Salicylaldehydate coordinated two-dimensional-conjugated metal-organic frameworks
A novel class of copper-based 2D-c-MOF was synthesized from 1,3,5-triformylphloroglucinol using green mechano-chemistry. Herein, metal coordination with the salicylaldehyde functional moiety was explored for the first time in MOFs. Moreover, an intrinsic semiconductive copper-based SA-MOF thin film...
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| Veröffentlicht in: | Chemical communications (Cambridge, England) England), 2023-02, Vol.59 (18), p.268-2611 |
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| creator | Mohammed, Abdul Khayum Pena-Sánchez, Pilar Pandikassala, Ajmal Gaber, Safa AlKhoori, Ayesha A Skorjanc, Tina Polychronopoulou, Kyriaki Kurungot, Sreekumar Gándara, Felipe Shetty, Dinesh |
| description | A novel class of copper-based 2D-c-MOF was synthesized from 1,3,5-triformylphloroglucinol using green mechano-chemistry. Herein, metal coordination with the salicylaldehyde functional moiety was explored for the first time in MOFs. Moreover, an intrinsic semiconductive copper-based SA-MOF thin film was fabricated using an
in situ
salt-free method at room temperature.
We have demonstrated a facile, scalable, and green synthetic route to produce a novel class of semiconductive 2D-c-MOFs (SA-MOFs). This novel MOF chemistry opens rich opportunities for the exploration of functionally diverse open frameworks. |
| doi_str_mv | 10.1039/d2cc06283f |
| format | Article |
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in situ
salt-free method at room temperature.
We have demonstrated a facile, scalable, and green synthetic route to produce a novel class of semiconductive 2D-c-MOFs (SA-MOFs). This novel MOF chemistry opens rich opportunities for the exploration of functionally diverse open frameworks.</description><identifier>ISSN: 1359-7345</identifier><identifier>EISSN: 1364-548X</identifier><identifier>DOI: 10.1039/d2cc06283f</identifier><identifier>PMID: 36757151</identifier><language>eng</language><publisher>England: Royal Society of Chemistry</publisher><subject>Copper ; Metal-organic frameworks ; Room temperature ; Thin films</subject><ispartof>Chemical communications (Cambridge, England), 2023-02, Vol.59 (18), p.268-2611</ispartof><rights>Copyright Royal Society of Chemistry 2023</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c304t-1bfcc66a1967704c5686f0ff01f8a18e3a7297fc2a7556ae09f11f127ad0c86b3</citedby><cites>FETCH-LOGICAL-c304t-1bfcc66a1967704c5686f0ff01f8a18e3a7297fc2a7556ae09f11f127ad0c86b3</cites><orcidid>0000-0001-8626-1751 ; 0000-0003-4887-2855 ; 0000-0002-6823-0465 ; 0000-0001-5456-0386 ; 0000-0002-0723-9941 ; 0000-0001-5446-7923 ; 0000-0002-5331-2716 ; 0000-0002-1671-6260</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27924,27925</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/36757151$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Mohammed, Abdul Khayum</creatorcontrib><creatorcontrib>Pena-Sánchez, Pilar</creatorcontrib><creatorcontrib>Pandikassala, Ajmal</creatorcontrib><creatorcontrib>Gaber, Safa</creatorcontrib><creatorcontrib>AlKhoori, Ayesha A</creatorcontrib><creatorcontrib>Skorjanc, Tina</creatorcontrib><creatorcontrib>Polychronopoulou, Kyriaki</creatorcontrib><creatorcontrib>Kurungot, Sreekumar</creatorcontrib><creatorcontrib>Gándara, Felipe</creatorcontrib><creatorcontrib>Shetty, Dinesh</creatorcontrib><title>Salicylaldehydate coordinated two-dimensional-conjugated metal-organic frameworks</title><title>Chemical communications (Cambridge, England)</title><addtitle>Chem Commun (Camb)</addtitle><description>A novel class of copper-based 2D-c-MOF was synthesized from 1,3,5-triformylphloroglucinol using green mechano-chemistry. Herein, metal coordination with the salicylaldehyde functional moiety was explored for the first time in MOFs. Moreover, an intrinsic semiconductive copper-based SA-MOF thin film was fabricated using an
in situ
salt-free method at room temperature.
