Zeolite NaY-mediated oxidation of dyes with H2O2: unique heterogeneous non-transition metal center cleavage of H2O2 under visible light irradiation
This study investigated the visible-light catalysis mediated by zeolite NaY on the oxidation of dyes with H2O2. The results demonstrated that zeolite NaY acts as a sink for the electron from the photo-excited dye in the heterogeneous catalysis. Furthermore, the electron can effectively activate H2O2...
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| Veröffentlicht in: | Science China. Chemistry 2007-12, Vol.50 (6), p.770-775 |
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| container_end_page | 775 |
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| container_issue | 6 |
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| container_title | Science China. Chemistry |
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| creator | Liu, LiLi Ma, WanHong Song, WenJing Chen, ChunCheng Lin, Jun Zhao, JinCai Qian, XinHua Zhang, ShiBo |
| description | This study investigated the visible-light catalysis mediated by zeolite NaY on the oxidation of dyes with H2O2. The results demonstrated that zeolite NaY acts as a sink for the electron from the photo-excited dye in the heterogeneous catalysis. Furthermore, the electron can effectively activate H2O2 to produce ·OH radical that is a powerful oxidant for the oxidation of dye at room temperature. The effects of the framework topology, Si/Al ratio, and exchangeable cation of the zeolite on the oxidation of various dyes were also shown. |
| doi_str_mv | 10.1007/s11426-007-0138-1 |
| format | Article |
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The results demonstrated that zeolite NaY acts as a sink for the electron from the photo-excited dye in the heterogeneous catalysis. Furthermore, the electron can effectively activate H2O2 to produce ·OH radical that is a powerful oxidant for the oxidation of dye at room temperature. The effects of the framework topology, Si/Al ratio, and exchangeable cation of the zeolite on the oxidation of various dyes were also shown.</description><identifier>ISSN: 1006-9291</identifier><identifier>ISSN: 1674-7291</identifier><identifier>EISSN: 1862-2771</identifier><identifier>EISSN: 1869-1870</identifier><identifier>DOI: 10.1007/s11426-007-0138-1</identifier><language>eng</language><publisher>Heidelberg: Springer Nature B.V</publisher><subject>Catalysis ; Ductile-brittle transition ; Dyes ; Hydrogen peroxide ; Light irradiation ; Oxidation ; Oxidizing agents ; Room temperature ; Topology ; Transition metals ; Zeolites</subject><ispartof>Science China. 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All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c236t-c6c0d795258928cee36e3df08a9f7a1556036b601708797e9cb2f79da062cf5f3</citedby><cites>FETCH-LOGICAL-c236t-c6c0d795258928cee36e3df08a9f7a1556036b601708797e9cb2f79da062cf5f3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Uhttp://www.wanfangdata.com.cn/images/PeriodicalImages/zgkx-eb/zgkx-eb.jpg</thumbnail><linktohtml>$$Uhttps://www.proquest.com/docview/2918579920?pq-origsite=primo$$EHTML$$P50$$Gproquest$$H</linktohtml><link.rule.ids>314,780,784,21388,21389,21390,21391,23256,27924,27925,33530,33703,33744,34005,34314,43659,43787,43805,43953,44067,64385,64389,72341</link.rule.ids></links><search><creatorcontrib>Liu, LiLi</creatorcontrib><creatorcontrib>Ma, WanHong</creatorcontrib><creatorcontrib>Song, WenJing</creatorcontrib><creatorcontrib>Chen, ChunCheng</creatorcontrib><creatorcontrib>Lin, Jun</creatorcontrib><creatorcontrib>Zhao, JinCai</creatorcontrib><creatorcontrib>Qian, XinHua</creatorcontrib><creatorcontrib>Zhang, ShiBo</creatorcontrib><title>Zeolite NaY-mediated oxidation of dyes with H2O2: unique heterogeneous non-transition metal center cleavage of H2O2 under visible light irradiation</title><title>Science China. Chemistry</title><description>This study investigated the visible-light catalysis mediated by zeolite NaY on the oxidation of dyes with H2O2. The results demonstrated that zeolite NaY acts as a sink for the electron from the photo-excited dye in the heterogeneous catalysis. Furthermore, the electron can effectively activate H2O2 to produce ·OH radical that is a powerful oxidant for the oxidation of dye at room temperature. The effects of the framework topology, Si/Al ratio, and exchangeable cation of the zeolite on the oxidation of various dyes were also shown.