FeO nanostructure films as solar-thermal conversion materials for ammonia synthesis
Here, we report that black photothermal materials elevate solar heating temperatures across high solar absorption and low infrared radiation. Fe 3 O 4 nanostructure films can be heated to 350 °C under light irradiation, and this system shows effective visible-light-driven ammonia synthesis productio...
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| Veröffentlicht in: | Chemical communications (Cambridge, England) England), 2024-11, Vol.6 (89), p.1355-1358 |
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| container_end_page | 1358 |
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| container_issue | 89 |
| container_start_page | 1355 |
| container_title | Chemical communications (Cambridge, England) |
| container_volume | 6 |
| creator | Fu, Rong Lei, Di Li, Zhenlu Zhang, Hangjian Zhao, Xiaofei Tao, Shuo |
| description | Here, we report that black photothermal materials elevate solar heating temperatures across high solar absorption and low infrared radiation. Fe
3
O
4
nanostructure films can be heated to 350 °C under light irradiation, and this system shows effective visible-light-driven ammonia synthesis production of 3677 μg g
−1
h
−1
under gas-solid phase catalysis without noble metals.
Fe
3
O
4
film is composed of dispersed nanoparticles and irregular nanopores, where photons can be trapped by multi-reflection. The solar-thermal temperature can raise to above 350 °C and meet the temperature requirement for ammonia synthesis. |
| doi_str_mv | 10.1039/d4cc04112g |
| format | Article |
| fullrecord | <record><control><sourceid>rsc</sourceid><recordid>TN_cdi_rsc_primary_d4cc04112g</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>d4cc04112g</sourcerecordid><originalsourceid>FETCH-rsc_primary_d4cc04112g3</originalsourceid><addsrcrecordid>eNqFjjsLwjAUhYMo-FzchfsHqolNfcyiuDno4FYuMdVIk8i9reC_t4Lg6Fm-A98ZjhBjJadKpuvZRRsjtVLza0v0VLrQSaZX5_anZ-tkmeqsK_rMd9lEZaueOO7sAQKGyBXVpqrJQuFKz4AMHEukpLpZ8liCieFpiV0M4LGy5LBkKCIBeh-DQ-BXaLbseCg6RSPt6MuBmOy2p80-ITb5g5xHeuW_p-k__wZYgEL8</addsrcrecordid><sourcetype>Publisher</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype></control><display><type>article</type><title>FeO nanostructure films as solar-thermal conversion materials for ammonia synthesis</title><source>Royal Society Of Chemistry Journals 2008-</source><source>Alma/SFX Local Collection</source><creator>Fu, Rong ; Lei, Di ; Li, Zhenlu ; Zhang, Hangjian ; Zhao, Xiaofei ; Tao, Shuo</creator><creatorcontrib>Fu, Rong ; Lei, Di ; Li, Zhenlu ; Zhang, Hangjian ; Zhao, Xiaofei ; Tao, Shuo</creatorcontrib><description>Here, we report that black photothermal materials elevate solar heating temperatures across high solar absorption and low infrared radiation. Fe
3
O
4
nanostructure films can be heated to 350 °C under light irradiation, and this system shows effective visible-light-driven ammonia synthesis production of 3677 μg g
−1
h
−1
under gas-solid phase catalysis without noble metals.
Fe
3
O
4
film is composed of dispersed nanoparticles and irregular nanopores, where photons can be trapped by multi-reflection. The solar-thermal temperature can raise to above 350 °C and meet the temperature requirement for ammonia synthesis.</description><identifier>ISSN: 1359-7345</identifier><identifier>EISSN: 1364-548X</identifier><identifier>DOI: 10.1039/d4cc04112g</identifier><ispartof>Chemical communications (Cambridge, England), 2024-11, Vol.6 (89), p.1355-1358</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27924,27925</link.rule.ids></links><search><creatorcontrib>Fu, Rong</creatorcontrib><creatorcontrib>Lei, Di</creatorcontrib><creatorcontrib>Li, Zhenlu</creatorcontrib><creatorcontrib>Zhang, Hangjian</creatorcontrib><creatorcontrib>Zhao, Xiaofei</creatorcontrib><creatorcontrib>Tao, Shuo</creatorcontrib><title>FeO nanostructure films as solar-thermal conversion materials for ammonia synthesis</title><title>Chemical communications (Cambridge, England)</title><description>Here, we report that black photothermal materials elevate solar heating temperatures across high solar absorption and low infrared radiation. Fe
3
O
4
nanostructure films can be heated to 350 °C under light irradiation, and this system shows effective visible-light-driven ammonia synthesis production of 3677 μg g
−1
h
−1
under gas-solid phase catalysis without noble metals.
