Enhanced comprehensive energy storage properties in Bi0.5Na0.5TiO3-based relaxor ferroelectric ceramics under a moderate electric field
Bismuth sodium titanate (Bi0.5Na0.5TiO3)-based relaxor ferroelectric ceramics have received ever-increasing interest for their potential application in dielectric capacitors owing to their sterling energy storage capability. Herein, the perovskite end-member Ba(Fe0.5Nb0.5)O3 (BFN) was incorporated i...
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| Veröffentlicht in: | Applied physics letters 2024-06, Vol.124 (25) |
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| creator | Jiang, Shunshun Zhang, Ji Luo, Huajie Liu, Lisha Li, Jinglei Karpinsky, Dmitry V. Wang, Jing Wang, Yaojin |
| description | Bismuth sodium titanate (Bi0.5Na0.5TiO3)-based relaxor ferroelectric ceramics have received ever-increasing interest for their potential application in dielectric capacitors owing to their sterling energy storage capability. Herein, the perovskite end-member Ba(Fe0.5Nb0.5)O3 (BFN) was incorporated into 0.7Bi0.5Na0.5TiO3-0.3SrTiO3 (0.7BNT-0.3ST) ceramics to improve the relaxor characteristics and refine the grain, leading to slim polarization–electric field (P–E) hysteresis loops and enhanced electric breakdown strength. Particularly, the 0.85(0.7BNT-0.3ST)-0.15BFN ceramics achieved a high recoverable energy density of 5.7 J/cm3 and a high energy storage efficiency of 86.4% under a moderate electric field of 390 kV/cm. Additionally, remarkable stability in frequency, cycling, and temperature and excellent charge/discharge behavior were achieved at the same time. The above findings reveal that BFN-modified BNT-ST ceramics display greatly improved comprehensive energy storage properties, making them promising candidates in the field of electrostatic energy storage. |
| doi_str_mv | 10.1063/5.0217327 |
| format | Article |
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Herein, the perovskite end-member Ba(Fe0.5Nb0.5)O3 (BFN) was incorporated into 0.7Bi0.5Na0.5TiO3-0.3SrTiO3 (0.7BNT-0.3ST) ceramics to improve the relaxor characteristics and refine the grain, leading to slim polarization–electric field (P–E) hysteresis loops and enhanced electric breakdown strength. Particularly, the 0.85(0.7BNT-0.3ST)-0.15BFN ceramics achieved a high recoverable energy density of 5.7 J/cm3 and a high energy storage efficiency of 86.4% under a moderate electric field of 390 kV/cm. Additionally, remarkable stability in frequency, cycling, and temperature and excellent charge/discharge behavior were achieved at the same time. The above findings reveal that BFN-modified BNT-ST ceramics display greatly improved comprehensive energy storage properties, making them promising candidates in the field of electrostatic energy storage.</description><identifier>ISSN: 0003-6951</identifier><identifier>EISSN: 1077-3118</identifier><identifier>DOI: 10.1063/5.0217327</identifier><identifier>CODEN: APPLAB</identifier><language>eng</language><publisher>Melville: American Institute of Physics</publisher><subject>Bismuth titanate ; Ceramics ; Electric fields ; Energy storage ; Ferroelectric materials ; Ferroelectricity ; Frequency stability ; Hysteresis loops ; Perovskites ; Relaxors ; Sodium titanate</subject><ispartof>Applied physics letters, 2024-06, Vol.124 (25)</ispartof><rights>Author(s)</rights><rights>2024 Author(s). Published under an exclusive license by AIP Publishing.