A setup for extreme-ultraviolet ultrafast angle-resolved photoelectron spectroscopy at 50-kHz repetition rate
Time- and angle-resolved photoelectron spectroscopy (trARPES) is a powerful method to track the ultrafast dynamics of quasiparticles and electronic bands in energy and momentum space. We present a setup for trARPES with 22.3 eV extreme-ultraviolet (XUV) femtosecond pulses at 50-kHz repetition rate,...
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| Veröffentlicht in: | Review of scientific instruments 2019-02, Vol.90 (2), p.023105-023105 |
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| creator | Buss, Jan Heye Wang, He Xu, Yiming Maklar, Julian Joucken, Frederic Zeng, Lingkun Stoll, Sebastian Jozwiak, Chris Pepper, John Chuang, Yi-De Denlinger, Jonathan D. Hussain, Zahid Lanzara, Alessandra Kaindl, Robert A. |
| description | Time- and angle-resolved photoelectron spectroscopy (trARPES) is a powerful method to track the ultrafast dynamics of quasiparticles and electronic bands in energy and momentum space. We present a setup for trARPES with 22.3 eV extreme-ultraviolet (XUV) femtosecond pulses at 50-kHz repetition rate, which enables fast data acquisition and access to dynamics across momentum space with high sensitivity. The design and operation of the XUV beamline, pump-probe setup, and ultra-high vacuum endstation are described in detail. By characterizing the effect of space-charge broadening, we determine an ultimate source-limited energy resolution of 60 meV, with typically 80–100 meV obtained at 1–2 × 1010 photons/s probe flux on the sample. The instrument capabilities are demonstrated via both equilibrium and time-resolved ARPES studies of transition-metal dichalcogenides. The 50-kHz repetition rate enables sensitive measurements of quasiparticles at low excitation fluences in semiconducting MoSe2, with an instrumental time resolution of 65 fs. Moreover, photo-induced phase transitions can be driven with the available pump fluence, as shown by charge density wave melting in 1T-TiSe2. The high repetition-rate setup thus provides a versatile platform for sensitive XUV trARPES, from quenching of electronic phases down to the perturbative limit. |
| doi_str_mv | 10.1063/1.5079677 |
| format | Article |
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We present a setup for trARPES with 22.3 eV extreme-ultraviolet (XUV) femtosecond pulses at 50-kHz repetition rate, which enables fast data acquisition and access to dynamics across momentum space with high sensitivity. The design and operation of the XUV beamline, pump-probe setup, and ultra-high vacuum endstation are described in detail. By characterizing the effect of space-charge broadening, we determine an ultimate source-limited energy resolution of 60 meV, with typically 80–100 meV obtained at 1–2 × 1010 photons/s probe flux on the sample. The instrument capabilities are demonstrated via both equilibrium and time-resolved ARPES studies of transition-metal dichalcogenides. The 50-kHz repetition rate enables sensitive measurements of quasiparticles at low excitation fluences in semiconducting MoSe2, with an instrumental time resolution of 65 fs. Moreover, photo-induced phase transitions can be driven with the available pump fluence, as shown by charge density wave melting in 1T-TiSe2. The high repetition-rate setup thus provides a versatile platform for sensitive XUV trARPES, from quenching of electronic phases down to the perturbative limit.</description><identifier>ISSN: 0034-6748</identifier><identifier>EISSN: 1089-7623</identifier><identifier>DOI: 10.1063/1.5079677</identifier><identifier>PMID: 30831755</identifier><identifier>CODEN: RSINAK</identifier><language>eng</language><publisher>United States: American Institute of Physics</publisher><subject>Charge density waves ; Energy resolution ; Femtosecond pulses ; Fluence ; High vacuum ; Momentum ; OTHER INSTRUMENTATION ; Phase transitions ; Photoelectron spectroscopy ; Photoelectrons ; Photons ; Repetition ; Scientific apparatus & instruments ; Spectrum analysis ; Transition metal compounds</subject><ispartof>Review of scientific instruments, 2019-02, Vol.90 (2), p.023105-023105</ispartof><rights>Author(s)</rights><rights>2019 Author(s). 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We present a setup for trARPES with 22.3 eV extreme-ultraviolet (XUV) femtosecond pulses at 50-kHz repetition rate, which enables fast data acquisition and access to dynamics across momentum space with high sensitivity. The design and operation of the XUV beamline, pump-probe setup, and ultra-high vacuum endstation are described in detail. By characterizing the effect of space-charge broadening, we determine an ultimate source-limited energy resolution of 60 meV, with typically 80–100 meV obtained at 1–2 × 1010 photons/s probe flux on the sample. The instrument capabilities are demonstrated via both equilibrium and time-resolved ARPES studies of transition-metal dichalcogenides. The 50-kHz repetition rate enables sensitive measurements of quasiparticles at low excitation fluences in semiconducting MoSe2, with an instrumental time resolution of 65 fs. Moreover, photo-induced phase transitions can be driven with the available pump fluence, as shown by charge density wave melting in 1T-TiSe2. The high repetition-rate setup thus provides a versatile platform for sensitive XUV trARPES, from quenching of electronic phases down to the perturbative limit.</abstract><cop>United States</cop><pub>American Institute of Physics</pub><pmid>30831755</pmid><doi>10.1063/1.5079677</doi><tpages>11</tpages><orcidid>https://orcid.org/0000-0002-1218-042X</orcidid><orcidid>https://orcid.org/0000-0002-9056-0081</orcidid><orcidid>https://orcid.org/0000-0001-7645-1631</orcidid><orcidid>https://orcid.org/0000-0003-4123-4455</orcidid><orcidid>https://orcid.org/0000-0002-2773-3840</orcidid><orcidid>https://orcid.org/0000-0002-6434-5134</orcidid><orcidid>https://orcid.org/0000-0002-0980-3753</orcidid><orcidid>https://orcid.org/0000-0003-3639-5625</orcidid><orcidid>https://orcid.org/000000021218042X</orcidid><orcidid>https://orcid.org/0000000290560081</orcidid><orcidid>https://orcid.org/0000000264345134</orcidid><orcidid>https://orcid.org/0000000176451631</orcidid><orcidid>https://orcid.org/0000000209803753</orcidid><orcidid>https://orcid.org/0000000336395625</orcidid><orcidid>https://orcid.org/0000000227733840</orcidid><orcidid>https://orcid.org/0000000341234455</orcidid><oa>free_for_read</oa></addata></record> |
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| ispartof | Review of scientific instruments, 2019-02, Vol.90 (2), p.023105-023105 |
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| language | eng |
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| source | AIP Journals Complete; Alma/SFX Local Collection |
| subjects | Charge density waves Energy resolution Femtosecond pulses Fluence High vacuum Momentum OTHER INSTRUMENTATION Phase transitions Photoelectron spectroscopy Photoelectrons Photons Repetition Scientific apparatus & instruments Spectrum analysis Transition metal compounds |
| title | A setup for extreme-ultraviolet ultrafast angle-resolved photoelectron spectroscopy at 50-kHz repetition rate |
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