New flexible CsPbBr3-based scintillator for X-ray tomography

The evolution of lead halide perovskites used for X-ray imaging scintillators has been facilitated by the development of solution-processable semiconductors characterized by large-area, flexible, fast photoresponse. The stability and durability of these new perovskites are insufficient to achieve ex...

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Veröffentlicht in:Nuclear science and techniques 2022-08, Vol.33 (8), p.34-44, Article 98
Hauptverfasser: Lü, Zhi-Wei, Wei, Gong-Xiang, Wang, Han-Qiu, Guan, Yu, Jiang, Ning, Liu, Yun-Yan, Li, Zhao, Qin, Hua, Liu, Hui-Qiang
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Sprache:eng
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Zusammenfassung:The evolution of lead halide perovskites used for X-ray imaging scintillators has been facilitated by the development of solution-processable semiconductors characterized by large-area, flexible, fast photoresponse. The stability and durability of these new perovskites are insufficient to achieve extended computed tomography scanning times with hard X-rays. In this study, we fabricated a self-assembled CsPbBr 3 -based scintillator film with a flexible large-area uniform thickness using a new room-temperature solution-processable method. The sensitivity and responsivity of X-ray photon conversion were quantitatively measured and showed a good linear response relationship suitable for X-ray imaging. We also demonstrated, for the first time, that the self-assembled CsPbBr 3 -based scintillator has good stability for hard X-ray microtomography. Therefore, such an inexpensive solution-processed semiconductor easily prepared at room temperature can be used as a hard X-ray scintillator and equipped with flexible CsPbBr 3 -based X-ray detectors. It has great potential in three-dimensional high-resolution phase-contrast X-ray-imaging applications in biomedicine and material science because of its heavy Pb and Br atoms.
ISSN:1001-8042
2210-3147
DOI:10.1007/s41365-022-01085-z