PCDD/Fs in soil around a hospital waste incinerator: comparison after three years of operation
Polychlorinated dibenzo-p-dioxins and dibenzofurans (PCDD/Fs) can be formed during the cooling of flue gases in waste incinerator. These pollutants are either in the gas phase or attached to the fine particles, escaping dust collection. After stack emission, they are slowly oxidized photochemically...
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Veröffentlicht in: | Journal of environmental sciences (China) 2012-04, Vol.24 (4), p.699-703 |
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description | Polychlorinated dibenzo-p-dioxins and dibenzofurans (PCDD/Fs) can be formed during the cooling of flue gases in waste incinerator. These pollutants are either in the gas phase or attached to the fine particles, escaping dust collection. After stack emission, they are slowly oxidized photochemically (gas phase), or eventually are deposited (dry and wet deposition of particulate) in earth surface. In 2007 and 2010, 11 soil samples were collected in the vicinity of a hospital waste incinerator (HWI), prior and after its startup. In order to find out any variation of PCDD/Fs in soil, in brief dioxins, their concentrations were analyzed by high-resolution gas chromatography with high-resolution mass spectrometry (HRGC/HRMS). Compared to the baseline survey (2007), PCDD/Fs in soil significantly increased, by average, +81.6% in total PCDD/Fs and +132.7% in international toxic equivalency (I-TEQ) unit. By principal component analysis (PCA), both the PCDD/Fs homologue and the HxCDF isomer profile in soil were found to become more similar with fly ash. Generally, this incinerator influences the soil only in a limited area. More comprehensive supervision, stricter management and more advanced technology should be implemented in this plant to reduce pollutants emission, even though the level of PCDD/Fs in soil is quite low at present. |
doi_str_mv | 10.1016/S1001-0742(11)60752-3 |
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These pollutants are either in the gas phase or attached to the fine particles, escaping dust collection. After stack emission, they are slowly oxidized photochemically (gas phase), or eventually are deposited (dry and wet deposition of particulate) in earth surface. In 2007 and 2010, 11 soil samples were collected in the vicinity of a hospital waste incinerator (HWI), prior and after its startup. In order to find out any variation of PCDD/Fs in soil, in brief dioxins, their concentrations were analyzed by high-resolution gas chromatography with high-resolution mass spectrometry (HRGC/HRMS). Compared to the baseline survey (2007), PCDD/Fs in soil significantly increased, by average, +81.6% in total PCDD/Fs and +132.7% in international toxic equivalency (I-TEQ) unit. By principal component analysis (PCA), both the PCDD/Fs homologue and the HxCDF isomer profile in soil were found to become more similar with fly ash. Generally, this incinerator influences the soil only in a limited area. More comprehensive supervision, stricter management and more advanced technology should be implemented in this plant to reduce pollutants emission, even though the level of PCDD/Fs in soil is quite low at present.</description><identifier>ISSN: 1001-0742</identifier><identifier>EISSN: 1878-7320</identifier><identifier>DOI: 10.1016/S1001-0742(11)60752-3</identifier><identifier>PMID: 22894105</identifier><language>eng</language><publisher>Netherlands: Elsevier B.V</publisher><subject>Benzofurans - analysis ; Benzofurans - chemistry ; China ; Data Collection ; Deposition ; Dibenzofurans, Polychlorinated ; dioxin ; Environmental Monitoring ; Flue gases ; Gas phases ; Geography ; Hospitals ; Incineration - instrumentation ; Incinerators ; Isomerism ; Medical Waste Disposal - instrumentation ; PCDD ; Pollutants ; Polychlorinated Dibenzodioxins - analogs & derivatives ; Polychlorinated Dibenzodioxins - analysis ; Polychlorinated Dibenzodioxins - chemistry ; Principal Component Analysis ; soil ; Soil (material) ; Soil - chemistry ; Soil Pollutants - analysis ; variation ; waste incinerator ; Wastes ; 医院 ; 土壤 ; 垃圾焚烧炉 ; 气相色谱分析 ; 污染物排放 ; 运作 ; 颗粒沉积</subject><ispartof>Journal of environmental sciences (China), 2012-04, Vol.24 (4), p.699-703</ispartof><rights>2012 The Research Centre for Eco-Environmental Sciences, Chinese Academy of Sciences</rights><rights>Copyright © Wanfang Data Co. Ltd. All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c488t-bee4979ed75b89ffb406f0d48d63e01409753e72ed62a82b11cf5275629ad55c3</citedby><cites>FETCH-LOGICAL-c488t-bee4979ed75b89ffb406f0d48d63e01409753e72ed62a82b11cf5275629ad55c3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Uhttp://image.cqvip.com/vip1000/qk/85265X/85265X.jpg</thumbnail><linktohtml>$$Uhttps://www.sciencedirect.com/science/article/pii/S1001074211607523$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,776,780,3537,27901,27902,65306</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/22894105$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Li, Xiaodong</creatorcontrib><creatorcontrib>Yan, Mi</creatorcontrib><creatorcontrib>Yang, Jie</creatorcontrib><creatorcontrib>Chen, Tong</creatorcontrib><creatorcontrib>Lu, Shengyong</creatorcontrib><creatorcontrib>Yan, Jianhua</creatorcontrib><title>PCDD/Fs in soil around a hospital waste incinerator: comparison after three years of operation</title><title>Journal of environmental sciences (China)</title><addtitle>Journal of Environmental Sciences</addtitle><description>Polychlorinated dibenzo-p-dioxins and dibenzofurans (PCDD/Fs) can be formed during the cooling of flue gases in waste incinerator. These pollutants are either in the gas phase or attached to the fine particles, escaping dust collection. After stack emission, they are slowly oxidized photochemically (gas phase), or eventually are deposited (dry and wet deposition of particulate) in earth surface. In 2007 and 2010, 11 soil samples were collected in the vicinity of a hospital waste incinerator (HWI), prior and after its startup. In order to find out any variation of PCDD/Fs in soil, in brief dioxins, their concentrations were analyzed by high-resolution gas chromatography with high-resolution mass spectrometry (HRGC/HRMS). Compared to the baseline survey (2007), PCDD/Fs in soil significantly increased, by average, +81.6% in total PCDD/Fs and +132.7% in international toxic equivalency (I-TEQ) unit. By principal component analysis (PCA), both the PCDD/Fs homologue and the HxCDF isomer profile in soil were found to become more similar with fly ash. Generally, this incinerator influences the soil only in a limited area. More comprehensive supervision, stricter management and more advanced technology should be implemented in this plant to reduce pollutants emission, even though the level of PCDD/Fs in soil is quite low at present.</description><subject>Benzofurans - analysis</subject><subject>Benzofurans - chemistry</subject><subject>China</subject><subject>Data Collection</subject><subject>Deposition</subject><subject>Dibenzofurans, Polychlorinated</subject><subject>dioxin</subject><subject>Environmental Monitoring</subject><subject>Flue gases</subject><subject>Gas phases</subject><subject>Geography</subject><subject>Hospitals</subject><subject>Incineration - instrumentation</subject><subject>Incinerators</subject><subject>Isomerism</subject><subject>Medical Waste Disposal - instrumentation</subject><subject>PCDD</subject><subject>Pollutants</subject><subject>Polychlorinated Dibenzodioxins - analogs & derivatives</subject><subject>Polychlorinated Dibenzodioxins - analysis</subject><subject>Polychlorinated Dibenzodioxins - chemistry</subject><subject>Principal