule. Our results show that molecular qubits, with milliseconds coherence time, are promising candidates for quantum information processing.
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subjects Physical Sciences
Physics
Physics, Multidisciplinary
Science & Technology
title Experimental Protection of the Spin Coherence of a Molecular Qubit Exceeding a Millisecond
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