Magnetic functional heterojunction reactors with 3D specific recognition for selective photocatalysis and synergistic photodegradation in binary antibiotic solutions
We report on the development of the emerging magnetic functional heterojunction reactors with three-dimensional (3D) specific recognition. Upon synthesis via surface imprinting and visible light-induced polymerization, the developed magnetic functional heterojunction reactors not only possess the em...
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| Veröffentlicht in: | Journal of materials chemistry. A, Materials for energy and sustainability Materials for energy and sustainability, 2019, Vol.7 (23), p.13986-14 |
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| container_title | Journal of materials chemistry. A, Materials for energy and sustainability |
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| creator | Lu, Ziyang Zhou, Guosheng Song, Minshan Wang, Dandan Huo, Pengwei Fan, Weiqiang Dong, Hongjun Tang, Hua Yan, Feng Xing, Guozhong |
| description | We report on the development of the emerging magnetic functional heterojunction reactors with three-dimensional (3D) specific recognition. Upon synthesis
via
surface imprinting and visible light-induced polymerization, the developed magnetic functional heterojunction reactors not only possess the emblematic conductive polymer POPD, but they are also equipped with the imprinted cavities in the corresponding 3D specific recognition outer layer. Our experimental data show that POPD forms a heterojunction with TiO
2
and remarkably enhances the photocatalytic activity. Owing to the presence of imprinted cavities, the magnetic functional heterojunction reactors exhibit excellent 3D specific recognition and selective degradation of danofloxacin mesylate in a binary antibiotic solution. Importantly, through in-depth understanding of the mechanism and systematic experiments, the electron transfer mode, 3D specific recognition mode, selective photodegradation mode and photodegradation pathways are methodically discussed and thoroughly illustrated. The present study demonstrates that the 3D specific recognition can be utilized to selectively degrade a specific organic pollutant in a variety of practical environmental protection applications.
Magnetic functional heterojunction reactors, containing a 3D specific recognition layer and TiO
2
-POPD heterojunction, improve the selectivity and photocatalytic activity. |
| doi_str_mv | 10.1039/c9ta01863h |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_rsc_p</sourceid><recordid>TN_cdi_rsc_primary_c9ta01863h</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2238514282</sourcerecordid><originalsourceid>FETCH-LOGICAL-c344t-a2d674005a85b992492ee4bd1a3682bf721836fcb99bd6a189ceaaafdbf9bc633</originalsourceid><addsrcrecordid>eNp9kU1PAyEURSdGExt1494E486kysB0CktTP2qicaPryRvm0dKMw8ijmv4g_6f0I7qTDYRzLhBulp3m_CrnUl8bHYHnqpTzvWwg-IgPx4Uu93_XSh1mJ0QLnobivNR6kH0_w6zD6Ayzy85E5zto2RwjBr_YbbCAYKIPxL5cnDN5y6hH42zKBDR-1rmNZX1ghC2mzCeyfu6jNxChXZEjBl3DaNVhmDlaX7bBDc4CNLBJu47VroOwSmp0tfNri3y7XFM6zg4stIQnu_koe7u_e51Mh08vD4-Tm6ehkUURhyCaclxwPgI1qrUWhRaIRd3kIEslajsWuZKlNYnVTQm50gYBwDa11bUppTzKLrbn9sF_LJFitfDLkL6EKiGkGuWFUCJZl1vLBE8U0FZ9cO_p7VXOq3UT1US_3myamCb5bCsHMr_eX1OJn__Hq76x8gfiE5cN</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2238514282</pqid></control><display><type>article</type><title>Magnetic functional heterojunction reactors with 3D specific recognition for selective photocatalysis and synergistic photodegradation in binary antibiotic solutions</title><source>Royal Society Of Chemistry Journals 2008-</source><creator>Lu, Ziyang ; Zhou, Guosheng ; Song, Minshan ; Wang, Dandan ; Huo, Pengwei ; Fan, Weiqiang ; Dong, Hongjun ; Tang, Hua ; Yan, Feng ; Xing, Guozhong</creator><creatorcontrib>Lu, Ziyang ; Zhou, Guosheng ; Song, Minshan ; Wang, Dandan ; Huo, Pengwei ; Fan, Weiqiang ; Dong, Hongjun ; Tang, Hua ; Yan, Feng ; Xing, Guozhong</creatorcontrib><description>We report on the development of the emerging magnetic functional heterojunction reactors with three-dimensional (3D) specific recognition. Upon synthesis
via
surface imprinting and visible light-induced polymerization, the developed magnetic functional heterojunction reactors not only possess the emblematic conductive polymer POPD, but they are also equipped with the imprinted cavities in the corresponding 3D specific recognition outer layer. Our experimental data show that POPD forms a heterojunction with TiO
2
and remarkably enhances the photocatalytic activity. Owing to the presence of imprinted cavities, the magnetic functional heterojunction reactors exhibit excellent 3D specific recognition and selective degradation of danofloxacin mesylate in a binary antibiotic solution. Importantly, through in-depth understanding of the mechanism and systematic experiments, the electron transfer mode, 3D specific recognition mode, selective photodegradation mode and photodegradation pathways are methodically discussed and thoroughly illustrated. The present study demonstrates that the 3D specific recognition can be utilized to selectively degrade a specific organic pollutant in a variety of practical environmental protection applications.
