Probing gaseous molecular structure by molecular-frame photoelectron angular distributions
Carbon 1s photoelectron angular distributions of an iodomethane molecule were measured relative to the recoil-frame determined by the momentum correlation between I+ and CH3+ at photoelectron energies of 3, 6.1, and 12 eV. The energy dependent behavior of the recoil-frame photoelectron angular distr...
Gespeichert in:
| Veröffentlicht in: | The Journal of chemical physics 2019-09, Vol.151 (10) |
|---|---|
| Hauptverfasser: | , , , , , , , , , , , , , |
| Format: | Artikel |
| Sprache: | eng |
| Schlagworte: | |
| Online-Zugang: | Volltext |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | |
|---|---|
| container_issue | 10 |
| container_start_page | |
| container_title | The Journal of chemical physics |
| container_volume | 151 |
| creator | Fukuzawa, Hironobu Yamada, Syuhei Sakakibara, Yuta Tachibana, Tetsuya Ito, Yuta Takanashi, Tsukasa Nishiyama, Toshiyuki Sakai, Tsukasa Nagaya, Kiyonobu Saito, Norio Oura, Masaki Stener, Mauro Decleva, Piero Ueda, Kiyoshi |
| description | Carbon 1s photoelectron angular distributions of an iodomethane molecule were measured relative to the recoil-frame determined by the momentum correlation between I+ and CH3+ at photoelectron energies of 3, 6.1, and 12 eV. The energy dependent behavior of the recoil-frame photoelectron angular distributions is reproduced reasonably well by the time-dependent density functional theory with B-spline methods. We discuss potential applications of the fully differential photoelectron angular distribution measurements in the molecular frame to three-dimensional molecular structural determinations identifying the directions and lengths of the bonds. |
| doi_str_mv | 10.1063/1.5115801 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_scita</sourceid><recordid>TN_cdi_scitation_primary_10_1063_1_5115801</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2287144007</sourcerecordid><originalsourceid>FETCH-LOGICAL-c393t-6723ae5ef534b6b21a357c051d273ec781e23964a9ee1d6af35f39c3ccb721733</originalsourceid><addsrcrecordid>eNqdkEtLAzEUhYMoWB8L_8GAK4Wp9yaTZGYpxRcUdKEbNyGTSeqUdjImGaH_3qktdO_qwOE793IOIVcIUwTB7nDKEXkJeEQmCGWVS1HBMZkAUMwrAeKUnMW4BACUtJiQz7fg67ZbZAsdrR9itvYra4aVDllMYTBpCDarNwc7d0GvbdZ_-eTt6KXgu0x3i79I046hth5S67t4QU6cXkV7uddz8vH48D57zuevTy-z-3luWMVSLiRl2nLrOCtqUVPUjEsDHBsqmTWyREtZJQpdWYuN0I5xxyrDjKklRcnYObne3e2D_x5sTGrph9CNLxWlpcSiAJAjdbOjTPAxButUH9q1DhuFoLbTKVT76Ub2dsdG0ya9LfM_-MeHA6j6xrFfwAx9-A</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2287144007</pqid></control><display><type>article</type><title>Probing gaseous molecular structure by molecular-frame photoelectron angular distributions</title><source>AIP Journals Complete</source><source>Alma/SFX Local Collection</source><creator>Fukuzawa, Hironobu ; Yamada, Syuhei ; Sakakibara, Yuta ; Tachibana, Tetsuya ; Ito, Yuta ; Takanashi, Tsukasa ; Nishiyama, Toshiyuki ; Sakai, Tsukasa ; Nagaya, Kiyonobu ; Saito, Norio ; Oura, Masaki ; Stener, Mauro ; Decleva, Piero ; Ueda, Kiyoshi</creator><creatorcontrib>Fukuzawa, Hironobu ; Yamada, Syuhei ; Sakakibara, Yuta ; Tachibana, Tetsuya ; Ito, Yuta ; Takanashi, Tsukasa ; Nishiyama, Toshiyuki ; Sakai, Tsukasa ; Nagaya, Kiyonobu ; Saito, Norio ; Oura, Masaki ; Stener, Mauro ; Decleva, Piero ; Ueda, Kiyoshi</creatorcontrib><description>Carbon 1s photoelectron angular distributions of an iodomethane molecule were measured relative to the recoil-frame determined by the momentum correlation between I+ and CH3+ at photoelectron energies of 3, 6.1, and 12 eV. The energy dependent behavior of the recoil-frame photoelectron angular distributions is reproduced reasonably well by the time-dependent density functional theory with B-spline methods. We discuss potential applications of the fully differential photoelectron angular distribution measurements in the molecular frame to three-dimensional molecular structural determinations identifying the directions and lengths of the bonds.</description><identifier>ISSN: 0021-9606</identifier><identifier>EISSN: 1089-7690</identifier><identifier>DOI: 10.1063/1.5115801</identifier><identifier>CODEN: JCPSA6</identifier><language>eng</language><publisher>Melville: American Institute of Physics</publisher><subject>Angular distribution ; Density functional theory ; Molecular structure ; Photoelectrons ; Recoil ; Time dependence</subject><ispartof>The Journal of chemical physics, 2019-09, Vol.151 (10)</ispartof><rights>Author(s)</rights><rights>2019 Author(s). Published under license by AIP Publishing.