Efficient Nd 3 + → Yb 3 + energy transfer in Nd 3 + , Yb 3 + : Gd 3 Ga 5 O 12 multicenter garnet crystal

For seeking better laser crystals with good optical properties and high efficiency, especially for application in a high power solid-state laser, Yb 3 + , Nd 3 + : Gd 3 Ga 5 O 12 crystal (abbreviated as Yb,Nd:GGG below) was grown by Czochralski method. A complete optical characterization was reporte...

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Veröffentlicht in:Journal of applied physics 2009-04, Vol.105 (8), p.083113-083113-6
Hauptverfasser: Jia, Zhitai, Arcangeli, Andrea, Tao, Xutang, Zhang, Jian, Dong, Chunming, Jiang, Minhua, Bonelli, Lucia, Tonelli, Mauro
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container_issue 8
container_start_page 083113
container_title Journal of applied physics
container_volume 105
creator Jia, Zhitai
Arcangeli, Andrea
Tao, Xutang
Zhang, Jian
Dong, Chunming
Jiang, Minhua
Bonelli, Lucia
Tonelli, Mauro
description For seeking better laser crystals with good optical properties and high efficiency, especially for application in a high power solid-state laser, Yb 3 + , Nd 3 + : Gd 3 Ga 5 O 12 crystal (abbreviated as Yb,Nd:GGG below) was grown by Czochralski method. A complete optical characterization was reported including absorption and emission spectra at different temperatures and fluorescence lifetimes. Very efficient Nd 3 + F 4 3 / 2 → Yb 3 + F 2 5 / 2 energy transfer was found whereas the back transfer was completely quenched at low temperature ( T < 200   K ) . From the data of Nd 3 + fluorescence lifetime and emission spectrum we achieved the energy-transfer efficiency as large as 94% at 77 K and 84% at 300 K, respectively. After fitting the decay curve we got the energy-transfer microparameter with a value of 2.1 × 10 − 39   cm 6 s − 1 at 300 K.
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A complete optical characterization was reported including absorption and emission spectra at different temperatures and fluorescence lifetimes. Very efficient Nd 3 + F 4 3 / 2 → Yb 3 + F 2 5 / 2 energy transfer was found whereas the back transfer was completely quenched at low temperature ( T &lt; 200   K ) . From the data of Nd 3 + fluorescence lifetime and emission spectrum we achieved the energy-transfer efficiency as large as 94% at 77 K and 84% at 300 K, respectively. 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title Efficient Nd 3 + → Yb 3 + energy transfer in Nd 3 + , Yb 3 + : Gd 3 Ga 5 O 12 multicenter garnet crystal
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