Facile synthesis of hierarchical SnSe nanosheets-hydrogel evaporators for sustainable solar-powered desalination
In contrast to the demand for freshwater that is increasing continuously due to population growth and economic growth, the availability of freshwater resources is decreasing rapidly due to environmental pollution and climate change. Solar-powered desalination is an eco-friendly and efficient way to...
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Veröffentlicht in: | Journal of materials chemistry. A, Materials for energy and sustainability Materials for energy and sustainability, 2022-05, Vol.1 (19), p.1672-1681 |
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container_title | Journal of materials chemistry. A, Materials for energy and sustainability |
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creator | Li, Feng Cai, Xiaoqing Jing, Gaoxing Huang, Ruijia Song, Guangjie Wang, Dong Chen, Wenwen |
description | In contrast to the demand for freshwater that is increasing continuously due to population growth and economic growth, the availability of freshwater resources is decreasing rapidly due to environmental pollution and climate change. Solar-powered desalination is an eco-friendly and efficient way to produce freshwater. Herein, a facile method based on the Rayleigh-Bénard convection was developed to synthesize hierarchical nanomaterials-hydrogel evaporators. The SnSe nanosheets were encapsulated in poly(hydroxyethyl 2-methacrylate) hydrogel, and the resultant thin, porous SnSe-hydrogel composite layer was seamlessly integrated into the hydrogel matrix. Under one-sun irradiation, the SnSe-hydrogel evaporator demonstrated a high water-evaporation rate (2.20 kg m
−2
h
−1
) and high energy conversion efficiency (91.70%). Moreover, the evaporator not only had excellent long-term mechanical properties, but also demonstrated excellent ion-rejection rates during a long-term seawater evaporation test, which indicated the potential application of the evaporator to sustainable solar-powered desalination in the offing or on ocean-going vessels. Our results provide a route for the synthesis of functional nanocomposite hydrogels for solar-powered water purification, sensing, biomedical, and other fields.
A facile method based on the Rayleigh-Bénard convection was developed to synthesize hierarchical SnSe nanosheets-hydrogel evaporators, which have potential applications in sustainable solar-powered desalination due to their excellent water-evaporation performance. |
doi_str_mv | 10.1039/d2ta01264b |
format | Article |
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−2
h
−1
) and high energy conversion efficiency (91.70%). Moreover, the evaporator not only had excellent long-term mechanical properties, but also demonstrated excellent ion-rejection rates during a long-term seawater evaporation test, which indicated the potential application of the evaporator to sustainable solar-powered desalination in the offing or on ocean-going vessels. Our results provide a route for the synthesis of functional nanocomposite hydrogels for solar-powered water purification, sensing, biomedical, and other fields.
A facile method based on the Rayleigh-Bénard convection was developed to synthesize hierarchical SnSe nanosheets-hydrogel evaporators, which have potential applications in sustainable solar-powered desalination due to their excellent water-evaporation performance.</description><identifier>ISSN: 2050-7488</identifier><identifier>EISSN: 2050-7496</identifier><identifier>DOI: 10.1039/d2ta01264b</identifier><language>eng</language><publisher>Cambridge: Royal Society of Chemistry</publisher><subject>Climate change ; Convection ; Desalination ; Economic development ; Economic growth ; Energy conversion ; Energy conversion efficiency ; Evaporation ; Evaporation rate ; Evaporators ; Freshwater resources ; Hydrogels ; Irradiation ; Mechanical properties ; Nanocomposites ; Nanomaterials ; Nanosheets ; Nanotechnology ; Population growth ; Radiation ; Rayleigh-Benard convection ; Rejection rate ; Seawater ; Solar energy ; Synthesis ; Water availability ; Water purification</subject><ispartof>Journal of materials chemistry. A, Materials for energy and sustainability, 2022-05, Vol.1 (19), p.1672-1681</ispartof><rights>Copyright Royal Society of Chemistry 2022</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c281t-702c152af2c30f0cdf5f74b6b265638e552896d69527b7bec82626504a71b5be3</citedby><cites>FETCH-LOGICAL-c281t-702c152af2c30f0cdf5f74b6b265638e552896d69527b7bec82626504a71b5be3</cites><orcidid>0000-0001-5137-0771 ; 