Component Analysis</subject><subject>soil</subject><subject>Soil (material)</subject><subject>Soil - chemistry</subject><subject>Soil Pollutants - analysis</subject><subject>variation</subject><subject>waste incinerator</subject><subject>Wastes</subject><subject>医院</subject><subject>土壤</subject><subject>垃圾焚烧炉</subject><subject>气相色谱分析</subject><subject>污染物排放</subject><subject>运作</subject><subject>颗粒沉积</subject><issn>1001-0742</issn><issn>1878-7320</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2012</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqN0U9u1DAUBvAIgWgpHAFkNqgsQv38PyuEphSQKoEErI2TvHQ8ythTO6HqVTgLd-IKeDozbMvKlvyzP-t9VfUc6BugoM6-AqVQUy3YKcBrRbVkNX9QHYPRptac0YdlfyBH1ZOcV5RSIal8XB0xZhoBVB5XP74szs_PLjLxgeToR-JSnENPHFnGvPGTG8mNyxOW884HTG6K6c_vX6SL641LPsdA3DBhItMyIZJbdCmTOJC42Vofw9Pq0eDGjM_260n1_eL9t8XH-vLzh0-Ld5d1J4yZ6hZRNLrBXsvWNMPQCqoG2gvTK44UBG205KgZ9oo5w1qAbpBMS8Ua10vZ8ZPq1e7dGxcGF67sKs4plES7wmyRUWBUUNAFnu7gJsXrGfNk1z53OI4uYJyzBaWBK2lK3r2UcsEoZ4L9B4UycMMNFCp3tEsx54SD3SS_dum2oK1T9q5buy3OAti7bi0v917sI-Z2jf2_W4cyC3i7A1jm_NNjsrnzGDrsfcJusn3090a83H9tGcPVtS9jPKQIUKCMafhfJ8u9gg</recordid><startdate>201204</startdate><enddate>201204</enddate><creator>Li, Xiaodong</creator><creator>Yan, Mi</creator><creator>Yang, Jie</creator><creator>Chen, Tong</creator><creator>Lu, Shengyong</creator><creator>Yan, Jianhua</creator><general>Elsevier B.V</general><general>State Key Laboratory of Clean Energy Utilization, Zhejiang University, Hangzhou 310027, China</general><scope>2RA</scope><scope>92L</scope><scope>CQIGP</scope><scope>W92</scope><scope>~WA</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7ST</scope><scope>7TV</scope><scope>C1K</scope><scope>SOI</scope><scope>7X8</scope><scope>7SU</scope><scope>8FD</scope><scope>FR3</scope><scope>KR7</scope><scope>2B.</scope><scope>4A8</scope><scope>92I</scope><scope>93N</scope><scope>PSX</scope><scope>TCJ</scope></search><sort><creationdate>201204</creationdate><title>PCDD/Fs in soil around a hospital waste incinerator: comparison after three years of operation</title><author>Li, Xiaodong ; Yan, Mi ; Yang, Jie ; Chen, Tong ; Lu, Shengyong ; Yan, Jianhua</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c488t-bee4979ed75b89ffb406f0d48d63e01409753e72ed62a82b11cf5275629ad55c3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2012</creationdate><topic>Benzofurans - analysis</topic><topic>Benzofurans - chemistry</topic><topic>China</topic><topic>Data Collection</topic><topic>Deposition</topic><topic>Dibenzofurans, Polychlorinated</topic><topic>dioxin</topic><topic>Environmental Monitoring</topic><topic>Flue gases</topic><topic>Gas phases</topic><topic>Geography</topic><topic>Hospitals</topic><topic>Incineration - instrumentation</topic><topic>Incinerators</topic><topic>Isomerism</topic><topic>Medical Waste Disposal - instrumentation</topic><topic>PCDD</topic><topic>Pollutants</topic><topic>Polychlorinated Dibenzodioxins - analogs & derivatives</topic><topic>Polychlorinated Dibenzodioxins - analysis</topic><topic>Polychlorinated Dibenzodioxins - chemistry</topic><topic>Principal Component Analysis</topic><topic>soil</topic><topic>Soil (material)</topic><topic>Soil - chemistry</topic><topic>Soil Pollutants - analysis</topic><topic>variation</topic><topic>waste incinerator</topic><topic>Wastes</topic><topic>医院</topic><topic>土壤</topic><topic>垃圾焚烧炉</topic><topic>气相色谱分析</topic><topic>污染物排放</topic><topic>运作</topic><topic>颗粒沉积</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Li, Xiaodong</creatorcontrib><creatorcontrib>Yan, Mi</creatorcontrib><creatorcontrib>Yang, Jie</creatorcontrib><creatorcontrib>Chen, Tong</creatorcontrib><creatorcontrib>Lu, Shengyong</creatorcontrib><creatorcontrib>Yan, Jianhua</creatorcontrib><collection>中文科技期刊数据库</collection><collection>中文科技期刊数据库-CALIS站点</collection><collection>中文科技期刊数据库-7.0平台</collection><collection>中文科技期刊数据库-工程技术</collection><collection>中文科技期刊数据库- 