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><orcidid>0000-0003-2561-1855 ; 0000-0001-5447-6301 ; 0000-0001-5858-5046 ; 0000-0001-9471-5493 ; 0000-0002-7752-1758</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://pubs.aip.org/apl/article-lookup/doi/10.1063/5.0217327$$EHTML$$P50$$Gscitation$$H</linktohtml><link.rule.ids>314,780,784,794,4512,27924,27925,76384</link.rule.ids></links><search><creatorcontrib>Jiang, Shunshun</creatorcontrib><creatorcontrib>Zhang, Ji</creatorcontrib><creatorcontrib>Luo, Huajie</creatorcontrib><creatorcontrib>Liu, Lisha</creatorcontrib><creatorcontrib>Li, Jinglei</creatorcontrib><creatorcontrib>Karpinsky, Dmitry V.</creatorcontrib><creatorcontrib>Wang, Jing</creatorcontrib><creatorcontrib>Wang, Yaojin</creatorcontrib><title>Enhanced comprehensive energy storage properties in Bi0.5Na0.5TiO3-based relaxor ferroelectric ceramics under a moderate electric field</title><title>Applied physics letters</title><description>Bismuth sodium titanate (Bi0.5Na0.5TiO3)-based relaxor ferroelectric ceramics have received ever-increasing interest for their potential application in dielectric capacitors owing to their sterling energy storage capability. Herein, the perovskite end-member Ba(Fe0.5Nb0.5)O3 (BFN) was incorporated into 0.7Bi0.5Na0.5TiO3-0.3SrTiO3 (0.7BNT-0.3ST) ceramics to improve the relaxor characteristics and refine the grain, leading to slim polarization–electric field (P–E) hysteresis loops and enhanced electric breakdown strength. Particularly, the 0.85(0.7BNT-0.3ST)-0.15BFN ceramics achieved a high recoverable energy density of 5.7 J/cm3 and a high energy storage efficiency of 86.4% under a moderate electric field of 390 kV/cm. Additionally, remarkable stability in frequency, cycling, and temperature and excellent charge/discharge behavior were achieved at the same time. The above findings reveal that BFN-modified BNT-ST ceramics display greatly improved comprehensive energy storage properties, making them promising candidates in the field of electrostatic energy storage.</description><subject>Bismuth titanate</subject><subject>Ceramics</subject><subject>Electric fields</subject><subject>Energy storage</subject><subject>Ferroelectric materials</subject><subject>Ferroelectricity</subject><subject>Frequency stability</subject><subject>Hysteresis loops</subject><subject>Perovskites</subject><subject>Relaxors</subject><subject>Sodium titanate</subject><issn>0003-6951</issn><issn>1077-3118</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNo1kM1OwzAQhC0EEqVw4A0scUNKsePYcY5QlR-popdyjhxn3bpKnGC7iD4Br41Ry2VHK327oxmEbimZUSLYA5-RnJYsL8_QhJKyzBil8hxNCCEsExWnl-gqhF1aec7YBP0s3FY5DS3WQz962IIL9gswOPCbAw5x8GoDePTDCD5aCNg6_GTJjL-rNNZ2xbJGhXTvoVPfg8cGvB-gAx291ViDV73VAe9dCx4r3A9JVUwO_4ix0LXX6MKoLsDNSafo43mxnr9my9XL2_xxmY20kDGrRCV5VRXUgK6EKYigouBAGgNSKiNp25i8kTktcpkScllKUEpKTmnBGijYFN0d_6ZEn3sIsd4Ne--SZc2IkLKSNBeJuj9SQduooh1cPXrbK3-oKan_iq55fSqa_QIVbnAc</recordid><startdate>20240617</startdate><enddate>20240617</enddate><creator>Jiang, Shunshun</creator><creator>Zhang, Ji</creator><creator>Luo, Huajie</creator><creator>Liu, Lisha</creator><creator>Li, Jinglei</creator><creator>Karpinsky, Dmitry V.</creator><creator>Wang, Jing</creator><creator>Wang, Yaojin</creator><general>American Institute of Physics</general><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope><orcidid>https://orcid.org/0000-0003-2561-1855</orcidid><orcidid>https://orcid.org/0000-0001-5447-6301</orcidid><orcidid>https://orcid.org/0000-0001-5858-5046</orcidid><orcidid>https://orcid.org/0000-0001-9471-5493</orcidid><orcidid>https://orcid.org/0000-0002-7752-1758</orcidid></search><sort><creationdate>20240617</creationdate><title>Enhanced comprehensive energy storage properties in Bi0.5Na0.5TiO3-based relaxor ferroelectric ceramics under a moderate electric field</title><author>Jiang, Shunshun ; Zhang, Ji ; Luo, Huajie ; Liu, Lisha ; Li, Jinglei ; Karpinsky, Dmitry V. ; Wang, Jing ; Wang, Yaojin</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-p148t-969859941fec96f4061645e0bfe88af81dbf2b8214280525878eaa8851143be43</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>Bismuth titanate</topic><topic>Ceramics</topic><topic>Electric fields</topic><topic>Energy storage</topic><topic>Ferroelectric materials</topic><topic>Ferroelectricity</topic><topic>Frequency stability</topic><topic>Hysteresis loops</topic><topic>Perovskites</topic><topic>Relaxors</topic><topic>Sodium titanate</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Jiang, Shunshun</creatorcontrib><creatorcontrib>Zhang, Ji</creatorcontrib><creatorcontrib>Luo, Huajie</creatorcontrib><creatorcontrib>Liu, Lisha</creatorcontrib><creatorcontrib>Li, Jinglei</creatorcontrib><creatorcontrib>Karpinsky, Dmitry V.</creatorcontrib><creatorcontrib>Wang, Jing</creatorcontrib><creatorcontrib>Wang, Yaojin</creatorcontrib><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Applied physics letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Jiang, Shunshun</au><au>Zhang, Ji</au><au>Luo, Huajie</au><au>Liu, Lisha</au><au>Li, Jinglei</au><au>Karpinsky, Dmitry V.</au><au>Wang, Jing</au><au>Wang, Yaojin</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Enhanced comprehensive energy storage properties in Bi0.5Na0.5TiO3-based relaxor ferroelectric ceramics under a moderate electric field</atitle><jtitle>Applied physics letters</jtitle><date>2024-06-17</date><risdate>2024</risdate><volume>124</volume><issue>25</issue><issn>0003-6951</issn><eissn>1077-3118</eissn><coden>APPLAB</coden><abstract>Bismuth sodium titanate (Bi0.5Na0.5TiO3)-based relaxor ferroelectric ceramics have received ever-increasing interest for their potential application in dielectric capacitors owing to their sterling energy storage capability. Herein, the perovskite end-member Ba(Fe0.5Nb0.5)O3 (BFN) was incorporated into 0.7Bi0.5Na0.5TiO3-0.3SrTiO3 (0.7BNT-0.3ST) ceramics to improve the relaxor characteristics and refine the grain, leading to slim polarization–electric field (P–E) hysteresis loops and enhanced electric breakdown strength. Particularly, the 0.85(0.7BNT-0.3ST)-0.15BFN ceramics achieved a high recoverable energy density of 5.7 J/cm3 and a high energy storage efficiency of 86.4% under a moderate electric field of 390 kV/cm. Additionally, remarkable stability in frequency, cycling, and temperature and excellent charge/discharge behavior were achieved at the same time. The above findings reveal that BFN-modified BNT-ST ceramics display greatly improved comprehensive energy storage properties, making them promising candidates in the field of electrostatic energy storage.</abstract><cop>Melville</cop><pub>American Institute of Physics</pub><doi>10.1063/5.0217327</doi><tpages>6</tpages><orcidid>https://orcid.org/0000-0003-2561-1855</orcidid><orcidid>https://orcid.org/0000-0001-5447-6301</orcidid><orcidid>https://orcid.org/0000-0001-5858-5046</orcidid><orcidid>https://orcid.org/0000-0001-9471-5493</orcidid><orcidid>https://orcid.org/0000-0002-7752-1758</orcidid></addata></record> |
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| source | AIP Journals Complete |
| subjects | Bismuth titanate Ceramics Electric fields Energy storage Ferroelectric materials Ferroelectricity Frequency stability Hysteresis loops Perovskites Relaxors Sodium titanate |
| title | Enhanced comprehensive energy storage properties in Bi0.5Na0.5TiO3-based relaxor ferroelectric ceramics under a moderate electric field |
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