Magnetic functional heterojunction reactors, containing a 3D specific recognition layer and TiO
2
-POPD heterojunction, improve the selectivity and photocatalytic activity.</description><identifier>ISSN: 2050-7488</identifier><identifier>EISSN: 2050-7496</identifier><identifier>DOI: 10.1039/c9ta01863h</identifier><language>eng</language><publisher>Cambridge: Royal Society of Chemistry</publisher><subject>Antibiotics ; Biodegradation ; Catalytic activity ; Cavities ; Electron transfer ; Environmental protection ; Heterojunctions ; Iron oxides ; Light effects ; Mapping ; Photocatalysis ; Photodegradation ; Pollutants ; Polymerization ; Reactors ; Recognition ; Selectivity ; Titanium dioxide ; Wavelengths ; X ray photoelectron spectroscopy</subject><ispartof>Journal of materials chemistry. A, Materials for energy and sustainability, 2019, Vol.7 (23), p.13986-14</ispartof><rights>Copyright Royal Society of Chemistry 2019</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c344t-a2d674005a85b992492ee4bd1a3682bf721836fcb99bd6a189ceaaafdbf9bc633</citedby><cites>FETCH-LOGICAL-c344t-a2d674005a85b992492ee4bd1a3682bf721836fcb99bd6a189ceaaafdbf9bc633</cites><orcidid>0000-0001-8873-3695 ; 0000-0002-5387-1542 ; 0000-0002-4171-1015</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,4014,27914,27915,27916</link.rule.ids></links><search><creatorcontrib>Lu, Ziyang</creatorcontrib><creatorcontrib>Zhou, Guosheng</creatorcontrib><creatorcontrib>Song, Minshan</creatorcontrib><creatorcontrib>Wang, Dandan</creatorcontrib><creatorcontrib>Huo, Pengwei</creatorcontrib><creatorcontrib>Fan, Weiqiang</creatorcontrib><creatorcontrib>Dong, Hongjun</creatorcontrib><creatorcontrib>Tang, Hua</creatorcontrib><creatorcontrib>Yan, Feng</creatorcontrib><creatorcontrib>Xing, Guozhong</creatorcontrib><title>Magnetic functional heterojunction reactors with 3D specific recognition for selective photocatalysis and synergistic photodegradation in binary antibiotic solutions</title><title>Journal of materials chemistry. A, Materials for energy and sustainability</title><description>We report on the development of the emerging magnetic functional heterojunction reactors with three-dimensional (3D) specific recognition. Upon synthesis
via
surface imprinting and visible light-induced polymerization, the developed magnetic functional heterojunction reactors not only possess the emblematic conductive polymer POPD, but they are also equipped with the imprinted cavities in the corresponding 3D specific recognition outer layer. Our experimental data show that POPD forms a heterojunction with TiO
2
and remarkably enhances the photocatalytic activity. Owing to the presence of imprinted cavities, the magnetic functional heterojunction reactors exhibit excellent 3D specific recognition and selective degradation of danofloxacin mesylate in a binary antibiotic solution. Importantly, through in-depth understanding of the mechanism and systematic experiments, the electron transfer mode, 3D specific recognition mode, selective photodegradation mode and photodegradation pathways are methodically discussed and thoroughly illustrated. The present study demonstrates that the 3D specific recognition can be utilized to selectively degrade a specific organic pollutant in a variety of practical environmental protection applications.