镜像站点</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>Environment Abstracts</collection><collection>Pollution Abstracts</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Environment Abstracts</collection><collection>MEDLINE - Academic</collection><collection>Environmental Engineering Abstracts</collection><collection>Technology Research Database</collection><collection>Engineering Research Database</collection><collection>Civil Engineering Abstracts</collection><collection>Wanfang Data Journals - Hong Kong</collection><collection>WANFANG Data Centre</collection><collection>Wanfang Data Journals</collection><collection>万方数据期刊 - 香港版</collection><collection>China Online Journals (COJ)</collection><collection>China Online Journals (COJ)</collection><jtitle>Journal of environmental sciences (China)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Li, Xiaodong</au><au>Yan, Mi</au><au>Yang, Jie</au><au>Chen, Tong</au><au>Lu, Shengyong</au><au>Yan, Jianhua</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>PCDD/Fs in soil around a hospital waste incinerator: comparison after three years of operation</atitle><jtitle>Journal of environmental sciences (China)</jtitle><addtitle>Journal of Environmental Sciences</addtitle><date>2012-04</date><risdate>2012</risdate><volume>24</volume><issue>4</issue><spage>699</spage><epage>703</epage><pages>699-703</pages><issn>1001-0742</issn><eissn>1878-7320</eissn><abstract>Polychlorinated dibenzo-p-dioxins and dibenzofurans (PCDD/Fs) can be formed during the cooling of flue gases in waste incinerator. These pollutants are either in the gas phase or attached to the fine particles, escaping dust collection. After stack emission, they are slowly oxidized photochemically (gas phase), or eventually are deposited (dry and wet deposition of particulate) in earth surface. In 2007 and 2010, 11 soil samples were collected in the vicinity of a hospital waste incinerator (HWI), prior and after its startup. In order to find out any variation of PCDD/Fs in soil, in brief dioxins, their concentrations were analyzed by high-resolution gas chromatography with high-resolution mass spectrometry (HRGC/HRMS). Compared to the baseline survey (2007), PCDD/Fs in soil significantly increased, by average, +81.6% in total PCDD/Fs and +132.7% in international toxic equivalency (I-TEQ) unit. By principal component analysis (PCA), both the PCDD/Fs homologue and the HxCDF isomer profile in soil were found to become more similar with fly ash. Generally, this incinerator influences the soil only in a limited area. More comprehensive supervision, stricter management and more advanced technology should be implemented in this plant to reduce pollutants emission, even though the level of PCDD/Fs in soil is quite low at present.</abstract><cop>Netherlands</cop><pub>Elsevier B.V</pub><pmid>22894105</pmid><doi>10.1016/S1001-0742(11)60752-3</doi><tpages>5</tpages></addata></record> |
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source | MEDLINE; Elsevier ScienceDirect Journals; Alma/SFX Local Collection |
subjects | Benzofurans - analysis Benzofurans - chemistry China Data Collection Deposition Dibenzofurans, Polychlorinated dioxin Environmental Monitoring Flue gases Gas phases Geography Hospitals Incineration - instrumentation Incinerators Isomerism Medical Waste Disposal - instrumentation PCDD Pollutants Polychlorinated Dibenzodioxins - analogs & derivatives Polychlorinated Dibenzodioxins - analysis Polychlorinated Dibenzodioxins - chemistry Principal Component Analysis soil Soil (material) Soil - chemistry Soil Pollutants - analysis variation waste incinerator Wastes 医院 土壤 垃圾焚烧炉 气相色谱分析 污染物排放 运作 颗粒沉积 |
title | PCDD/Fs in soil around a hospital waste incinerator: comparison after three years of operation |
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