Ground-Based Atmospheric CO2, CH4, and CO Column Measurements at Golmud in the Qinghai-Tibetan Plateau and Comparisons with TROPOMI/S5P Satellite Observations

Measurements of carbon dioxide (CO 2 ), methane (CH 4 ), and carbon monoxide (CO) are of great importance in the Qinghai-Tibetan region, as it is the highest and largest plateau in the world affecting global weather and climate systems. In this study, for the first time, we present CO 2 , CH 4 , and...

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Veröffentlicht in:Advances in atmospheric sciences 2023-02, Vol.40 (2), p.223-234
Hauptverfasser: Zhou, Minqiang, Ni, Qichen, Cai, Zhaonan, Langerock, Bavo, Jiang, Jingyi, Che, Ke, Wang, Jiaxin, Nan, Weidong, Liu, Yi, Wang, Pucai
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container_issue 2
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container_title Advances in atmospheric sciences
container_volume 40
creator Zhou, Minqiang
Ni, Qichen
Cai, Zhaonan
Langerock, Bavo
Jiang, Jingyi
Che, Ke
Wang, Jiaxin
Nan, Weidong
Liu, Yi
Wang, Pucai
description Measurements of carbon dioxide (CO 2 ), methane (CH 4 ), and carbon monoxide (CO) are of great importance in the Qinghai-Tibetan region, as it is the highest and largest plateau in the world affecting global weather and climate systems. In this study, for the first time, we present CO 2 , CH 4 , and CO column measurements carried out by a Bruker EM27/SUN Fourier-transform infrared spectrometer (FTIR) at Golmud (36.42°E, 94.91°N, 2808 m) in August 2021. The mean and standard deviation of the column-average dry-air mixing ratio of CO 2 , CH 4 , and CO (XCO 2 , XCH 4 , and XCO) are 409.3 ± 0.4 ppm, 1905.5 ± 19.4 ppb, and 103.1 ± 7.7 ppb, respectively. The differences between the FTIR co-located TROPOMI/S5P satellite measurements at Golmud are 0.68 ± 0.64% (13.1 ± 12.2 ppb) for XCH 4 and 9.81 ± 3.48% (−10.7 ± 3.8 ppb) for XCO, which are within their retrieval uncertainties. High correlations for both XCH 4 and XCO are observed between the FTIR and S5P satellite measurements. Using the FLEXPART model and satellite measurements, we find that enhanced CH 4 and CO columns in Golmud are affected by anthropogenic emissions transported from North India. This study provides an insight into the variations of the CO 2 , CH 4 , and CO columns in the Qinghai-Tibetan Plateau.
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High correlations for both XCH 4 and XCO are observed between the FTIR and S5P satellite measurements. Using the FLEXPART model and satellite measurements, we find that enhanced CH 4 and CO columns in Golmud are affected by anthropogenic emissions transported from North India. 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subjects Anthropogenic factors
Atmospheric Sciences
Carbon dioxide
Carbon dioxide measurements
Carbon monoxide
Carbon Neutrality: Important Roles of Renewable Energies
Carbon Sinks
Climate system
Earth and Environmental Science
Earth Sciences
Emissions
Fourier transforms
FTIR spectrometers
Geophysics/Geodesy
Global weather
Infrared spectrometers
Infrared spectroscopy
Meteorological satellites
Meteorology
Methane
Mixing ratio
NETs
non-CO2 GHGs
Original Paper
Plateaus
Satellite observation
Satellites
title Ground-Based Atmospheric CO2, CH4, and CO Column Measurements at Golmud in the Qinghai-Tibetan Plateau and Comparisons with TROPOMI/S5P Satellite Observations
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