Evaluation of reversible and irreversible domain wall motions in relaxor ferroelectrics: Influence of acceptor ions

The intrinsic, reversible, and irreversible extrinsic dielectric responses of 0.27Pb(In1/2Nb1/2)O3–0.46Pb(Mg1/3Nb2/3)O3–0.27PbTiO3 relaxor single crystals with and without Mn doping have been extracted by using Rayleigh analysis from 0.1 Hz to 1000 Hz, and the influence of acceptor ions has been qua...

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Veröffentlicht in:Applied physics letters 2019-06, Vol.114 (23)
Hauptverfasser: Yang, Liya, Fang, Hong, Zheng, Limei, Du, Juan, Wang, Lihai, Lu, Xiaoyan, Lü, Weiming, Zhang, Rui, Cao, Wenwu
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container_issue 23
container_start_page
container_title Applied physics letters
container_volume 114
creator Yang, Liya
Fang, Hong
Zheng, Limei
Du, Juan
Wang, Lihai
Lu, Xiaoyan
Lü, Weiming
Zhang, Rui
Cao, Wenwu
description The intrinsic, reversible, and irreversible extrinsic dielectric responses of 0.27Pb(In1/2Nb1/2)O3–0.46Pb(Mg1/3Nb2/3)O3–0.27PbTiO3 relaxor single crystals with and without Mn doping have been extracted by using Rayleigh analysis from 0.1 Hz to 1000 Hz, and the influence of acceptor ions has been quantitatively evaluated. The results show that the lattice deformation under an ac electric field is slightly inhibited by Mn2+/Mn3+, while both reversible and irreversible domain wall motions are greatly suppressed to below 20% of the non-Mn doped values. As a result, the mechanical quality factor, which is closely related to domain wall motions, is significantly enhanced. Meanwhile, the large piezoelectricity, which is dominated by intrinsic contribution, is maintained.
doi_str_mv 10.1063/1.5094935
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The results show that the lattice deformation under an ac electric field is slightly inhibited by Mn2+/Mn3+, while both reversible and irreversible domain wall motions are greatly suppressed to below 20% of the non-Mn doped values. As a result, the mechanical quality factor, which is closely related to domain wall motions, is significantly enhanced. 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subjects Applied physics
Crystals
Deformation
Domain walls
Electric fields
Ferroelectric materials
Ferroelectricity
Piezoelectricity
Q factors
Relaxors
Single crystals
title Evaluation of reversible and irreversible domain wall motions in relaxor ferroelectrics: Influence of acceptor ions
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