Construction of MoO@MoS heterostructures on carbon cloth for the hydrogen evolution reaction
MoS 2 as one graphene-like 2D layered transition metal sulfide has attracted great attention. However, its application for the HER is still restricted by the poor electrical conductivity and structural restacking. In this work, we developed a facile method to prepare MoO 2 @MoS 2 heterostructures in...
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| Veröffentlicht in: | New journal of chemistry 2021-11, Vol.45 (42), p.19826-1983 |
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| container_end_page | 1983 |
|---|---|
| container_issue | 42 |
| container_start_page | 19826 |
| container_title | New journal of chemistry |
| container_volume | 45 |
| creator | Tian, Jingyang Yang, Chundi Liu, Zhirui Li, Funan He, Xiao Chen, Wei Xia, Nan Nan Lin, Chong |
| description | MoS
2
as one graphene-like 2D layered transition metal sulfide has attracted great attention. However, its application for the HER is still restricted by the poor electrical conductivity and structural restacking. In this work, we developed a facile method to prepare MoO
2
@MoS
2
heterostructures
in situ
by partial conversion of MoO
x
into MoS
2
on carbon cloth. Based on the two-time hydrothermal process, the MoS
2
nanosheets can be dispersed and grow on carbon cloth. Excellent electrochemical HER activity of MoO
2
@MoS
2
/CC-2 can be achieved with a low overpotential of 115 mV at 10 mA cm
−2
(
η
10
) in 0.5 M H
2
SO
4
. Furthermore, it still shows durable electrocatalytic stability for 13 h. The outstanding electrocatalytic activity may be ascribed to the synergistic effect between the MoO
2
and MoS
2
heterostructures.
MoO
2
@MoS
2
heterostructures
in situ
grown on carbon cloth were developed for efficient hydrogen evolution reaction. |
| doi_str_mv | 10.1039/d1nj04245a |
| format | Article |
| fullrecord | <record><control><sourceid>rsc</sourceid><recordid>TN_cdi_rsc_primary_d1nj04245a</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>d1nj04245a</sourcerecordid><originalsourceid>FETCH-rsc_primary_d1nj04245a3</originalsourceid><addsrcrecordid>eNqFjjsLwjAURoMo-FzchfyBam6bRroJoriIg45CiTU1ltorN6ngv_cJjk7ngwOHj7EhiDGIKJkcoSqEDGWsG6wDkUqCJFTQfG6QMhCxVG3Wda4QAmCqoMP2c6ycpzrzZ6w45nyNm9kat9wabwg_qibj-FNnmg4vlOgtz5G4t4bb-5HwZCpubljW7wwZ_e71WSvXpTODL3tstFzs5quAXJZe6XzRdE9_l6N__gHNpUYg</addsrcrecordid><sourcetype>Publisher</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype></control><display><type>article</type><title>Construction of MoO@MoS heterostructures on carbon cloth for the hydrogen evolution reaction</title><source>Royal Society Of Chemistry Journals 2008-</source><source>Alma/SFX Local Collection</source><creator>Tian, Jingyang ; Yang, Chundi ; Liu, Zhirui ; Li, Funan ; He, Xiao ; Chen, Wei ; Xia, Nan Nan ; Lin, Chong</creator><creatorcontrib>Tian, Jingyang ; Yang, Chundi ; Liu, Zhirui ; Li, Funan ; He, Xiao ; Chen, Wei ; Xia, Nan Nan ; Lin, Chong</creatorcontrib><description>MoS
2
as one graphene-like 2D layered transition metal sulfide has attracted great attention. However, its application for the HER is still restricted by the poor electrical conductivity and structural restacking. In this work, we developed a facile method to prepare MoO
2
@MoS
2
heterostructures
in situ
by partial conversion of MoO
x
into MoS
2
on carbon cloth. Based on the two-time hydrothermal process, the MoS
2
nanosheets can be dispersed and grow on carbon cloth. Excellent electrochemical HER activity of MoO
2
@MoS
2
/CC-2 can be achieved with a low overpotential of 115 mV at 10 mA cm
−2
(
η
10
) in 0.5 M H
2
SO
4
. Furthermore, it still shows durable electrocatalytic stability for 13 h. The outstanding electrocatalytic activity may be ascribed to the synergistic effect between the MoO
2
and MoS
2
heterostructures.
MoO
2
@MoS
2
heterostructures
in situ
grown on carbon cloth were developed for efficient hydrogen evolution reaction.</description><identifier>ISSN: 1144-0546</identifier><identifier>EISSN: 1369-9261</identifier><identifier>DOI: 10.1039/d1nj04245a</identifier><ispartof>New journal of chemistry, 2021-11, Vol.45 (42), p.19826-1983</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27923,27924</link.rule.ids></links><search><creatorcontrib>Tian, Jingyang</creatorcontrib><creatorcontrib>Yang, Chundi</creatorcontrib><creatorcontrib>Liu, Zhirui</creatorcontrib><creatorcontrib>Li, Funan</creatorcontrib><creatorcontrib>He, Xiao</creatorcontrib><creatorcontrib>Chen, Wei</creatorcontrib><creatorcontrib>Xia, Nan Nan</creatorcontrib><creatorcontrib>Lin, Chong</creatorcontrib><title>Construction of MoO@MoS heterostructures on carbon cloth for the hydrogen evolution reaction</title><title>New journal of chemistry</title><description>MoS
2
as one graphene-like 2D layered transition metal sulfide has attracted great attention. However, its application for the HER is still restricted by the poor electrical conductivity and structural restacking. In this work, we developed a facile method to prepare MoO
2
@MoS
2
heterostructures
in situ
by partial conversion of MoO
x
into MoS
2
on carbon cloth. Based on the two-time hydrothermal process, the MoS
2
nanosheets can be dispersed and grow on carbon cloth. Excellent electrochemical HER activity of MoO
2
@MoS
2
/CC-2 can be achieved with a low overpotential of 115 mV at 10 mA cm
−2
(
η
10
) in 0.5 M H
2
SO
4
. Furthermore, it still shows durable electrocatalytic stability for 13 h. The outstanding electrocatalytic activity may be ascribed to the synergistic effect between the MoO
2
and MoS
2
heterostructures.
