Copper-barium-decorated carbon-nanotube composite for electrocatalytic CO reduction to C2 products
A copper-barium-decorated carbon nanotube nanocomposite was designed to promote CO 2 reduction to C2 products (ethylene and ethanol). We achieved a faradaic efficiency of 71% and partial current density of 355 mA cm −2 at −0.7 V vs. RHE. Operando methods revealed catalyst transformation and the cata...
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| Veröffentlicht in: | Journal of materials chemistry. A, Materials for energy and sustainability Materials for energy and sustainability, 2023-06, Vol.11 (25), p.13217-13222 |
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| container_end_page | 13222 |
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| container_issue | 25 |
| container_start_page | 13217 |
| container_title | Journal of materials chemistry. A, Materials for energy and sustainability |
| container_volume | 11 |
| creator | Wu, Feng-Yi Tsai, Hsin-Jung Lee, Tsung-Ju Lin, Zih-Yi Peng, Kang-Shun Chen, Pei-Hsuan Hiraoka, Nozomu Liao, Yen-Fa Hu, Chih-Wei Hsu, Shao-Hui Lu, Ying-Rui Hung, Sung-Fu |
| description | A copper-barium-decorated carbon nanotube nanocomposite was designed to promote CO
2
reduction to C2 products (ethylene and ethanol). We achieved a faradaic efficiency of 71% and partial current density of 355 mA cm
−2
at −0.7 V
vs.
RHE.
Operando
methods revealed catalyst transformation and the catalytic mechanism.
A copper-barium-decorated carbon nanotube nanocomposite enabled a faradaic efficiency of 71% and partial current density of 355 mA cm
−2
at −0.7 V
vs.
RHE. |
| doi_str_mv | 10.1039/d3ta01912h |
| format | Article |
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2
reduction to C2 products (ethylene and ethanol). We achieved a faradaic efficiency of 71% and partial current density of 355 mA cm
−2
at −0.7 V
vs.
RHE.
Operando
methods revealed catalyst transformation and the catalytic mechanism.
A copper-barium-decorated carbon nanotube nanocomposite enabled a faradaic efficiency of 71% and partial current density of 355 mA cm
−2
at −0.7 V
vs.
RHE.</description><identifier>ISSN: 2050-7488</identifier><identifier>EISSN: 2050-7496</identifier><identifier>DOI: 10.1039/d3ta01912h</identifier><ispartof>Journal of materials chemistry. A, Materials for energy and sustainability, 2023-06, Vol.11 (25), p.13217-13222</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27924,27925</link.rule.ids></links><search><creatorcontrib>Wu, Feng-Yi</creatorcontrib><creatorcontrib>Tsai, Hsin-Jung</creatorcontrib><creatorcontrib>Lee, Tsung-Ju</creatorcontrib><creatorcontrib>Lin, Zih-Yi</creatorcontrib><creatorcontrib>Peng, Kang-Shun</creatorcontrib><creatorcontrib>Chen, Pei-Hsuan</creatorcontrib><creatorcontrib>Hiraoka, Nozomu</creatorcontrib><creatorcontrib>Liao, Yen-Fa</creatorcontrib><creatorcontrib>Hu, Chih-Wei</creatorcontrib><creatorcontrib>Hsu, Shao-Hui</creatorcontrib><creatorcontrib>Lu, Ying-Rui</creatorcontrib><creatorcontrib>Hung, Sung-Fu</creatorcontrib><title>Copper-barium-decorated carbon-nanotube composite for electrocatalytic CO reduction to C2 products</title><title>Journal of materials chemistry. A, Materials for energy and sustainability</title><description>A copper-barium-decorated carbon nanotube nanocomposite was designed to promote CO
2
reduction to C2 products (ethylene and ethanol). We achieved a faradaic efficiency of 71% and partial current density of 355 mA cm
−2
at −0.7 V
vs.
RHE.
Operando
methods revealed catalyst transformation and the catalytic mechanism.
A copper-barium-decorated carbon nanotube nanocomposite enabled a faradaic efficiency of 71% and partial current density of 355 mA cm
−2
at −0.7 V
vs.
