Constructing a new polymer acceptor enabled non-halogenated solvent-processed all-polymer solar cell with an efficiency of 13.8
A new polymer acceptor, PS1 , was developed by connecting the non-fullerene acceptor building block of dithienothiophen[3,2- b ]pyrrolobenzotriazole capped with 3-(dicyanomethylidene)-indan-1-one through a thiophene spacer. The solubilizing alkyl side groups in the central unit enabled PS1 to be rea...
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| Veröffentlicht in: | Chemical communications (Cambridge, England) England), 2021-01, Vol.57 (7), p.935-938 |
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| container_title | Chemical communications (Cambridge, England) |
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| creator | Zhu, Chunguang Li, Zhenye Zhong, Wenkai Peng, Feng Zeng, Zhaomiyi Ying, Lei Huang, Fei Cao, Yong |
| description | A new polymer acceptor,
PS1
, was developed by connecting the non-fullerene acceptor building block of dithienothiophen[3,2-
b
]pyrrolobenzotriazole capped with 3-(dicyanomethylidene)-indan-1-one through a thiophene spacer. The solubilizing alkyl side groups in the central unit enabled
PS1
to be readily dissolved in non-chlorinated solvents. By using 2-methyltetrahydrofuran as the processing solvent, the all-polymer solar cell (all-PSC) containing
PS1
and a polymer donor PTzBI-oF in the light-harvesting layer exhibited an impressively high power conversion efficiency of 13.8%.
The new polymer donor
PS1
can be easily dissolved in a non-chlorinated solvent, and it exhibited a remarkable PCE when processed with 2-methyltetrahydrofuran. |
| doi_str_mv | 10.1039/d0cc07213c |
| format | Article |
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PS1
, was developed by connecting the non-fullerene acceptor building block of dithienothiophen[3,2-
b
]pyrrolobenzotriazole capped with 3-(dicyanomethylidene)-indan-1-one through a thiophene spacer. The solubilizing alkyl side groups in the central unit enabled
PS1
to be readily dissolved in non-chlorinated solvents. By using 2-methyltetrahydrofuran as the processing solvent, the all-polymer solar cell (all-PSC) containing
PS1
and a polymer donor PTzBI-oF in the light-harvesting layer exhibited an impressively high power conversion efficiency of 13.8%.
The new polymer donor
PS1
can be easily dissolved in a non-chlorinated solvent, and it exhibited a remarkable PCE when processed with 2-methyltetrahydrofuran.</description><identifier>ISSN: 1359-7345</identifier><identifier>EISSN: 1364-548X</identifier><identifier>DOI: 10.1039/d0cc07213c</identifier><identifier>PMID: 33398311</identifier><language>eng</language><publisher>England: Royal Society of Chemistry</publisher><subject>Energy conversion efficiency ; Fullerenes ; Halogenation ; Photovoltaic cells ; Polymers ; Solar cells ; Solvents</subject><ispartof>Chemical communications (Cambridge, England), 2021-01, Vol.57 (7), p.935-938</ispartof><rights>Copyright Royal Society of Chemistry 2021</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c337t-c527183afb2196be1d8b3e3bc4e11182b7905cb0ba7e252ccd7af6e2a9269cd33</citedby><cites>FETCH-LOGICAL-c337t-c527183afb2196be1d8b3e3bc4e11182b7905cb0ba7e252ccd7af6e2a9269cd33</cites><orcidid>0000-0003-1137-2355 ; 0000-0001-9665-6642</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27922,27923</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/33398311$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Zhu, Chunguang</creatorcontrib><creatorcontrib>Li, Zhenye</creatorcontrib><creatorcontrib>Zhong, Wenkai</creatorcontrib><creatorcontrib>Peng, Feng</creatorcontrib><creatorcontrib>Zeng, Zhaomiyi</creatorcontrib><creatorcontrib>Ying, Lei</creatorcontrib><creatorcontrib>Huang, Fei</creatorcontrib><creatorcontrib>Cao, Yong</creatorcontrib><title>Constructing a new polymer acceptor enabled non-halogenated solvent-processed all-polymer solar cell with an efficiency of 13.8</title><title>Chemical communications (Cambridge, England)</title><addtitle>Chem Commun (Camb)</addtitle><description>A new polymer acceptor,
PS1
, was developed by connecting the non-fullerene acceptor building block of dithienothiophen[3,2-
b
]pyrrolobenzotriazole capped with 3-(dicyanomethylidene)-indan-1-one through a thiophene spacer. The solubilizing alkyl side groups in the central unit enabled
PS1
to be readily dissolved in non-chlorinated solvents. By using 2-methyltetrahydrofuran as the processing solvent, the all-polymer solar cell (all-PSC) containing
PS1
and a polymer donor PTzBI-oF in the light-harvesting layer exhibited an impressively high power conversion efficiency of 13.8%.