MoO
2
@MoS
2
heterostructures
in situ
grown on carbon cloth were developed for efficient hydrogen evolution reaction.</description><issn>1144-0546</issn><issn>1369-9261</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><sourceid/><recordid>eNqFjjsLwjAURoMo-FzchfyBam6bRroJoriIg45CiTU1ltorN6ngv_cJjk7ngwOHj7EhiDGIKJkcoSqEDGWsG6wDkUqCJFTQfG6QMhCxVG3Wda4QAmCqoMP2c6ycpzrzZ6w45nyNm9kat9wabwg_qibj-FNnmg4vlOgtz5G4t4bb-5HwZCpubljW7wwZ_e71WSvXpTODL3tstFzs5quAXJZe6XzRdE9_l6N__gHNpUYg</recordid><startdate>20211101</startdate><enddate>20211101</enddate><creator>Tian, Jingyang</creator><creator>Yang, Chundi</creator><creator>Liu, Zhirui</creator><creator>Li, Funan</creator><creator>He, Xiao</creator><creator>Chen, Wei</creator><creator>Xia, Nan Nan</creator><creator>Lin, Chong</creator><scope/></search><sort><creationdate>20211101</creationdate><title>Construction of MoO@MoS heterostructures on carbon cloth for the hydrogen evolution reaction</title><author>Tian, Jingyang ; Yang, Chundi ; Liu, Zhirui ; Li, Funan ; He, Xiao ; Chen, Wei ; Xia, Nan Nan ; Lin, Chong</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-rsc_primary_d1nj04245a3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><creationdate>2021</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Tian, Jingyang</creatorcontrib><creatorcontrib>Yang, Chundi</creatorcontrib><creatorcontrib>Liu, Zhirui</creatorcontrib><creatorcontrib>Li, Funan</creatorcontrib><creatorcontrib>He, Xiao</creatorcontrib><creatorcontrib>Chen, Wei</creatorcontrib><creatorcontrib>Xia, Nan Nan</creatorcontrib><creatorcontrib>Lin, Chong</creatorcontrib><jtitle>New journal of chemistry</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Tian, Jingyang</au><au>Yang, Chundi</au><au>Liu, Zhirui</au><au>Li, Funan</au><au>He, Xiao</au><au>Chen, Wei</au><au>Xia, Nan Nan</au><au>Lin, Chong</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Construction of MoO@MoS heterostructures on carbon cloth for the hydrogen evolution reaction</atitle><jtitle>New journal of chemistry</jtitle><date>2021-11-01</date><risdate>2021</risdate><volume>45</volume><issue>42</issue><spage>19826</spage><epage>1983</epage><pages>19826-1983</pages><issn>1144-0546</issn><eissn>1369-9261</eissn><abstract>MoS
2
as one graphene-like 2D layered transition metal sulfide has attracted great attention. However, its application for the HER is still restricted by the poor electrical conductivity and structural restacking. In this work, we developed a facile method to prepare MoO
2
@MoS
2
heterostructures
in situ
by partial conversion of MoO
x
into MoS
2
on carbon cloth. Based on the two-time hydrothermal process, the MoS
2
nanosheets can be dispersed and grow on carbon cloth. Excellent electrochemical HER activity of MoO
2
@MoS
2
/CC-2 can be achieved with a low overpotential of 115 mV at 10 mA cm
−2
(
η
10
) in 0.5 M H
2
SO
4
. Furthermore, it still shows durable electrocatalytic stability for 13 h. The outstanding electrocatalytic activity may be ascribed to the synergistic effect between the MoO
2
and MoS
2
heterostructures.
MoO
2
@MoS
2
heterostructures
in situ
grown on carbon cloth were developed for efficient hydrogen evolution reaction.</abstract><doi>10.1039/d1nj04245a</doi><tpages>5</tpages></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 1144-0546 |
| ispartof | New journal of chemistry, 2021-11, Vol.45 (42), p.19826-1983 |
| issn | 1144-0546 1369-9261 |
| language | |
| recordid | cdi_rsc_primary_d1nj04245a |
| source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| title | Construction of MoO@MoS heterostructures on carbon cloth for the hydrogen evolution reaction |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-12T01%3A50%3A44IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-rsc&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Construction%20of%20MoO@MoS%20heterostructures%20on%20carbon%20cloth%20for%20the%20hydrogen%20evolution%20reaction&rft.jtitle=New%20journal%20of%20chemistry&rft.au=Tian,%20Jingyang&rft.date=2021-11-01&rft.volume=45&rft.issue=42&rft.spage=19826&rft.epage=1983&rft.pages=19826-1983&rft.issn=1144-0546&rft.eissn=1369-9261&rft_id=info:doi/10.1039/d1nj04245a&rft_dat=%3Crsc%3Ed1nj04245a%3C/rsc%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_id=info:pmid/&rfr_iscdi=true |