Structural and optical properties of epitaxial ScxAl1−xN coherently grown on GaN bulk substrates by sputtering method
Three scandium aluminum nitride (ScAlN) thin films with different Sc compositions of 6%, 10%, and 14% were heteroepitaxially grown on n-type GaN bulk substrates by a low-temperature sputtering method. Atomically flat and smooth surfaces were observed by atomic force microscopy. The ScAlN films were...
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Veröffentlicht in: | Applied physics letters 2024-07, Vol.125 (2) |
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creator | Maeda, Takuya Wakamoto, Yusuke Kaneki, Shota Fujikura, Hajime Kobayashi, Atsushi |
description | Three scandium aluminum nitride (ScAlN) thin films with different Sc compositions of 6%, 10%, and 14% were heteroepitaxially grown on n-type GaN bulk substrates by a low-temperature sputtering method. Atomically flat and smooth surfaces were observed by atomic force microscopy. The ScAlN films were coherently grown on GaN, and the c-axis lattice constants increased with increase in the Sc composition, confirmed by x-ray diffraction. The refractive index and the extinction coefficient of ScAlN were extracted by variable angle spectroscopic ellipsometry. The refractive index slightly increased and the extinction coefficient showed red shift with increase in the Sc composition. The optical bandgap of the ScAlN films was also extracted, which slightly shrunk with increase in the Sc composition. |
doi_str_mv | 10.1063/5.0213662 |
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Atomically flat and smooth surfaces were observed by atomic force microscopy. The ScAlN films were coherently grown on GaN, and the c-axis lattice constants increased with increase in the Sc composition, confirmed by x-ray diffraction. The refractive index and the extinction coefficient of ScAlN were extracted by variable angle spectroscopic ellipsometry. The refractive index slightly increased and the extinction coefficient showed red shift with increase in the Sc composition. The optical bandgap of the ScAlN films was also extracted, which slightly shrunk with increase in the Sc composition.</description><identifier>ISSN: 0003-6951</identifier><identifier>EISSN: 1077-3118</identifier><identifier>DOI: 10.1063/5.0213662</identifier><identifier>CODEN: APPLAB</identifier><language>eng</language><publisher>Melville: American Institute of Physics</publisher><subject>Composition ; Doppler effect ; Epitaxial growth ; Gallium nitrides ; Lattice parameters ; Low temperature ; Optical properties ; Red shift ; Refractivity ; Scandium ; Spectroellipsometry ; Sputtering ; Substrates ; Thin films</subject><ispartof>Applied physics letters, 2024-07, Vol.125 (2)</ispartof><rights>Author(s)</rights><rights>2024 Author(s). 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The optical bandgap of the ScAlN films was also extracted, which slightly shrunk with increase in the Sc composition.</description><subject>Composition</subject><subject>Doppler effect</subject><subject>Epitaxial growth</subject><subject>Gallium nitrides</subject><subject>Lattice parameters</subject><subject>Low temperature</subject><subject>Optical properties</subject><subject>Red shift</subject><subject>Refractivity</subject><subject>Scandium</subject><subject>Spectroellipsometry</subject><subject>Sputtering</subject><subject>Substrates</subject><subject>Thin films</subject><issn>0003-6951</issn><issn>1077-3118</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNotUMtOAjEUbYwmIrrwD5q4MxnsY_pgSYiiCcEFum7aoQODQzu2nQB_4NpP9Euswc2999ycnJNzALjFaIQRpw9shAimnJMzMMBIiIJiLM_BACFECz5m-BJcxbjNkBFKB2C_TKGvUh90C7VbQd-lpsp3F3xnQ2pshL6GtmuSPjT5v6wOkxb_fH0fFrDyGxusS-0RroPfO-gdnOkFNH37AWNvYgo6ZQFzhLHrU7KhcWu4s2njV9fgotZttDf_ewjenx7fps_F_HX2Mp3Miw6XMhVlbbkxGrOKSMtMyTmVWvOaCKHHWmJEjbaMjEucoSCCG1ZyS0pkpNTCGDoEdyfdHOiztzGpre-Dy5aK5npKJvPMrPsTK1Y5aGq8U11odjocFUbqr1jF1H-x9BeAIWz8</recordid><startdate>20240708</startdate><enddate>20240708</enddate><creator>Maeda, Takuya</creator><creator>Wakamoto, Yusuke</creator><creator>Kaneki, Shota</creator><creator>Fujikura, Hajime</creator><creator>Kobayashi, Atsushi</creator><general>American Institute of Physics</general><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope><orcidid>https://orcid.org/0000-0002-2736-5611</orcidid><orcidid>https://orcid.org/0000-0003-0806-8571</orcidid><orcidid>https://orcid.org/0009-0007-7340-0899</orcidid><orcidid>https://orcid.org/0000-0001-5795-6490</orcidid><orcidid>https://orcid.org/0000-0002-7281-6151</orcidid></search><sort><creationdate>20240708</creationdate><title>Structural and optical properties of epitaxial ScxAl1−xN coherently grown on GaN bulk substrates by sputtering method</title><author>Maeda, Takuya ; Wakamoto, Yusuke ; Kaneki, Shota ; Fujikura, Hajime ; Kobayashi, Atsushi</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-p148t-4fe6bba15c28e5b46638aa6f277a9a8103bae52941a9a7276b546e240b88a7bb3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>Composition</topic><topic>Doppler effect</topic><topic>Epitaxial growth</topic><topic>Gallium nitrides</topic><topic>Lattice parameters</topic><topic>Low temperature</topic><topic>Optical properties</topic><topic>Red shift</topic><topic>Refractivity</topic><topic>Scandium</topic><topic>Spectroellipsometry</topic><topic>Sputtering</topic><topic>Substrates</topic><topic>Thin films</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Maeda, Takuya</creatorcontrib><creatorcontrib>Wakamoto, Yusuke</creatorcontrib><creatorcontrib>Kaneki, Shota</creatorcontrib><creatorcontrib>Fujikura, Hajime</creatorcontrib><creatorcontrib>Kobayashi, Atsushi</creatorcontrib><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Applied physics letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Maeda, Takuya</au><au>Wakamoto, Yusuke</au><au>Kaneki, Shota</au><au>Fujikura, Hajime</au><au>Kobayashi, Atsushi</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Structural and optical properties of epitaxial ScxAl1−xN coherently grown on GaN bulk substrates by sputtering method</atitle><jtitle>Applied physics letters</jtitle><date>2024-07-08</date><risdate>2024</risdate><volume>125</volume><issue>2</issue><issn>0003-6951</issn><eissn>1077-3118</eissn><coden>APPLAB</coden><abstract>Three scandium aluminum nitride (ScAlN) thin films with different Sc compositions of 6%, 10%, and 14% were heteroepitaxially grown on n-type GaN bulk substrates by a low-temperature sputtering method. Atomically flat and smooth surfaces were observed by atomic force microscopy. The ScAlN films were coherently grown on GaN, and the c-axis lattice constants increased with increase in the Sc composition, confirmed by x-ray diffraction. The refractive index and the extinction coefficient of ScAlN were extracted by variable angle spectroscopic ellipsometry. The refractive index slightly increased and the extinction coefficient showed red shift with increase in the Sc composition. 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subjects | Composition Doppler effect Epitaxial growth Gallium nitrides Lattice parameters Low temperature Optical properties Red shift Refractivity Scandium Spectroellipsometry Sputtering Substrates Thin films |
title | Structural and optical properties of epitaxial ScxAl1−xN coherently grown on GaN bulk substrates by sputtering method |
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