</description><subject>Catalysis</subject><subject>Ductile-brittle transition</subject><subject>Dyes</subject><subject>Hydrogen peroxide</subject><subject>Light irradiation</subject><subject>Oxidation</subject><subject>Oxidizing agents</subject><subject>Room temperature</subject><subject>Topology</subject><subject>Transition metals</subject><subject>Zeolites</subject><issn>1006-9291</issn><issn>1674-7291</issn><issn>1862-2771</issn><issn>1869-1870</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2007</creationdate><recordtype>article</recordtype><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNpFkctuFDEQRVsIJELgA9hZyoaNSdk97Qc7FBESKUo2sCAby-Mu9zjpsYPtyYPfyA_jziCxqqvSqVuqul33kcFnBiCPC2MrLmiTFFivKHvVHTAlOOVSstdNAwiquWZvu3el3ACsVqDgoHu-xjSHiuTS_qJbHIOtOJL0GEZbQ4okeTI-YSEPoW7IGb_iX8guht87JBusmNOEEdOukJgirdnGEl7GtljtTBzGxhA3o723Ey5mi0VzGFv7PpSwnpHMYdpUEnK2y_Y2_b574-1c8MO_etj9PP324-SMXlx9Pz_5ekEd70WlTjgYpR74oDRXDrEX2I8elNVeWjYMAnqxFsAkKKklarfmXurRguDOD74_7D7tfR9s9DZO5ibtcmwbzZ_p9tHgmrd3ggBQDT3ao3c5teNL_c-2n6pBas2hUWxPuZxKyejNXQ5bm58MA7PEZPYxmUUuMRnW_wU0joZc</recordid><startdate>20071201</startdate><enddate>20071201</enddate><creator>Liu, LiLi</creator><creator>Ma, WanHong</creator><creator>Song, WenJing</creator><creator>Chen, ChunCheng</creator><creator>Lin, Jun</creator><creator>Zhao, JinCai</creator><creator>Qian, XinHua</creator><creator>Zhang, ShiBo</creator><general>Springer Nature B.V</general><general>Institute of Chemistry, Chinese Academy of Sciences, Beijing 100080, China%Department of Chemistry, Renmin University of China, Beijing 100872, China%Fushun Petrochemical Company, PetroChina Company Limited, Fushun 113008, China</general><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7XB</scope><scope>88I</scope><scope>8FE</scope><scope>8FG</scope><scope>8FK</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>GNUQQ</scope><scope>HCIFZ</scope><scope>KB.</scope><scope>M2P</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>Q9U</scope><scope>2B.</scope><scope>4A8</scope><scope>92I</scope><scope>93N</scope><scope>PSX</scope><scope>TCJ</scope></search><sort><creationdate>20071201</creationdate><title>Zeolite NaY-mediated oxidation of dyes with H2O2: unique heterogeneous non-transition metal center cleavage of H2O2 under visible light irradiation</title><author>Liu, LiLi ; 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Chemistry</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Liu, LiLi</au><au>Ma, WanHong</au><au>Song, WenJing</au><au>Chen, ChunCheng</au><au>Lin, Jun</au><au>Zhao, JinCai</au><au>Qian, XinHua</au><au>Zhang, ShiBo</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Zeolite NaY-mediated oxidation of dyes with H2O2: unique heterogeneous non-transition metal center cleavage of H2O2 under visible light irradiation</atitle><jtitle>Science China. Chemistry</jtitle><date>2007-12-01</date><risdate>2007</risdate><volume>50</volume><issue>6</issue><spage>770</spage><epage>775</epage><pages>770-775</pages><issn>1006-9291</issn><issn>1674-7291</issn><eissn>1862-2771</eissn><eissn>1869-1870</eissn><abstract>This study investigated the visible-light catalysis mediated by zeolite NaY on the oxidation of dyes with H2O2. The results demonstrated that zeolite NaY acts as a sink for the electron from the photo-excited dye in the heterogeneous catalysis. Furthermore, the electron can effectively activate H2O2 to produce ·OH radical that is a powerful oxidant for the oxidation of dye at room temperature. The effects of the framework topology, Si/Al ratio, and exchangeable cation of the zeolite on the oxidation of various dyes were also shown.</abstract><cop>Heidelberg</cop><pub>Springer Nature B.V</pub><doi>10.1007/s11426-007-0138-1</doi><tpages>6</tpages></addata></record> |
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| subjects | Catalysis Ductile-brittle transition Dyes Hydrogen peroxide Light irradiation Oxidation Oxidizing agents Room temperature Topology Transition metals Zeolites |
| title | Zeolite NaY-mediated oxidation of dyes with H2O2: unique heterogeneous non-transition metal center cleavage of H2O2 under visible light irradiation |
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