Fe
3
O
4
film is composed of dispersed nanoparticles and irregular nanopores, where photons can be trapped by multi-reflection. The solar-thermal temperature can raise to above 350 °C and meet the temperature requirement for ammonia synthesis.</description><issn>1359-7345</issn><issn>1364-548X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><sourceid/><recordid>eNqFjjsLwjAUhYMo-FzchfsHqolNfcyiuDno4FYuMdVIk8i9reC_t4Lg6Fm-A98ZjhBjJadKpuvZRRsjtVLza0v0VLrQSaZX5_anZ-tkmeqsK_rMd9lEZaueOO7sAQKGyBXVpqrJQuFKz4AMHEukpLpZ8liCieFpiV0M4LGy5LBkKCIBeh-DQ-BXaLbseCg6RSPt6MuBmOy2p80-ITb5g5xHeuW_p-k__wZYgEL8</recordid><startdate>20241105</startdate><enddate>20241105</enddate><creator>Fu, Rong</creator><creator>Lei, Di</creator><creator>Li, Zhenlu</creator><creator>Zhang, Hangjian</creator><creator>Zhao, Xiaofei</creator><creator>Tao, Shuo</creator><scope/></search><sort><creationdate>20241105</creationdate><title>FeO nanostructure films as solar-thermal conversion materials for ammonia synthesis</title><author>Fu, Rong ; Lei, Di ; Li, Zhenlu ; Zhang, Hangjian ; Zhao, Xiaofei ; Tao, Shuo</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-rsc_primary_d4cc04112g3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><creationdate>2024</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Fu, Rong</creatorcontrib><creatorcontrib>Lei, Di</creatorcontrib><creatorcontrib>Li, Zhenlu</creatorcontrib><creatorcontrib>Zhang, Hangjian</creatorcontrib><creatorcontrib>Zhao, Xiaofei</creatorcontrib><creatorcontrib>Tao, Shuo</creatorcontrib><jtitle>Chemical communications (Cambridge, England)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Fu, Rong</au><au>Lei, Di</au><au>Li, Zhenlu</au><au>Zhang, Hangjian</au><au>Zhao, Xiaofei</au><au>Tao, Shuo</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>FeO nanostructure films as solar-thermal conversion materials for ammonia synthesis</atitle><jtitle>Chemical communications (Cambridge, England)</jtitle><date>2024-11-05</date><risdate>2024</risdate><volume>6</volume><issue>89</issue><spage>1355</spage><epage>1358</epage><pages>1355-1358</pages><issn>1359-7345</issn><eissn>1364-548X</eissn><abstract>Here, we report that black photothermal materials elevate solar heating temperatures across high solar absorption and low infrared radiation. Fe
3
O
4
nanostructure films can be heated to 350 °C under light irradiation, and this system shows effective visible-light-driven ammonia synthesis production of 3677 μg g
−1
h
−1
under gas-solid phase catalysis without noble metals.
Fe
3
O
4
film is composed of dispersed nanoparticles and irregular nanopores, where photons can be trapped by multi-reflection. The solar-thermal temperature can raise to above 350 °C and meet the temperature requirement for ammonia synthesis.</abstract><doi>10.1039/d4cc04112g</doi><tpages>4</tpages></addata></record> |
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| ispartof | Chemical communications (Cambridge, England), 2024-11, Vol.6 (89), p.1355-1358 |
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| source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| title | FeO nanostructure films as solar-thermal conversion materials for ammonia synthesis |
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