We have demonstrated a facile, scalable, and green synthetic route to produce a novel class of semiconductive 2D-c-MOFs (SA-MOFs). This novel MOF chemistry opens rich opportunities for the exploration of functionally diverse open frameworks.</description><subject>Copper</subject><subject>Metal-organic frameworks</subject><subject>Room temperature</subject><subject>Thin films</subject><issn>1359-7345</issn><issn>1364-548X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNpFkEtLw0AUhQdRbK1u3CsFd0J0HplHlhKtCgURFdyF6TxqapKpMwkl_97pw3o393DPx-FyADhH8AZBkt1qrBRkWBB7AIaIsDShqfg8XGuaJZykdABOQljAOIiKYzAgjFOOKBqC1zdZlaqvZKXNV69la8bKOa_LJko9blcu0WVtmlC6RlaJcs2im2-s2rTx4PxcNqUaWy9rs3L-O5yCIyurYM52ewQ-Jg_v-VMyfXl8zu-miSIwbRM0s0oxJlHGOIepokwwC62FyAqJhCGS44xbhSWnlEkDM4uQRZhLDZVgMzICV9vcpXc_nQltsXCdj0-GAnMBCSaCp5G63lLKuxC8scXSl7X0fYFgsW6vuMd5vmlvEuHLXWQ3q43eo391ReBiC_ig9u5__eQX0dd1Hw</recordid><startdate>20230228</startdate><enddate>20230228</enddate><creator>Mohammed, Abdul Khayum</creator><creator>Pena-Sánchez, Pilar</creator><creator>Pandikassala, Ajmal</creator><creator>Gaber, Safa</creator><creator>AlKhoori, Ayesha A</creator><creator>Skorjanc, Tina</creator><creator>Polychronopoulou, Kyriaki</creator><creator>Kurungot, Sreekumar</creator><creator>Gándara, Felipe</creator><creator>Shetty, Dinesh</creator><general>Royal Society of Chemistry</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><orcidid>https://orcid.org/0000-0001-8626-1751</orcidid><orcidid>https://orcid.org/0000-0003-4887-2855</orcidid><orcidid>https://orcid.org/0000-0002-6823-0465</orcidid><orcidid>https://orcid.org/0000-0001-5456-0386</orcidid><orcidid>https://orcid.org/0000-0002-0723-9941</orcidid><orcidid>https://orcid.org/0000-0001-5446-7923</orcidid><orcidid>https://orcid.org/0000-0002-5331-2716</orcidid><orcidid>https://orcid.org/0000-0002-1671-6260</orcidid></search><sort><creationdate>20230228</creationdate><title>Salicylaldehydate coordinated two-dimensional-conjugated metal-organic frameworks</title><author>Mohammed, Abdul Khayum ; Pena-Sánchez, Pilar ; Pandikassala, Ajmal ; Gaber, Safa ; AlKhoori, Ayesha A ; Skorjanc, Tina ; Polychronopoulou, Kyriaki ; Kurungot, Sreekumar ; Gándara, Felipe ; Shetty, Dinesh</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c304t-1bfcc66a1967704c5686f0ff01f8a18e3a7297fc2a7556ae09f11f127ad0c86b3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Copper</topic><topic>Metal-organic frameworks</topic><topic>Room temperature</topic><topic>Thin films</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Mohammed, Abdul Khayum</creatorcontrib><creatorcontrib>Pena-Sánchez, Pilar</creatorcontrib><creatorcontrib>Pandikassala, Ajmal</creatorcontrib><creatorcontrib>Gaber, Safa</creatorcontrib><creatorcontrib>AlKhoori, Ayesha A</creatorcontrib><creatorcontrib>Skorjanc, Tina</creatorcontrib><creatorcontrib>Polychronopoulou, Kyriaki</creatorcontrib><creatorcontrib>Kurungot, Sreekumar</creatorcontrib><creatorcontrib>Gándara, Felipe</creatorcontrib><creatorcontrib>Shetty, Dinesh</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Chemical communications (Cambridge, England)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Mohammed, Abdul Khayum</au><au>Pena-Sánchez, Pilar</au><au>Pandikassala, Ajmal</au><au>Gaber, Safa</au><au>AlKhoori, Ayesha A</au><au>Skorjanc, Tina</au><au>Polychronopoulou, Kyriaki</au><au>Kurungot, Sreekumar</au><au>Gándara, Felipe</au><au>Shetty, Dinesh</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Salicylaldehydate coordinated two-dimensional-conjugated metal-organic frameworks</atitle><jtitle>Chemical communications (Cambridge, England)</jtitle><addtitle>Chem Commun (Camb)</addtitle><date>2023-02-28</date><risdate>2023</risdate><volume>59</volume><issue>18</issue><spage>268</spage><epage>2611</epage><pages>268-2611</pages><issn>1359-7345</issn><eissn>1364-548X</eissn><abstract>A novel class of copper-based 2D-c-MOF was synthesized from 1,3,5-triformylphloroglucinol using green mechano-chemistry. Herein, metal coordination with the salicylaldehyde functional moiety was explored for the first time in MOFs. Moreover, an intrinsic semiconductive copper-based SA-MOF thin film was fabricated using an
in situ
salt-free method at room temperature.
We have demonstrated a facile, scalable, and green synthetic route to produce a novel class of semiconductive 2D-c-MOFs (SA-MOFs). This novel MOF chemistry opens rich opportunities for the exploration of functionally diverse open frameworks.</abstract><cop>England</cop><pub>Royal Society of Chemistry</pub><pmid>36757151</pmid><doi>10.1039/d2cc06283f</doi><tpages>4</tpages><orcidid>https://orcid.org/0000-0001-8626-1751</orcidid><orcidid>https://orcid.org/0000-0003-4887-2855</orcidid><orcidid>https://orcid.org/0000-0002-6823-0465</orcidid><orcidid>https://orcid.org/0000-0001-5456-0386</orcidid><orcidid>https://orcid.org/0000-0002-0723-9941</orcidid><orcidid>https://orcid.org/0000-0001-5446-7923</orcidid><orcidid>https://orcid.org/0000-0002-5331-2716</orcidid><orcidid>https://orcid.org/0000-0002-1671-6260</orcidid></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 1359-7345 |
| ispartof | Chemical communications (Cambridge, England), 2023-02, Vol.59 (18), p.268-2611 |
| issn | 1359-7345 1364-548X |
| language | eng |
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| source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| subjects | Copper Metal-organic frameworks Room temperature Thin films |
| title | Salicylaldehydate coordinated two-dimensional-conjugated metal-organic frameworks |
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