Magnetic functional heterojunction reactors, containing a 3D specific recognition layer and TiO
2
-POPD heterojunction, improve the selectivity and photocatalytic activity.</description><subject>Antibiotics</subject><subject>Biodegradation</subject><subject>Catalytic activity</subject><subject>Cavities</subject><subject>Electron transfer</subject><subject>Environmental protection</subject><subject>Heterojunctions</subject><subject>Iron oxides</subject><subject>Light effects</subject><subject>Mapping</subject><subject>Photocatalysis</subject><subject>Photodegradation</subject><subject>Pollutants</subject><subject>Polymerization</subject><subject>Reactors</subject><subject>Recognition</subject><subject>Selectivity</subject><subject>Titanium dioxide</subject><subject>Wavelengths</subject><subject>X ray photoelectron spectroscopy</subject><issn>2050-7488</issn><issn>2050-7496</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNp9kU1PAyEURSdGExt1494E486kysB0CktTP2qicaPryRvm0dKMw8ijmv4g_6f0I7qTDYRzLhBulp3m_CrnUl8bHYHnqpTzvWwg-IgPx4Uu93_XSh1mJ0QLnobivNR6kH0_w6zD6Ayzy85E5zto2RwjBr_YbbCAYKIPxL5cnDN5y6hH42zKBDR-1rmNZX1ghC2mzCeyfu6jNxChXZEjBl3DaNVhmDlaX7bBDc4CNLBJu47VroOwSmp0tfNri3y7XFM6zg4stIQnu_koe7u_e51Mh08vD4-Tm6ehkUURhyCaclxwPgI1qrUWhRaIRd3kIEslajsWuZKlNYnVTQm50gYBwDa11bUppTzKLrbn9sF_LJFitfDLkL6EKiGkGuWFUCJZl1vLBE8U0FZ9cO_p7VXOq3UT1US_3myamCb5bCsHMr_eX1OJn__Hq76x8gfiE5cN</recordid><startdate>2019</startdate><enddate>2019</enddate><creator>Lu, Ziyang</creator><creator>Zhou, Guosheng</creator><creator>Song, Minshan</creator><creator>Wang, Dandan</creator><creator>Huo, Pengwei</creator><creator>Fan, Weiqiang</creator><creator>Dong, Hongjun</creator><creator>Tang, Hua</creator><creator>Yan, Feng</creator><creator>Xing, Guozhong</creator><general>Royal Society of Chemistry</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7SR</scope><scope>7ST</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>C1K</scope><scope>JG9</scope><scope>L7M</scope><scope>SOI</scope><orcidid>https://orcid.org/0000-0001-8873-3695</orcidid><orcidid>https://orcid.org/0000-0002-5387-1542</orcidid><orcidid>https://orcid.org/0000-0002-4171-1015</orcidid></search><sort><creationdate>2019</creationdate><title>Magnetic functional heterojunction reactors with 3D specific recognition for selective photocatalysis and synergistic photodegradation in binary antibiotic solutions</title><author>Lu, Ziyang ; Zhou, Guosheng ; Song, Minshan ; Wang, Dandan ; Huo, Pengwei ; Fan, Weiqiang ; Dong, Hongjun ; Tang, Hua ; Yan, Feng ; Xing, Guozhong</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c344t-a2d674005a85b992492ee4bd1a3682bf721836fcb99bd6a189ceaaafdbf9bc633</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Antibiotics</topic><topic>Biodegradation</topic><topic>Catalytic activity</topic><topic>Cavities</topic><topic>Electron transfer</topic><topic>Environmental protection</topic><topic>Heterojunctions</topic><topic>Iron oxides</topic><topic>Light effects</topic><topic>Mapping</topic><topic>Photocatalysis</topic><topic>Photodegradation</topic><topic>Pollutants</topic><topic>Polymerization</topic><topic>Reactors</topic><topic>Recognition</topic><topic>Selectivity</topic><topic>Titanium dioxide</topic><topic>Wavelengths</topic><topic>X ray photoelectron spectroscopy</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Lu, Ziyang</creatorcontrib><creatorcontrib>Zhou, Guosheng</creatorcontrib><creatorcontrib>Song, Minshan</creatorcontrib><creatorcontrib>Wang, Dandan</creatorcontrib><creatorcontrib>Huo, Pengwei</creatorcontrib><creatorcontrib>Fan, Weiqiang</creatorcontrib><creatorcontrib>Dong, Hongjun</creatorcontrib><creatorcontrib>Tang, Hua</creatorcontrib><creatorcontrib>Yan, Feng</creatorcontrib><creatorcontrib>Xing, Guozhong</creatorcontrib><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>Environment Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Environment