Enhanced energy storage density by inducing defect dipoles in lead free relaxor ferroelectric BaTiO3-based ceramics
In this work, Mn-doped 0.9BaTiO3-0.1Bi(Mg2/3Nb1/3)O3 ceramics were prepared by the conventional solid state reaction method, and the effect of defect dipoles on energy storage properties of lead free relaxor ferroelectric BaTiO3-based ceramics was studied. The crystal structure, dielectric propertie...
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| Veröffentlicht in: | Applied physics letters 2017-03, Vol.110 (13) |
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| creator | Li, Wen-Bo Zhou, Di Pang, Li-Xia |
| description | In this work, Mn-doped 0.9BaTiO3-0.1Bi(Mg2/3Nb1/3)O3
ceramics were
prepared by the conventional solid state reaction method, and the effect of defect dipoles
on energy storage
properties of
lead free relaxor
ferroelectric BaTiO3-based ceramics was studied. The
crystal structure, dielectric properties, and energy storage properties were explored in detail. It was found that
polarization
hysteresis (P-E) loops of 0.9BaTiO3-0.1Bi(Mg2/3Nb1/3)O3-x wt. % MnCO3 (0.2–0.5)
ceramics took on
high maximum polarization (Pmax
) and low remanent
polarization
(Pr
). Meanwhile, recoverable energy density
(Wrec
) and energy conversion efficiency (η) were
obviously enhanced by inducing defect dipoles into
BaTiO3-Bi(Mg2/3Nb1/3)O3
relaxor
ferroelectrics. The
0.9BaTiO3-0.1Bi(Mg2/3Nb1/3)O3-0.3 wt. % MnCO3
ceramic was found
to exhibit good energy storage properties with a Wrec
of about
1.70 J/cm3 and a η ∼ 90% under an electric field of 210 kV/cm.
The breakdown electric
field and Wrec
of BaTiO3-based
materials were
significantly increased in the present work, and they might be good candidates for high
power energy
storage applications. |
| doi_str_mv | 10.1063/1.4979467 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_scita</sourceid><recordid>TN_cdi_scitation_primary_10_1063_1_4979467</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2124500553</sourcerecordid><originalsourceid>FETCH-LOGICAL-c327t-25989f4172f1207c27173ce41b0db6232acba97f66e43e3c589418acb6e457563</originalsourceid><addsrcrecordid>eNqdkEtLAzEUhYMoWB8L_0HAlcLUPCaTzlJLfUChm7oOmcxNTZkmYzIV598bacG9q8v5-LgHDkI3lEwpqfgDnZa1rMtKnqAJJVIWnNLZKZoQQnhR1YKeo4uUtjkKxvkEpYX_0N5Ai8FD3Iw4DSHqDeAWfHLDiJsRO9_ujfObzCyYAbeuDx2kzHEHusU2AuAInf4OEVuIMUCXvegMftJrt-JFo1NuMBD1zpl0hc6s7hJcH-8len9erOevxXL18jZ_XBaGMzkUTNSz2pZUMksZkYZJKrmBkjakbSrGmTaNrqWtKig5cCNmdUlnGeYspKj4Jbo9_O1j-NxDGtQ27KPPlYpRVoq8geDZujtYJoaUIljVR7fTcVSUqN9NFVXHTbN7f3CTcYMeXPD_k79C_BNV31r-A_WkhSg</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2124500553</pqid></control><display><type>article</type><title>Enhanced energy storage density by inducing defect dipoles in lead free relaxor ferroelectric BaTiO3-based ceramics</title><source>AIP Journals Complete</source><source>Alma/SFX Local Collection</source><creator>Li, Wen-Bo ; Zhou, Di ; Pang, Li-Xia</creator><creatorcontrib>Li, Wen-Bo ; Zhou, Di ; Pang, Li-Xia</creatorcontrib><description>In this work, Mn-doped 0.9BaTiO3-0.1Bi(Mg2/3Nb1/3)O3
ceramics were
prepared by the conventional solid state reaction method, and the effect of defect dipoles
on energy storage
properties of
lead free relaxor
ferroelectric BaTiO3-based ceramics was studied. The
crystal structure, dielectric properties, and energy storage properties were explored in detail. It was found that
polarization
hysteresis (P-E) loops of 0.9BaTiO3-0.1Bi(Mg2/3Nb1/3)O3-x wt. % MnCO3 (0.2–0.5)
