Enhanced solar absorption and photoelectrochemical properties of Al-reduced TiO/TiO/CdS heterojunction nanorods
Oxygen-deficient TiO 2 -based composites have attracted widespread attention due to their promoted light-harvesting capacity and energy conversion efficiency, beneficial for water splitting. Despite being a facile, secure-safe and undefiled route for preparing blackened TiO 2 , the Al-reduction meth...
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| Veröffentlicht in: | New journal of chemistry 2023-06, Vol.47 (22), p.1672-1678 |
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| container_issue | 22 |
| container_start_page | 1672 |
| container_title | New journal of chemistry |
| container_volume | 47 |
| creator | Li, Xiao Hou, Jingshan Wang, Jing Huang, Yanwei Zhao, Guoying Zhang, Ganghua Fang, Yongzheng |
| description | Oxygen-deficient TiO
2
-based composites have attracted widespread attention due to their promoted light-harvesting capacity and energy conversion efficiency, beneficial for water splitting. Despite being a facile, secure-safe and undefiled route for preparing blackened TiO
2
, the Al-reduction method has not been adopted for preparing TiO
2
/TiO
2−
x
/CdS composite films. Herein, TiO
2
/TiO
2−
x
/CdS composite nanorods were successfully fabricated by combining hydrothermal, Al-reduction and chemical bath deposition (CBD) techniques. Enhanced visible-light absorption and photoelectrochemical performances have been achieved using TiO
2
/TiO
2−
x
/CdS heterojunction nanorods. The photocurrent density of TiO
2
/TiO
2−
x
/CdS was obtained to be 7.75 mA cm
−2
at 0 V
vs.
Ag/AgCl under AM 1.5 G illumination, which was 77.5-fold and 12.1-fold higher than those of bare TiO
2
and CdS, respectively. This work may offer new insights for realizing TiO
2
-based composites with improved solar absorption for photoelectrochemical applications.
TiO
2
/TiO
2−
x
/CdS heterojunction nanorods with high PEC performance were successfully prepared by combining hydrothermal synthesis, Al-reduction and CBD techniques. |
| doi_str_mv | 10.1039/d3nj01610b |
| format | Article |
| fullrecord | <record><control><sourceid>rsc</sourceid><recordid>TN_cdi_rsc_primary_d3nj01610b</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>d3nj01610b</sourcerecordid><originalsourceid>FETCH-rsc_primary_d3nj01610b3</originalsourceid><addsrcrecordid>eNqFj8FqAjEURUOpUG3duC_kB0bzOmPKLEWU7rqoe4nJk8mQyQsvmYV_r5aCyy4u98KBA1eIBaglqLpduTr2CjSo05OYQq3bqv3Q8Hzb0DSVWjf6Rcxy7pUC-NQwFbSLnYkWncwUDEtzysSpeIrSRCdTR4UwoC1MtsPBWxNkYkrIxWOWdJabUDG68a44-O_VPVv3IzssyNSP0f7KoonE5PKbmJxNyDj_61fxvt8dtl8VZ3tM7AfDl-PjRf0fvwKnmkzq</addsrcrecordid><sourcetype>Publisher</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype></control><display><type>article</type><title>Enhanced solar absorption and photoelectrochemical properties of Al-reduced TiO/TiO/CdS heterojunction nanorods</title><source>Royal Society Of Chemistry Journals 2008-</source><source>Alma/SFX Local Collection</source><creator>Li, Xiao ; Hou, Jingshan ; Wang, Jing ; Huang, Yanwei ; Zhao, Guoying ; Zhang, Ganghua ; Fang, Yongzheng</creator><creatorcontrib>Li, Xiao ; Hou, Jingshan ; Wang, Jing ; Huang, Yanwei ; Zhao, Guoying ; Zhang, Ganghua ; Fang, Yongzheng</creatorcontrib><description>Oxygen-deficient TiO
2
-based composites have attracted widespread attention due to their promoted light-harvesting capacity and energy conversion efficiency, beneficial for water splitting. Despite being a facile, secure-safe and undefiled route for preparing blackened TiO
2
, the Al-reduction method has not been adopted for preparing TiO
2
/TiO
2−
x
/CdS composite films. Herein, TiO
2
/TiO
2−
x
/CdS composite nanorods were successfully fabricated by combining hydrothermal, Al-reduction and chemical bath deposition (CBD) techniques. Enhanced visible-light absorption and photoelectrochemical performances have been achieved using TiO
2
/TiO
2−
x
/CdS heterojunction nanorods. The photocurrent density of TiO
2
/TiO
2−
x
/CdS was obtained to be 7.75 mA cm
−2
at 0 V
vs.
