Continuous-wave cavity ring-down polarimetry

We present a new cavity-based polarimetric scheme for highly sensitive and time-resolved measurements of birefringence and dichroism, linear and circular, that employs rapidly pulsed single-frequency continuous wave (CW) laser sources and extends current cavity-based spectropolarimetric techniques....

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Veröffentlicht in:The Journal of chemical physics 2020-04, Vol.152 (16), p.164202-164202
Hauptverfasser: Visschers, Jim C., Tretiak, Oleg, Budker, Dmitry, Bougas, Lykourgos
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container_end_page 164202
container_issue 16
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container_title The Journal of chemical physics
container_volume 152
creator Visschers, Jim C.
Tretiak, Oleg
Budker, Dmitry
Bougas, Lykourgos
description We present a new cavity-based polarimetric scheme for highly sensitive and time-resolved measurements of birefringence and dichroism, linear and circular, that employs rapidly pulsed single-frequency continuous wave (CW) laser sources and extends current cavity-based spectropolarimetric techniques. We demonstrate how the use of a CW laser source allows for gains in spectral resolution, signal intensity, and data acquisition rate compared to traditional pulsed-based cavity ring-down polarimetry (CRDP). We discuss a particular CW-CRDP modality that is different from intensity-based cavity-enhanced polarimetric schemes as it relies on the determination of the polarization rotation frequency during a ring-down event generated by large intracavity polarization anisotropies. We present the principles of CW-CRDP and validate the applicability of this technique for the measurement of the non-resonant Faraday effect in solid SiO2 and CeF3 and gaseous butane. We give a general analysis of the fundamental sensitivity limits for CRDP techniques and show how the presented frequency-based methodology alleviates the requirement for high finesse cavities to achieve high polarimetric sensitivities and, thus, allows for the extension of cavity-based polarimetric schemes into different spectral regimes, but most importantly renders the CW-CRDP methodology particularly suitable for robust portable polarimetric instrumentations.
doi_str_mv 10.1063/5.0004476
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source AIP Journals Complete; Alma/SFX Local Collection
subjects Birefringence
Continuous radiation
Dichroism
Faraday effect
Holes
Physics
Polarimetry
Polarization
Silicon dioxide
Spectral resolution
title Continuous-wave cavity ring-down polarimetry
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