ceramics took on
high maximum polarization (Pmax
) and low remanent
polarization
(Pr
). Meanwhile, recoverable energy density
(Wrec
) and energy conversion efficiency (η) were
obviously enhanced by inducing defect dipoles into
BaTiO3-Bi(Mg2/3Nb1/3)O3
relaxor
ferroelectrics. The
0.9BaTiO3-0.1Bi(Mg2/3Nb1/3)O3-0.3 wt. % MnCO3
ceramic was found
to exhibit good energy storage properties with a Wrec
of about
1.70 J/cm3 and a η ∼ 90% under an electric field of 210 kV/cm.
The breakdown electric
field and Wrec
of BaTiO3-based
materials were
significantly increased in the present work, and they might be good candidates for high
power energy
storage applications.</description><identifier>ISSN: 0003-6951</identifier><identifier>EISSN: 1077-3118</identifier><identifier>DOI: 10.1063/1.4979467</identifier><identifier>CODEN: APPLAB</identifier><language>eng</language><publisher>Melville: American Institute of Physics</publisher><subject>Applied physics ; Barium titanates ; Ceramics ; Defects ; Dielectric properties ; Dielectric relaxation ; Dipoles ; Energy ; Energy conversion efficiency ; Energy storage ; Ferroelectric materials ; Ferroelectricity ; Flux density</subject><ispartof>Applied physics letters, 2017-03, Vol.110 (13)</ispartof><rights>Author(s)</rights><rights>2017 Author(s). Published by AIP Publishing.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c327t-25989f4172f1207c27173ce41b0db6232acba97f66e43e3c589418acb6e457563</citedby><cites>FETCH-LOGICAL-c327t-25989f4172f1207c27173ce41b0db6232acba97f66e43e3c589418acb6e457563</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://pubs.aip.org/apl/article-lookup/doi/10.1063/1.4979467$$EHTML$$P50$$Gscitation$$H</linktohtml><link.rule.ids>314,776,780,790,4497,27903,27904,76130</link.rule.ids></links><search><creatorcontrib>Li, Wen-Bo</creatorcontrib><creatorcontrib>Zhou, Di</creatorcontrib><creatorcontrib>Pang, Li-Xia</creatorcontrib><title>Enhanced energy storage density by inducing defect dipoles in lead free relaxor ferroelectric BaTiO3-based ceramics</title><title>Applied physics letters</title><description>In this work, Mn-doped 0.9BaTiO3-0.1Bi(Mg2/3Nb1/3)O3
ceramics were
prepared by the conventional solid state reaction method, and the effect of defect dipoles
on energy storage
properties of
lead free relaxor
ferroelectric BaTiO3-based ceramics was studied. The
crystal structure, dielectric properties, and energy storage properties were explored in detail. It was found that
polarization
hysteresis (P-E) loops of 0.9BaTiO3-0.1Bi(Mg2/3Nb1/3)O3-x wt. % MnCO3 (0.2–0.5)