Ag/AgCl under AM 1.5 G illumination, which was 77.5-fold and 12.1-fold higher than those of bare TiO
2
and CdS, respectively. This work may offer new insights for realizing TiO
2
-based composites with improved solar absorption for photoelectrochemical applications.
TiO
2
/TiO
2−
x
/CdS heterojunction nanorods with high PEC performance were successfully prepared by combining hydrothermal synthesis, Al-reduction and CBD techniques.</description><identifier>ISSN: 1144-0546</identifier><identifier>EISSN: 1369-9261</identifier><identifier>DOI: 10.1039/d3nj01610b</identifier><ispartof>New journal of chemistry, 2023-06, Vol.47 (22), p.1672-1678</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,27901,27902</link.rule.ids></links><search><creatorcontrib>Li, Xiao</creatorcontrib><creatorcontrib>Hou, Jingshan</creatorcontrib><creatorcontrib>Wang, Jing</creatorcontrib><creatorcontrib>Huang, Yanwei</creatorcontrib><creatorcontrib>Zhao, Guoying</creatorcontrib><creatorcontrib>Zhang, Ganghua</creatorcontrib><creatorcontrib>Fang, Yongzheng</creatorcontrib><title>Enhanced solar absorption and photoelectrochemical properties of Al-reduced TiO/TiO/CdS heterojunction nanorods</title><title>New journal of chemistry</title><description>Oxygen-deficient TiO
2
-based composites have attracted widespread attention due to their promoted light-harvesting capacity and energy conversion efficiency, beneficial for water splitting. Despite being a facile, secure-safe and undefiled route for preparing blackened TiO
2
, the Al-reduction method has not been adopted for preparing TiO
2
/TiO
2−
x
/CdS composite films. Herein, TiO
2
/TiO
2−
x
/CdS composite nanorods were successfully fabricated by combining hydrothermal, Al-reduction and chemical bath deposition (CBD) techniques. Enhanced visible-light absorption and photoelectrochemical performances have been achieved using TiO
2
/TiO
2−
x
/CdS heterojunction nanorods. The photocurrent density of TiO
2
/TiO
2−
x
/CdS was obtained to be 7.75 mA cm
−2
at 0 V
vs.
Ag/AgCl under AM 1.5 G illumination, which was 77.5-fold and 12.1-fold higher than those of bare TiO
2
and CdS, respectively. This work may offer new insights for realizing TiO
2
-based composites with improved solar absorption for photoelectrochemical applications.
