Structural adaptations of electrosprayed aromatic oligoamide foldamers on Ag(111)
Aromatic foldamers are promising for applications such as molecular recognition and molecular machinery. For many of these, defect free, 2D-crystaline monolayers are needed. To this end, submonolayers were prepared in ultra-high vacuum (UHV) on Ag(111) via electrospray controlled ion beam deposition...
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| Veröffentlicht in: | Chemical communications (Cambridge, England) England), 2022-08, Vol.58 (64), p.8938-8941 |
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| container_title | Chemical communications (Cambridge, England) |
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| creator | Meier, Dennis Schoof, Benedikt Wang, Jinhua Li, Xuesong Walz, Andreas Huettig, Annette Schlichting, Hartmut Rosu, Frédéric Gabelica, Valérie Maurizot, Victor Reichert, Joachim Papageorgiou, Anthoula C Huc, Ivan Barth, Johannes V |
| description | Aromatic foldamers are promising for applications such as molecular recognition and molecular machinery. For many of these, defect free, 2D-crystaline monolayers are needed. To this end, submonolayers were prepared in ultra-high vacuum (UHV) on Ag(111)
via
electrospray controlled ion beam deposition (ES-CIBD). On the surface, the unfolded state is unambiguously identified by real-space single-molecule imaging using scanning tunnelling microscopy (STM) and it is found to assemble in regular structures.
Stable molecular helices unexpectedly unfold to ribbons on a planar metal surface under ultra-high vacuum. These ribbons self-assemble in regular two-dimensional islands. |
| doi_str_mv | 10.1039/d2cc03286d |
| format | Article |
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via
electrospray controlled ion beam deposition (ES-CIBD). On the surface, the unfolded state is unambiguously identified by real-space single-molecule imaging using scanning tunnelling microscopy (STM) and it is found to assemble in regular structures.
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via
electrospray controlled ion beam deposition (ES-CIBD). On the surface, the unfolded state is unambiguously identified by real-space single-molecule imaging using scanning tunnelling microscopy (STM) and it is found to assemble in regular structures.
Stable molecular helices unexpectedly unfold to ribbons on a planar metal surface under ultra-high vacuum. These ribbons self-assemble in regular two-dimensional islands.</description><subject>Chemical Sciences</subject><subject>Crystal defects</subject><subject>Electrospraying</subject><subject>High vacuum</subject><subject>Ion beams</subject><subject>Molecular machines</subject><subject>Physics</subject><subject>Scanning tunneling microscopy</subject><subject>Silver</subject><issn>1359-7345</issn><issn>1364-548X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><recordid>eNpd0ctr3DAQB2ATWkia9NJ7wNDLJuBUo4ctHRdvXrBQShrITczqkXixV1vJDux_H203pFBdJGY-hDS_ovgG5AoIUz8sNYYwKmt7VJwAq3kluHz6tD8LVTWMi-PiS0prkhcIeVL8ehjjZMYpYl-ixe2IYxc2qQy-dL0zYwxpG3HnbIkxDLlpytB3zwGHzrrSh97i4GL2m3L-PAOAi7Pis8c-ua_v-2nxeHP9u72rlj9v79v5sjJM8rGyjfDU01VDVkDAS7BGSSkRqOLgGOG1WblGWse9QFAri04J8OicV17Vgp0WF4d7X7DX29gNGHc6YKfv5ku9rxFOG0EFf4VsZwe7jeHP5NKohy4Z1_e4cWFKmtYKGtkIwTP9_h9dhylu8k80bfZjY7JWWV0elMkDStH5jxcA0fsk9IK27d8kFhmfH3BM5sP9S4q9AXBUg-0</recordid><startdate>20220809</startdate><enddate>20220809</enddate><creator>Meier, Dennis</creator><creator>Schoof, Benedikt</creator><creator>Wang, Jinhua</creator><creator>Li, Xuesong</creator><creator>Walz, Andreas</creator><creator>Huettig, Annette</creator><creator>Schlichting, Hartmut</creator><creator>Rosu, Frédéric</creator><creator>Gabelica, Valérie</creator><creator>Maurizot, Victor</creator><creator>Reichert, Joachim</creator><creator>Papageorgiou, Anthoula C</creator><creator>Huc, Ivan</creator><creator>Barth, Johannes V</creator><general>Royal Society of Chemistry</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><scope>7X8</scope><scope>1XC</scope><scope>VOOES</scope><orcidid>https://orcid.org/0000-0003-3674-7539</orcidid><orcidid>https://orcid.org/0000-0003-1054-0097</orcidid><orcidid>https://orcid.org/0000-0001-7036-9696</orcidid><orcidid>https://orcid.org/0000-0003-4383-2889</orcidid><orcidid>https://orcid.org/0000-0001-6104-796X</orcidid><orcidid>https://orcid.org/0000-0001-9496-0165</orcidid></search><sort><creationdate>20220809</creationdate><title>Structural adaptations of electrosprayed aromatic oligoamide foldamers on Ag(111)</title><author>Meier, Dennis ; 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For many of these, defect free, 2D-crystaline monolayers are needed. To this end, submonolayers were prepared in ultra-high vacuum (UHV) on Ag(111)
via
electrospray controlled ion beam deposition (ES-CIBD). On the surface, the unfolded state is unambiguously identified by real-space single-molecule imaging using scanning tunnelling microscopy (STM) and it is found to assemble in regular structures.
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| ispartof | Chemical communications (Cambridge, England), 2022-08, Vol.58 (64), p.8938-8941 |
| issn | 1359-7345 1364-548X |
| language | eng |
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| source | Royal Society Of Chemistry Journals; Alma/SFX Local Collection |
| subjects | Chemical Sciences Crystal defects Electrospraying High vacuum Ion beams Molecular machines Physics Scanning tunneling microscopy Silver |
| title | Structural adaptations of electrosprayed aromatic oligoamide foldamers on Ag(111) |
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