RHE.</description><issn>2050-7488</issn><issn>2050-7496</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><sourceid/><recordid>eNqFjrFuwkAQRE8oSKBAQx9pf-CSsx2Ir7ZA6dKkR-vzIi6yvae9dcHfAxJKykwzT_OaMWZTuNfCVf6tqxRd4YvyPDPL0m2d_Xj3u6dfruuFWef8426pndt5vzRtwymR2BYlToPtKLCgUgcBpeXRjjiyTi1B4CFxjkpwYgHqKahwQMX-ojFA8wVC3RQ08gjK0JSQhO9DXpn5CftM60c_m5fD_rv5tJLDMUkcUC7Hv-_Vf_4KMRhIxA</recordid><startdate>20230627</startdate><enddate>20230627</enddate><creator>Wu, Feng-Yi</creator><creator>Tsai, Hsin-Jung</creator><creator>Lee, Tsung-Ju</creator><creator>Lin, Zih-Yi</creator><creator>Peng, Kang-Shun</creator><creator>Chen, Pei-Hsuan</creator><creator>Hiraoka, Nozomu</creator><creator>Liao, Yen-Fa</creator><creator>Hu, Chih-Wei</creator><creator>Hsu, Shao-Hui</creator><creator>Lu, Ying-Rui</creator><creator>Hung, Sung-Fu</creator><scope/></search><sort><creationdate>20230627</creationdate><title>Copper-barium-decorated carbon-nanotube composite for electrocatalytic CO reduction to C2 products</title><author>Wu, Feng-Yi ; Tsai, Hsin-Jung ; Lee, Tsung-Ju ; Lin, Zih-Yi ; Peng, Kang-Shun ; Chen, Pei-Hsuan ; Hiraoka, Nozomu ; Liao, Yen-Fa ; Hu, Chih-Wei ; Hsu, Shao-Hui ; Lu, Ying-Rui ; Hung, Sung-Fu</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-rsc_primary_d3ta01912h3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><creationdate>2023</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Wu, Feng-Yi</creatorcontrib><creatorcontrib>Tsai, Hsin-Jung</creatorcontrib><creatorcontrib>Lee, Tsung-Ju</creatorcontrib><creatorcontrib>Lin, Zih-Yi</creatorcontrib><creatorcontrib>Peng, Kang-Shun</creatorcontrib><creatorcontrib>Chen, Pei-Hsuan</creatorcontrib><creatorcontrib>Hiraoka, Nozomu</creatorcontrib><creatorcontrib>Liao, Yen-Fa</creatorcontrib><creatorcontrib>Hu, Chih-Wei</creatorcontrib><creatorcontrib>Hsu, Shao-Hui</creatorcontrib><creatorcontrib>Lu, Ying-Rui</creatorcontrib><creatorcontrib>Hung, Sung-Fu</creatorcontrib><jtitle>Journal of materials chemistry. A, Materials for energy and sustainability</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Wu, Feng-Yi</au><au>Tsai, Hsin-Jung</au><au>Lee, Tsung-Ju</au><au>Lin, Zih-Yi</au><au>Peng, Kang-Shun</au><au>Chen, Pei-Hsuan</au><au>Hiraoka, Nozomu</au><au>Liao, Yen-Fa</au><au>Hu, Chih-Wei</au><au>Hsu, Shao-Hui</au><au>Lu, Ying-Rui</au><au>Hung, Sung-Fu</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Copper-barium-decorated carbon-nanotube composite for electrocatalytic CO reduction to C2 products</atitle><jtitle>Journal of materials chemistry. A, Materials for energy and sustainability</jtitle><date>2023-06-27</date><risdate>2023</risdate><volume>11</volume><issue>25</issue><spage>13217</spage><epage>13222</epage><pages>13217-13222</pages><issn>2050-7488</issn><eissn>2050-7496</eissn><abstract>A copper-barium-decorated carbon nanotube nanocomposite was designed to promote CO
2
reduction to C2 products (ethylene and ethanol). We achieved a faradaic efficiency of 71% and partial current density of 355 mA cm
−2
at −0.7 V
vs.
RHE.
Operando
methods revealed catalyst transformation and the catalytic mechanism.
A copper-barium-decorated carbon nanotube nanocomposite enabled a faradaic efficiency of 71% and partial current density of 355 mA cm
−2
at −0.7 V
vs.
RHE.</abstract><doi>10.1039/d3ta01912h</doi><tpages>6</tpages></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 2050-7488 |
| ispartof | Journal of materials chemistry. A, Materials for energy and sustainability, 2023-06, Vol.11 (25), p.13217-13222 |
| issn | 2050-7488 2050-7496 |
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| recordid | cdi_rsc_primary_d3ta01912h |
| source | Royal Society Of Chemistry Journals 2008- |
| title | Copper-barium-decorated carbon-nanotube composite for electrocatalytic CO reduction to C2 products |
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