TiO
2
/TiO
2−
x
/CdS heterojunction nanorods with high PEC performance were successfully prepared by combining hydrothermal synthesis, Al-reduction and CBD techniques.</description><issn>1144-0546</issn><issn>1369-9261</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><sourceid/><recordid>eNqFj8FqAjEURUOpUG3duC_kB0bzOmPKLEWU7rqoe4nJk8mQyQsvmYV_r5aCyy4u98KBA1eIBaglqLpduTr2CjSo05OYQq3bqv3Q8Hzb0DSVWjf6Rcxy7pUC-NQwFbSLnYkWncwUDEtzysSpeIrSRCdTR4UwoC1MtsPBWxNkYkrIxWOWdJabUDG68a44-O_VPVv3IzssyNSP0f7KoonE5PKbmJxNyDj_61fxvt8dtl8VZ3tM7AfDl-PjRf0fvwKnmkzq</recordid><startdate>20230606</startdate><enddate>20230606</enddate><creator>Li, Xiao</creator><creator>Hou, Jingshan</creator><creator>Wang, Jing</creator><creator>Huang, Yanwei</creator><creator>Zhao, Guoying</creator><creator>Zhang, Ganghua</creator><creator>Fang, Yongzheng</creator><scope/></search><sort><creationdate>20230606</creationdate><title>Enhanced solar absorption and photoelectrochemical properties of Al-reduced TiO/TiO/CdS heterojunction nanorods</title><author>Li, Xiao ; Hou, Jingshan ; Wang, Jing ; Huang, Yanwei ; Zhao, Guoying ; Zhang, Ganghua ; Fang, Yongzheng</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-rsc_primary_d3nj01610b3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><creationdate>2023</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Li, Xiao</creatorcontrib><creatorcontrib>Hou, Jingshan</creatorcontrib><creatorcontrib>Wang, Jing</creatorcontrib><creatorcontrib>Huang, Yanwei</creatorcontrib><creatorcontrib>Zhao, Guoying</creatorcontrib><creatorcontrib>Zhang, Ganghua</creatorcontrib><creatorcontrib>Fang, Yongzheng</creatorcontrib><jtitle>New journal of chemistry</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Li, Xiao</au><au>Hou, Jingshan</au><au>Wang, Jing</au><au>Huang, Yanwei</au><au>Zhao, Guoying</au><au>Zhang, Ganghua</au><au>Fang, Yongzheng</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Enhanced solar absorption and photoelectrochemical properties of Al-reduced TiO/TiO/CdS heterojunction nanorods</atitle><jtitle>New journal of chemistry</jtitle><date>2023-06-06</date><risdate>2023</risdate><volume>47</volume><issue>22</issue><spage>1672</spage><epage>1678</epage><pages>1672-1678</pages><issn>1144-0546</issn><eissn>1369-9261</eissn><abstract>Oxygen-deficient TiO
2
-based composites have attracted widespread attention due to their promoted light-harvesting capacity and energy conversion efficiency, beneficial for water splitting. Despite being a facile, secure-safe and undefiled route for preparing blackened TiO
2
, the Al-reduction method has not been adopted for preparing TiO
2
/TiO
2−
x
/CdS composite films. Herein, TiO
2
/TiO
2−
x
/CdS composite nanorods were successfully fabricated by combining hydrothermal, Al-reduction and chemical bath deposition (CBD) techniques. Enhanced visible-light absorption and photoelectrochemical performances have been achieved using TiO
2
/TiO
2−
x
/CdS heterojunction nanorods. The photocurrent density of TiO
2
/TiO
2−
x
/CdS was obtained to be 7.75 mA cm
−2
at 0 V
vs.
Ag/AgCl under AM 1.5 G illumination, which was 77.5-fold and 12.1-fold higher than those of bare TiO
2
and CdS, respectively. This work may offer new insights for realizing TiO
2
-based composites with improved solar absorption for photoelectrochemical applications.
TiO
2
/TiO
2−
x
/CdS heterojunction nanorods with high PEC performance were successfully prepared by combining hydrothermal synthesis, Al-reduction and CBD techniques.</abstract><doi>10.1039/d3nj01610b</doi><tpages>7</tpages></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 1144-0546 |
| ispartof | New journal of chemistry, 2023-06, Vol.47 (22), p.1672-1678 |
| issn | 1144-0546 1369-9261 |
| language | |
| recordid | cdi_rsc_primary_d3nj01610b |
| source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| title | Enhanced solar absorption and photoelectrochemical properties of Al-reduced TiO/TiO/CdS heterojunction nanorods |
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