0000-0002-5958-2696</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27924,27925</link.rule.ids></links><search><creatorcontrib>Li, Feng</creatorcontrib><creatorcontrib>Cai, Xiaoqing</creatorcontrib><creatorcontrib>Jing, Gaoxing</creatorcontrib><creatorcontrib>Huang, Ruijia</creatorcontrib><creatorcontrib>Song, Guangjie</creatorcontrib><creatorcontrib>Wang, Dong</creatorcontrib><creatorcontrib>Chen, Wenwen</creatorcontrib><title>Facile synthesis of hierarchical SnSe nanosheets-hydrogel evaporators for sustainable solar-powered desalination</title><title>Journal of materials chemistry. A, Materials for energy and sustainability</title><description>In contrast to the demand for freshwater that is increasing continuously due to population growth and economic growth, the availability of freshwater resources is decreasing rapidly due to environmental pollution and climate change. Solar-powered desalination is an eco-friendly and efficient way to produce freshwater. Herein, a facile method based on the Rayleigh-Bénard convection was developed to synthesize hierarchical nanomaterials-hydrogel evaporators. The SnSe nanosheets were encapsulated in poly(hydroxyethyl 2-methacrylate) hydrogel, and the resultant thin, porous SnSe-hydrogel composite layer was seamlessly integrated into the hydrogel matrix. Under one-sun irradiation, the SnSe-hydrogel evaporator demonstrated a high water-evaporation rate (2.20 kg m
−2
h
−1
) and high energy conversion efficiency (91.70%). Moreover, the evaporator not only had excellent long-term mechanical properties, but also demonstrated excellent ion-rejection rates during a long-term seawater evaporation test, which indicated the potential application of the evaporator to sustainable solar-powered desalination in the offing or on ocean-going vessels. Our results provide a route for the synthesis of functional nanocomposite hydrogels for solar-powered water purification, sensing, biomedical, and other fields.
A facile method based on the Rayleigh-Bénard convection was developed to synthesize hierarchical SnSe nanosheets-hydrogel evaporators, which have potential applications in sustainable solar-powered desalination due to their excellent water-evaporation performance.</description><subject>Climate change</subject><subject>Convection</subject><subject>Desalination</subject><subject>Economic development</subject><subject>Economic growth</subject><subject>Energy conversion</subject><subject>Energy conversion efficiency</subject><subject>Evaporation</subject><subject>Evaporation rate</subject><subject>Evaporators</subject><subject>Freshwater resources</subject><subject>Hydrogels</subject><subject>Irradiation</subject><subject>Mechanical properties</subject><subject>Nanocomposites</subject><subject>Nanomaterials</subject><subject>Nanosheets</subject><subject>Nanotechnology</subject><subject>Population growth</subject><subject>Radiation</subject><subject>Rayleigh-Benard convection</subject><subject>Rejection rate</subject><subject>Seawater</subject><subject>Solar energy</subject><subject>Synthesis</subject><subject>Water availability</subject><subject>Water purification</subject><issn>2050-7488</issn><issn>2050-7496</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><recordid>eNpFkMFLwzAUh4MoOOYu3oWAN6GapEvaHud0Kgw8bJ5Lkr7YjtrUvEzZf2_nZL7Le_D7-D34CLnk7JaztLirRNSMCzU1J2QkmGRJNi3U6fHO83MyQdywYXLGVFGMSL_QtmmB4q6LNWCD1DtaNxB0sHVjdUtX3QpopzuPNUDEpN5Vwb9DS-FL9z7o6ANS5wPFLUbddNrs63yrQ9L7bwhQ0QpQt0MSG99dkDOnW4TJ3x6Tt8Xjev6cLF-fXuazZWJFzmOSMWG5FNoJmzLHbOWky6ZGGaGkSnOQUuSFqlQhRWYyAzYXaojYVGfcSAPpmFwfevvgP7eAsdz4beiGl6VQSgomBJcDdXOgbPCIAVzZh-ZDh13JWbmXWj6I9exX6v0AXx3ggPbI_UtPfwD-TnUc</recordid><startdate>20220517</startdate><enddate>20220517</enddate><creator>Li, Feng</creator><creator>Cai, Xiaoqing</creator><creator>Jing, Gaoxing</creator><creator>Huang, Ruijia</creator><creator>Song, Guangjie</creator><creator>Wang, Dong</creator><creator>Chen, Wenwen</creator><general>Royal Society of Chemistry</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7SR</scope><scope>7ST</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>C1K</scope><scope>JG9</scope><scope>L7M</scope><scope>SOI</scope><orcidid>https://orcid.org/0000-0001-5137-0771</orcidid><orcidid>https://orcid.org/0000-0002-5958-2696</orcidid></search><sort><creationdate>20220517</creationdate><title>Facile synthesis of hierarchical SnSe nanosheets-hydrogel evaporators for sustainable solar-powered desalination</title><author>Li, Feng ; Cai, Xiaoqing ; Jing, Gaoxing ; Huang, Ruijia ; Song, Guangjie ; Wang, Dong ; Chen, Wenwen</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c281t-702c152af2c30f0cdf5f74b6b265638e552896d69527b7bec82626504a71b5be3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Climate