Abstracts</collection><jtitle>Journal of materials chemistry. A, Materials for energy and sustainability</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Lu, Ziyang</au><au>Zhou, Guosheng</au><au>Song, Minshan</au><au>Wang, Dandan</au><au>Huo, Pengwei</au><au>Fan, Weiqiang</au><au>Dong, Hongjun</au><au>Tang, Hua</au><au>Yan, Feng</au><au>Xing, Guozhong</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Magnetic functional heterojunction reactors with 3D specific recognition for selective photocatalysis and synergistic photodegradation in binary antibiotic solutions</atitle><jtitle>Journal of materials chemistry. A, Materials for energy and sustainability</jtitle><date>2019</date><risdate>2019</risdate><volume>7</volume><issue>23</issue><spage>13986</spage><epage>14</epage><pages>13986-14</pages><issn>2050-7488</issn><eissn>2050-7496</eissn><abstract>We report on the development of the emerging magnetic functional heterojunction reactors with three-dimensional (3D) specific recognition. Upon synthesis
via
surface imprinting and visible light-induced polymerization, the developed magnetic functional heterojunction reactors not only possess the emblematic conductive polymer POPD, but they are also equipped with the imprinted cavities in the corresponding 3D specific recognition outer layer. Our experimental data show that POPD forms a heterojunction with TiO
2
and remarkably enhances the photocatalytic activity. Owing to the presence of imprinted cavities, the magnetic functional heterojunction reactors exhibit excellent 3D specific recognition and selective degradation of danofloxacin mesylate in a binary antibiotic solution. Importantly, through in-depth understanding of the mechanism and systematic experiments, the electron transfer mode, 3D specific recognition mode, selective photodegradation mode and photodegradation pathways are methodically discussed and thoroughly illustrated. The present study demonstrates that the 3D specific recognition can be utilized to selectively degrade a specific organic pollutant in a variety of practical environmental protection applications.
Magnetic functional heterojunction reactors, containing a 3D specific recognition layer and TiO
2
-POPD heterojunction, improve the selectivity and photocatalytic activity.</abstract><cop>Cambridge</cop><pub>Royal Society of Chemistry</pub><doi>10.1039/c9ta01863h</doi><tpages>15</tpages><orcidid>https://orcid.org/0000-0001-8873-3695</orcidid><orcidid>https://orcid.org/0000-0002-5387-1542</orcidid><orcidid>https://orcid.org/0000-0002-4171-1015</orcidid></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 2050-7488 |
| ispartof | Journal of materials chemistry. A, Materials for energy and sustainability, 2019, Vol.7 (23), p.13986-14 |
| issn | 2050-7488 2050-7496 |
| language | eng |
| recordid | cdi_rsc_primary_c9ta01863h |
| source | Royal Society Of Chemistry Journals 2008- |
| subjects | Antibiotics Biodegradation Catalytic activity Cavities Electron transfer Environmental protection Heterojunctions Iron oxides Light effects Mapping Photocatalysis Photodegradation Pollutants Polymerization Reactors Recognition Selectivity Titanium dioxide Wavelengths X ray photoelectron spectroscopy |
| title | Magnetic functional heterojunction reactors with 3D specific recognition for selective photocatalysis and synergistic photodegradation in binary antibiotic solutions |
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