ceramics took on
high maximum polarization (Pmax
) and low remanent
polarization
(Pr
). Meanwhile, recoverable energy density
(Wrec
) and energy conversion efficiency (η) were
obviously enhanced by inducing defect dipoles into
BaTiO3-Bi(Mg2/3Nb1/3)O3
relaxor
ferroelectrics. The
0.9BaTiO3-0.1Bi(Mg2/3Nb1/3)O3-0.3 wt. % MnCO3
ceramic was found
to exhibit good energy storage properties with a Wrec
of about
1.70 J/cm3 and a η ∼ 90% under an electric field of 210 kV/cm.
The breakdown electric
field and Wrec
of BaTiO3-based
materials were
significantly increased in the present work, and they might be good candidates for high
power energy
storage applications.</description><subject>Applied physics</subject><subject>Barium titanates</subject><subject>Ceramics</subject><subject>Defects</subject><subject>Dielectric properties</subject><subject>Dielectric relaxation</subject><subject>Dipoles</subject><subject>Energy</subject><subject>Energy conversion efficiency</subject><subject>Energy storage</subject><subject>Ferroelectric materials</subject><subject>Ferroelectricity</subject><subject>Flux density</subject><issn>0003-6951</issn><issn>1077-3118</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2017</creationdate><recordtype>article</recordtype><recordid>eNqdkEtLAzEUhYMoWB8L_0HAlcLUPCaTzlJLfUChm7oOmcxNTZkmYzIV598bacG9q8v5-LgHDkI3lEwpqfgDnZa1rMtKnqAJJVIWnNLZKZoQQnhR1YKeo4uUtjkKxvkEpYX_0N5Ai8FD3Iw4DSHqDeAWfHLDiJsRO9_ujfObzCyYAbeuDx2kzHEHusU2AuAInf4OEVuIMUCXvegMftJrt-JFo1NuMBD1zpl0hc6s7hJcH-8len9erOevxXL18jZ_XBaGMzkUTNSz2pZUMksZkYZJKrmBkjakbSrGmTaNrqWtKig5cCNmdUlnGeYspKj4Jbo9_O1j-NxDGtQ27KPPlYpRVoq8geDZujtYJoaUIljVR7fTcVSUqN9NFVXHTbN7f3CTcYMeXPD_k79C_BNV31r-A_WkhSg</recordid><startdate>20170327</startdate><enddate>20170327</enddate><creator>Li, Wen-Bo</creator><creator>Zhou, Di</creator><creator>Pang, Li-Xia</creator><general>American Institute of Physics</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope></search><sort><creationdate>20170327</creationdate><title>Enhanced energy storage density by inducing defect dipoles in lead free relaxor ferroelectric BaTiO3-based ceramics</title><author>Li, Wen-Bo ; Zhou, Di ; Pang, Li-Xia</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c327t-25989f4172f1207c27173ce41b0db6232acba97f66e43e3c589418acb6e457563</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2017</creationdate><topic>Applied physics</topic><topic>Barium titanates</topic><topic>Ceramics</topic><topic>Defects</topic><topic>Dielectric properties</topic><topic>Dielectric relaxation</topic><topic>Dipoles</topic><topic>Energy</topic><topic>Energy conversion efficiency</topic><topic>Energy storage</topic><topic>Ferroelectric materials</topic><topic>Ferroelectricity</topic><topic>Flux density</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Li, Wen-Bo</creatorcontrib><creatorcontrib>Zhou, Di</creatorcontrib><creatorcontrib>Pang, Li-Xia</creatorcontrib><collection>CrossRef</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Applied physics letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Li, Wen-Bo</au><au>Zhou, Di</au><au>Pang, Li-Xia</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Enhanced energy storage density by inducing defect dipoles in lead free relaxor ferroelectric BaTiO3-based ceramics</atitle><jtitle>Applied physics letters</jtitle><date>2017-03-27</date><risdate>2017</risdate><volume>110</volume><issue>13</issue><issn>0003-6951</issn><eissn>1077-3118</eissn><coden>APPLAB</coden><abstract>In this work, Mn-doped 0.9BaTiO3-0.1Bi(Mg2/3Nb1/3)O3
ceramics were
prepared by the conventional solid state reaction method, and the effect of defect dipoles
on energy storage
properties of
lead free relaxor
ferroelectric BaTiO3-based ceramics was studied. The
crystal structure, dielectric properties, and energy storage properties were explored in detail. It was found that
polarization
hysteresis (P-E) loops of 0.9BaTiO3-0.1Bi(Mg2/3Nb1/3)O3-x wt. % MnCO3 (0.2–0.5)
ceramics took on
high maximum polarization (Pmax
) and low remanent
polarization
(Pr
). Meanwhile, recoverable energy density
(Wrec
) and energy conversion efficiency (η) were
obviously enhanced by inducing defect dipoles into
BaTiO3-Bi(Mg2/3Nb1/3)O3
relaxor
ferroelectrics. The
0.9BaTiO3-0.1Bi(Mg2/3Nb1/3)O3-0.3 wt. % MnCO3
ceramic was found
to exhibit good energy storage properties with a Wrec
of about
1.70 J/cm3 and a η ∼ 90% under an electric field of 210 kV/cm.
The breakdown electric
field and Wrec
of BaTiO3-based
materials were
significantly increased in the present work, and they might be good candidates for high
power energy
storage applications.</abstract><cop>Melville</cop><pub>American Institute of Physics</pub><doi>10.1063/1.4979467</doi><tpages>5</tpages></addata></record> |
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| source | AIP Journals Complete; Alma/SFX Local Collection |
| subjects | Applied physics Barium titanates Ceramics Defects Dielectric properties Dielectric relaxation Dipoles Energy Energy conversion efficiency Energy storage Ferroelectric materials Ferroelectricity Flux density |
| title | Enhanced energy storage density by inducing defect dipoles in lead free relaxor ferroelectric BaTiO3-based ceramics |
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