Observation of polarization and thickness dependent third-harmonic generation in multilayer black phosphorus
We experimentally investigate the power, polarization, and thickness dependence of third-harmonic generation in multilayer black phosphorus (BP) flakes. We observe that the third-harmonic response radiated from BP is highly dependent on the polarization of the excitation owing to the anisotropic nat...
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Veröffentlicht in: | Applied physics letters 2016-12, Vol.109 (26) |
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creator | Wu, Hsin-Yu Yen, Yun Liu, Cheng-Hsien |
description | We experimentally investigate the power, polarization, and thickness dependence of third-harmonic
generation in multilayer black phosphorus (BP) flakes. We observe that the third-harmonic response
radiated from BP
is highly dependent on the polarization of the excitation owing to the anisotropic nature of
BP, as well as
being very sensitive to the flake thickness owing to the interference effects between
surface and bulk nonlinear contributions. Compared to the linear optical microscopic
examination, the demonstrated third-harmonic generation can be used for nonlinear optical
identification of the crystal orientation and thickness of multilayer
BP with higher
contrast and fewer restrictions on substrate materials. |
doi_str_mv | 10.1063/1.4972869 |
format | Article |
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generation in multilayer black phosphorus (BP) flakes. We observe that the third-harmonic response
radiated from BP
is highly dependent on the polarization of the excitation owing to the anisotropic nature of
BP, as well as
being very sensitive to the flake thickness owing to the interference effects between
surface and bulk nonlinear contributions. Compared to the linear optical microscopic
examination, the demonstrated third-harmonic generation can be used for nonlinear optical
identification of the crystal orientation and thickness of multilayer
BP with higher
contrast and fewer restrictions on substrate materials.</description><identifier>ISSN: 0003-6951</identifier><identifier>EISSN: 1077-3118</identifier><identifier>DOI: 10.1063/1.4972869</identifier><identifier>CODEN: APPLAB</identifier><language>eng</language><ispartof>Applied physics letters, 2016-12, Vol.109 (26)</ispartof><rights>Author(s)</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c365t-63fde000dc08d9c3738f9858d196cf63eb8bd9405a45c7b9741a9279dd5fd00d3</citedby><cites>FETCH-LOGICAL-c365t-63fde000dc08d9c3738f9858d196cf63eb8bd9405a45c7b9741a9279dd5fd00d3</cites><orcidid>0000-0001-7899-6926</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://pubs.aip.org/apl/article-lookup/doi/10.1063/1.4972869$$EHTML$$P50$$Gscitation$$H</linktohtml><link.rule.ids>314,776,780,790,4498,27901,27902,76353</link.rule.ids></links><search><creatorcontrib>Wu, Hsin-Yu</creatorcontrib><creatorcontrib>Yen, Yun</creatorcontrib><creatorcontrib>Liu, Cheng-Hsien</creatorcontrib><title>Observation of polarization and thickness dependent third-harmonic generation in multilayer black phosphorus</title><title>Applied physics letters</title><description>We experimentally investigate the power, polarization, and thickness dependence of third-harmonic
generation in multilayer black phosphorus (BP) flakes. We observe that the third-harmonic response
radiated from BP
is highly dependent on the polarization of the excitation owing to the anisotropic nature of
BP, as well as
being very sensitive to the flake thickness owing to the interference effects between
surface and bulk nonlinear contributions. Compared to the linear optical microscopic
examination, the demonstrated third-harmonic generation can be used for nonlinear optical
identification of the crystal orientation and thickness of multilayer
BP with higher
contrast and fewer restrictions on substrate materials.</description><issn>0003-6951</issn><issn>1077-3118</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2016</creationdate><recordtype>article</recordtype><recordid>eNqdkEtLAzEUhYMoWKsL_0G2ClOTyeS1lOILCt3oesjk4cROkyGZFuqvd-oU3Lu4XM7lO5d7DwC3GC0wYuQBLyrJS8HkGZhhxHlBMBbnYIYQIgWTFF-Cq5y_RklLQmagWzfZpr0afAwwOtjHTiX_PWkVDBxarzfB5gyN7W0wNgzHWTJFq9I2Bq_hpw02TQ4f4HbXDb5TB5tg0ym9gX0b81hpl6_BhVNdtjenPgcfz0_vy9ditX55Wz6uCk0YHQpGnLHjhUYjYaQmnAgnBRUGS6YdI7YRjZEVoqqimjeSV1jJkktjqDOjjczB3bRXp5hzsq7uk9-qdKgxqo8x1bg-xTSy9xObtR9-n_gfvI_pD6x748gPtlB5eA</recordid><startdate>20161226</startdate><enddate>20161226</enddate><creator>Wu, Hsin-Yu</creator><creator>Yen, Yun</creator><creator>Liu, Cheng-Hsien</creator><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0001-7899-6926</orcidid></search><sort><creationdate>20161226</creationdate><title>Observation of polarization and thickness dependent third-harmonic generation in multilayer black phosphorus</title><author>Wu, Hsin-Yu ; Yen, Yun ; Liu, Cheng-Hsien</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c365t-63fde000dc08d9c3738f9858d196cf63eb8bd9405a45c7b9741a9279dd5fd00d3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2016</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Wu, Hsin-Yu</creatorcontrib><creatorcontrib>Yen, Yun</creatorcontrib><creatorcontrib>Liu, Cheng-Hsien</creatorcontrib><collection>CrossRef</collection><jtitle>Applied physics letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Wu, Hsin-Yu</au><au>Yen, Yun</au><au>Liu, Cheng-Hsien</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Observation of polarization and thickness dependent third-harmonic generation in multilayer black phosphorus</atitle><jtitle>Applied physics letters</jtitle><date>2016-12-26</date><risdate>2016</risdate><volume>109</volume><issue>26</issue><issn>0003-6951</issn><eissn>1077-3118</eissn><coden>APPLAB</coden><abstract>We experimentally investigate the power, polarization, and thickness dependence of third-harmonic
generation in multilayer black phosphorus (BP) flakes. We observe that the third-harmonic response
radiated from BP
is highly dependent on the polarization of the excitation owing to the anisotropic nature of
BP, as well as
being very sensitive to the flake thickness owing to the interference effects between
surface and bulk nonlinear contributions. Compared to the linear optical microscopic
examination, the demonstrated third-harmonic generation can be used for nonlinear optical
identification of the crystal orientation and thickness of multilayer
BP with higher
contrast and fewer restrictions on substrate materials.</abstract><doi>10.1063/1.4972869</doi><tpages>5</tpages><orcidid>https://orcid.org/0000-0001-7899-6926</orcidid></addata></record> |
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title | Observation of polarization and thickness dependent third-harmonic generation in multilayer black phosphorus |
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