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c393t-6723ae5ef534b6b21a357c051d273ec781e23964a9ee1d6af35f39c3ccb721733</citedby><cites>FETCH-LOGICAL-c393t-6723ae5ef534b6b21a357c051d273ec781e23964a9ee1d6af35f39c3ccb721733</cites><orcidid>0000-0003-0608-0323 ; 0000-0002-8283-381X ; 0000-0003-3700-7903 ; 0000-0002-7322-887X ; 0000-0001-5115-5676 ; 0000-0001-9867-0800</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://pubs.aip.org/jcp/article-lookup/doi/10.1063/1.5115801$$EHTML$$P50$$Gscitation$$H</linktohtml><link.rule.ids>315,781,785,795,4513,27929,27930,76389</link.rule.ids></links><search><creatorcontrib>Fukuzawa, Hironobu</creatorcontrib><creatorcontrib>Yamada, Syuhei</creatorcontrib><creatorcontrib>Sakakibara, Yuta</creatorcontrib><creatorcontrib>Tachibana, Tetsuya</creatorcontrib><creatorcontrib>Ito, Yuta</creatorcontrib><creatorcontrib>Takanashi, Tsukasa</creatorcontrib><creatorcontrib>Nishiyama, Toshiyuki</creatorcontrib><creatorcontrib>Sakai, Tsukasa</creatorcontrib><creatorcontrib>Nagaya, Kiyonobu</creatorcontrib><creatorcontrib>Saito, Norio</creatorcontrib><creatorcontrib>Oura, Masaki</creatorcontrib><creatorcontrib>Stener, Mauro</creatorcontrib><creatorcontrib>Decleva, Piero</creatorcontrib><creatorcontrib>Ueda, Kiyoshi</creatorcontrib><title>Probing gaseous molecular structure by molecular-frame photoelectron angular distributions</title><title>The Journal of chemical physics</title><description>Carbon 1s photoelectron angular distributions of an iodomethane molecule were measured relative to the recoil-frame determined by the momentum correlation between I+ and CH3+ at photoelectron energies of 3, 6.1, and 12 eV. The energy dependent behavior of the recoil-frame photoelectron angular distributions is reproduced reasonably well by the time-dependent density functional theory with B-spline methods. We discuss potential applications of the fully differential photoelectron angular distribution measurements in the molecular frame to three-dimensional molecular structural determinations identifying the directions and lengths of the bonds.</description><subject>Angular distribution</subject><subject>Density functional theory</subject><subject>Molecular structure</subject><subject>Photoelectrons</subject><subject>Recoil</subject><subject>Time dependence</subject><issn>0021-9606</issn><issn>1089-7690</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNqdkEtLAzEUhYMoWB8L_8GAK4Wp9yaTZGYpxRcUdKEbNyGTSeqUdjImGaH_3qktdO_qwOE793IOIVcIUwTB7nDKEXkJeEQmCGWVS1HBMZkAUMwrAeKUnMW4BACUtJiQz7fg67ZbZAsdrR9itvYra4aVDllMYTBpCDarNwc7d0GvbdZ_-eTt6KXgu0x3i79I046hth5S67t4QU6cXkV7uddz8vH48D57zuevTy-z-3luWMVSLiRl2nLrOCtqUVPUjEsDHBsqmTWyREtZJQpdWYuN0I5xxyrDjKklRcnYObne3e2D_x5sTGrph9CNLxWlpcSiAJAjdbOjTPAxButUH9q1DhuFoLbTKVT76Ub2dsdG0ya9LfM_-MeHA6j6xrFfwAx9-A</recordid><startdate>20190914</startdate><enddate>20190914</enddate><creator>Fukuzawa, Hironobu</creator><creator>Yamada, Syuhei</creator><creator>Sakakibara, Yuta</creator><creator>Tachibana, Tetsuya</creator><creator>Ito, Yuta</creator><creator>Takanashi, Tsukasa</creator><creator>Nishiyama, Toshiyuki</creator><creator>Sakai, Tsukasa</creator><creator>Nagaya, Kiyonobu</creator><creator>Saito, Norio</creator><creator>Oura, Masaki</creator><creator>Stener, Mauro</creator><creator>Decleva, Piero</creator><creator>Ueda, Kiyoshi</creator><general>American Institute of Physics</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope><orcidid>https://orcid.org/0000-0003-0608-0323</orcidid><orcidid>https://orcid.org/0000-0002-8283-381X</orcidid><orcidid>https://orcid.org/0000-0003-3700-7903</orcidid><orcidid>https://orcid.org/0000-0002-7322-887X</orcidid><orcidid>https://orcid.org/0000-0001-5115-5676</orcidid><orcidid>https://orcid.org/0000-0001-9867-0800</orcidid></search><sort><creationdate>20190914</creationdate><title>Probing gaseous molecular structure by molecular-frame photoelectron angular distributions</title><author>Fukuzawa, Hironobu ; Yamada, Syuhei ; Sakakibara, Yuta ; Tachibana, Tetsuya ; Ito, Yuta ; Takanashi, Tsukasa ; Nishiyama, Toshiyuki ; Sakai, Tsukasa ; Nagaya, Kiyonobu ; Saito, Norio ; Oura, Masaki ; Stener, Mauro ; Decleva, Piero ; Ueda, Kiyoshi</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c393t-6723ae5ef534b6b21a357c051d273ec781e23964a9ee1d6af35f39c3ccb721733</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Angular distribution</topic><topic>Density functional theory</topic><topic>Molecular structure</topic><topic>Photoelectrons</topic><topic>Recoil</topic><topic>Time dependence</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Fukuzawa, Hironobu</creatorcontrib><creatorcontrib>Yamada, Syuhei</creatorcontrib><creatorcontrib>Sakakibara, Yuta</creatorcontrib><creatorcontrib>Tachibana, Tetsuya</creatorcontrib><creatorcontrib>Ito, Yuta</creatorcontrib><creatorcontrib>Takanashi, Tsukasa</creatorcontrib><creatorcontrib>Nishiyama, Toshiyuki</creatorcontrib><creatorcontrib>Sakai, Tsukasa</creatorcontrib><creatorcontrib>Nagaya, Kiyonobu</creatorcontrib><creatorcontrib>Saito, Norio</creatorcontrib><creatorcontrib>Oura, Masaki</creatorcontrib><creatorcontrib>Stener, Mauro</creatorcontrib><creatorcontrib>Decleva, Piero</creatorcontrib><creatorcontrib>Ueda, Kiyoshi</creatorcontrib><collection>CrossRef</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>The Journal of chemical physics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Fukuzawa, Hironobu</au><au>Yamada, Syuhei</au><au>Sakakibara, Yuta</au><au>Tachibana, Tetsuya</au><au>Ito, Yuta</au><au>Takanashi, Tsukasa</au><au>Nishiyama, Toshiyuki</au><au>Sakai, Tsukasa</au><au>Nagaya, Kiyonobu</au><au>Saito, Norio</au><au>Oura, Masaki</au><au>Stener, Mauro</au><au>Decleva, Piero</au><au>Ueda, Kiyoshi</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Probing gaseous molecular structure by molecular-frame photoelectron angular distributions</atitle><jtitle>The Journal of chemical physics</jtitle><date>2019-09-14</date><risdate>2019</risdate><volume>151</volume><issue>10</issue><issn>0021-9606</issn><eissn>1089-7690</eissn><coden>JCPSA6</coden><abstract>Carbon 1s photoelectron angular distributions of an iodomethane molecule were measured relative to the recoil-frame determined by the momentum correlation between I+ and CH3+ at photoelectron energies of 3, 6.1, and 12 eV. The energy dependent behavior of the recoil-frame photoelectron angular distributions is reproduced reasonably well by the time-dependent density functional theory with B-spline methods. We discuss potential applications of the fully differential photoelectron angular distribution measurements in the molecular frame to three-dimensional molecular structural determinations identifying the directions and lengths of the bonds.</abstract><cop>Melville</cop><pub>American Institute of Physics</pub><doi>10.1063/1.5115801</doi><tpages>6</tpages><orcidid>https://orcid.org/0000-0003-0608-0323</orcidid><orcidid>https://orcid.org/0000-0002-8283-381X</orcidid><orcidid>https://orcid.org/0000-0003-3700-7903</orcidid><orcidid>https://orcid.org/0000-0002-7322-887X</orcidid><orcidid>https://orcid.org/0000-0001-5115-5676</orcidid><orcidid>https://orcid.org/0000-0001-9867-0800</orcidid></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0021-9606 |
| ispartof | The Journal of chemical physics, 2019-09, Vol.151 (10) |
| issn | 0021-9606 1089-7690 |
| language | eng |
| recordid | cdi_scitation_primary_10_1063_1_5115801 |
| source | AIP Journals Complete; Alma/SFX Local Collection |
| subjects | Angular distribution Density functional theory Molecular structure Photoelectrons Recoil Time dependence |
| title | Probing gaseous molecular structure by molecular-frame photoelectron angular distributions |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2024-12-15T11%3A32%3A14IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_scita&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Probing%20gaseous%20molecular%20structure%20by%20molecular-frame%20photoelectron%20angular%20distributions&rft.jtitle=The%20Journal%20of%20chemical%20physics&rft.au=Fukuzawa,%20Hironobu&rft.date=2019-09-14&rft.volume=151&rft.issue=10&rft.issn=0021-9606&rft.eissn=1089-7690&rft.coden=JCPSA6&rft_id=info:doi/10.1063/1.5115801&rft_dat=%3Cproquest_scita%3E2287144007%3C/proquest_scita%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2287144007&rft_id=info:pmid/&rfr_iscdi=true |