The new polymer donor
PS1
can be easily dissolved in a non-chlorinated solvent, and it exhibited a remarkable PCE when processed with 2-methyltetrahydrofuran.</description><subject>Energy conversion efficiency</subject><subject>Fullerenes</subject><subject>Halogenation</subject><subject>Photovoltaic cells</subject><subject>Polymers</subject><subject>Solar cells</subject><subject>Solvents</subject><issn>1359-7345</issn><issn>1364-548X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><recordid>eNpdkUFv1DAQhS0Eou3ChTvIEheElGJ7kjg-okABqRIXkLhF9mTSpvLai51Q7Ym_jpdti4Qv9sx88_Tkx9gLKc6lAPNuFIhCKwn4iJ1KaOuqqbsfjw_vxlQa6uaEneV8I8qRTfeUnQCA6UDKU_a7jyEvacVlDlfc8kC3fBf9fkuJW0TaLTFxCtZ5GnmIobq2Pl6VxlLqHP0vCku1SxEp59Kx3lf362VqE0fynt_OyzW3gdM0zThTwD2PE5dw3j1jTybrMz2_uzfs-8XHb_3n6vLrpy_9-8sKAfRSYaO07MBOTknTOpJj54DAYU1Syk45bUSDTjirSTUKcdR2aklZo1qDI8CGvTnqFq8_V8rLsJ3zwZsNFNc8qFo3YLQuH7phr_9Db-KaQnFXqE62rRLmQL09UphizommYZfmrU37QYrhEMvwQfT931j6Ar-6k1zdlsYH9D6HArw8Ainjw_RfrvAHuBeSrw</recordid><startdate>20210128</startdate><enddate>20210128</enddate><creator>Zhu, Chunguang</creator><creator>Li, Zhenye</creator><creator>Zhong, Wenkai</creator><creator>Peng, Feng</creator><creator>Zeng, Zhaomiyi</creator><creator>Ying, Lei</creator><creator>Huang, Fei</creator><creator>Cao, Yong</creator><general>Royal Society of Chemistry</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0003-1137-2355</orcidid><orcidid>https://orcid.org/0000-0001-9665-6642</orcidid></search><sort><creationdate>20210128</creationdate><title>Constructing a new polymer acceptor enabled non-halogenated solvent-processed all-polymer solar cell with an efficiency of 13.8</title><author>Zhu, Chunguang ; Li, Zhenye ; Zhong, Wenkai ; Peng, Feng ; Zeng, Zhaomiyi ; Ying, Lei ; Huang, Fei ; Cao, Yong</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c337t-c527183afb2196be1d8b3e3bc4e11182b7905cb0ba7e252ccd7af6e2a9269cd33</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>Energy conversion efficiency</topic><topic>Fullerenes</topic><topic>Halogenation</topic><topic>Photovoltaic cells</topic><topic>Polymers</topic><topic>Solar cells</topic><topic>Solvents</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhu, Chunguang</creatorcontrib><creatorcontrib>Li, Zhenye</creatorcontrib><creatorcontrib>Zhong, Wenkai</creatorcontrib><creatorcontrib>Peng, Feng</creatorcontrib><creatorcontrib>Zeng, Zhaomiyi</creatorcontrib><creatorcontrib>Ying, Lei</creatorcontrib><creatorcontrib>Huang, Fei</creatorcontrib><creatorcontrib>Cao, Yong</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>Chemical communications (Cambridge, England)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zhu, Chunguang</au><au>Li, Zhenye</au><au>Zhong, Wenkai</au><au>Peng, Feng</au><au>Zeng, Zhaomiyi</au><au>Ying, Lei</au><au>Huang, Fei</au><au>Cao, Yong</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Constructing a new polymer acceptor enabled non-halogenated solvent-processed all-polymer solar cell with an efficiency of 13.8</atitle><jtitle>Chemical communications (Cambridge, England)</jtitle><addtitle>Chem Commun (Camb)</addtitle><date>2021-01-28</date><risdate>2021</risdate><volume>57</volume><issue>7</issue><spage>935</spage><epage>938</epage><pages>935-938</pages><issn>1359-7345</issn><eissn>1364-548X</eissn><abstract>A new polymer acceptor,
PS1
, was developed by connecting the non-fullerene acceptor building block of dithienothiophen[3,2-
b
]pyrrolobenzotriazole capped with 3-(dicyanomethylidene)-indan-1-one through a thiophene spacer. The solubilizing alkyl side groups in the central unit enabled
PS1
to be readily dissolved in non-chlorinated solvents. By using 2-methyltetrahydrofuran as the processing solvent, the all-polymer solar cell (all-PSC) containing
PS1
and a polymer donor PTzBI-oF in the light-harvesting layer exhibited an impressively high power conversion efficiency of 13.8%.
The new polymer donor
PS1
can be easily dissolved in a non-chlorinated solvent, and it exhibited a remarkable PCE when processed with 2-methyltetrahydrofuran.</abstract><cop>England</cop><pub>Royal Society of Chemistry</pub><pmid>33398311</pmid><doi>10.1039/d0cc07213c</doi><tpages>4</tpages><orcidid>https://orcid.org/0000-0003-1137-2355</orcidid><orcidid>https://orcid.org/0000-0001-9665-6642</orcidid></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 1359-7345 |
| ispartof | Chemical communications (Cambridge, England), 2021-01, Vol.57 (7), p.935-938 |
| issn | 1359-7345 1364-548X |
| language | eng |
| recordid | cdi_rsc_primary_d0cc07213c |
| source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| subjects | Energy conversion efficiency Fullerenes Halogenation Photovoltaic cells Polymers Solar cells Solvents |
| title | Constructing a new polymer acceptor enabled non-halogenated solvent-processed all-polymer solar cell with an efficiency of 13.8 |
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