change</topic><topic>Convection</topic><topic>Desalination</topic><topic>Economic development</topic><topic>Economic growth</topic><topic>Energy conversion</topic><topic>Energy conversion efficiency</topic><topic>Evaporation</topic><topic>Evaporation rate</topic><topic>Evaporators</topic><topic>Freshwater resources</topic><topic>Hydrogels</topic><topic>Irradiation</topic><topic>Mechanical properties</topic><topic>Nanocomposites</topic><topic>Nanomaterials</topic><topic>Nanosheets</topic><topic>Nanotechnology</topic><topic>Population growth</topic><topic>Radiation</topic><topic>Rayleigh-Benard convection</topic><topic>Rejection rate</topic><topic>Seawater</topic><topic>Solar energy</topic><topic>Synthesis</topic><topic>Water availability</topic><topic>Water purification</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Li, Feng</creatorcontrib><creatorcontrib>Cai, Xiaoqing</creatorcontrib><creatorcontrib>Jing, Gaoxing</creatorcontrib><creatorcontrib>Huang, Ruijia</creatorcontrib><creatorcontrib>Song, Guangjie</creatorcontrib><creatorcontrib>Wang, Dong</creatorcontrib><creatorcontrib>Chen, Wenwen</creatorcontrib><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>Environment Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Environment Abstracts</collection><jtitle>Journal of materials chemistry. A, Materials for energy and sustainability</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Li, Feng</au><au>Cai, Xiaoqing</au><au>Jing, Gaoxing</au><au>Huang, Ruijia</au><au>Song, Guangjie</au><au>Wang, Dong</au><au>Chen, Wenwen</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Facile synthesis of hierarchical SnSe nanosheets-hydrogel evaporators for sustainable solar-powered desalination</atitle><jtitle>Journal of materials chemistry. A, Materials for energy and sustainability</jtitle><date>2022-05-17</date><risdate>2022</risdate><volume>1</volume><issue>19</issue><spage>1672</spage><epage>1681</epage><pages>1672-1681</pages><issn>2050-7488</issn><eissn>2050-7496</eissn><abstract>In contrast to the demand for freshwater that is increasing continuously due to population growth and economic growth, the availability of freshwater resources is decreasing rapidly due to environmental pollution and climate change. Solar-powered desalination is an eco-friendly and efficient way to produce freshwater. Herein, a facile method based on the Rayleigh-Bénard convection was developed to synthesize hierarchical nanomaterials-hydrogel evaporators. The SnSe nanosheets were encapsulated in poly(hydroxyethyl 2-methacrylate) hydrogel, and the resultant thin, porous SnSe-hydrogel composite layer was seamlessly integrated into the hydrogel matrix. Under one-sun irradiation, the SnSe-hydrogel evaporator demonstrated a high water-evaporation rate (2.20 kg m
−2
h
−1
) and high energy conversion efficiency (91.70%). Moreover, the evaporator not only had excellent long-term mechanical properties, but also demonstrated excellent ion-rejection rates during a long-term seawater evaporation test, which indicated the potential application of the evaporator to sustainable solar-powered desalination in the offing or on ocean-going vessels. Our results provide a route for the synthesis of functional nanocomposite hydrogels for solar-powered water purification, sensing, biomedical, and other fields.
A facile method based on the Rayleigh-Bénard convection was developed to synthesize hierarchical SnSe nanosheets-hydrogel evaporators, which have potential applications in sustainable solar-powered desalination due to their excellent water-evaporation performance.</abstract><cop>Cambridge</cop><pub>Royal Society of Chemistry</pub><doi>10.1039/d2ta01264b</doi><tpages>1</tpages><orcidid>https://orcid.org/0000-0001-5137-0771</orcidid><orcidid>https://orcid.org/0000-0002-5958-2696</orcidid></addata></record> |
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source | Royal Society Of Chemistry Journals 2008- |
subjects | Climate change Convection Desalination Economic development Economic growth Energy conversion Energy conversion efficiency Evaporation Evaporation rate Evaporators Freshwater resources Hydrogels Irradiation Mechanical properties Nanocomposites Nanomaterials Nanosheets Nanotechnology Population growth Radiation Rayleigh-Benard convection Rejection rate Seawater Solar energy Synthesis Water availability Water purification |
title | Facile synthesis of hierarchical SnSe nanosheets-hydrogel evaporators for sustainable solar-powered desalination |
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