Photocatalytic production of hydrogen peroxide through selective two-electron reduction of dioxygen utilizing amine-functionalized MIL-125 deposited with nickel oxide nanoparticles
Photocatalytic H 2 O 2 production via two-electron reduction of O 2 was realized by visible-light irradiation of a metal-organic framework, MIL-125-NH 2 , in the presence of TEOA and benzylalcohol. Deposition of NiO nanoparticles onto MIL-125-NH 2 dramatically enhanced the catalytic activity. Furthe...
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| Veröffentlicht in: | Chemical communications (Cambridge, England) England), 2018, Vol.54 (67), p.927-9273 |
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| container_issue | 67 |
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| container_title | Chemical communications (Cambridge, England) |
| container_volume | 54 |
| creator | Isaka, Yusuke Kondo, Yoshifumi Kawase, Yudai Kuwahara, Yasutaka Mori, Kohsuke Yamashita, Hiromi |
| description | Photocatalytic H
2
O
2
production
via
two-electron reduction of O
2
was realized by visible-light irradiation of a metal-organic framework, MIL-125-NH
2
, in the presence of TEOA and benzylalcohol. Deposition of NiO nanoparticles onto MIL-125-NH
2
dramatically enhanced the catalytic activity. Further studies suggested that fast disproportionation of the O
2
&z.rad;
−
intermediate to H
2
O
2
resulted in the enhancement.
Photocatalytic H
2
O
2
production
via
two-electron reduction of O
2
is realized by visible-light irradiation of a Ti-based metal-organic framework, MIL-125-NH
2
. |
| doi_str_mv | 10.1039/c8cc02679c |
| format | Article |
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2
O
2
production
via
two-electron reduction of O
2
was realized by visible-light irradiation of a metal-organic framework, MIL-125-NH
2
, in the presence of TEOA and benzylalcohol. Deposition of NiO nanoparticles onto MIL-125-NH
2
dramatically enhanced the catalytic activity. Further studies suggested that fast disproportionation of the O
2
&z.rad;
−
intermediate to H
2
O
2
resulted in the enhancement.
Photocatalytic H
2
O
2
production
via
two-electron reduction of O
2
is realized by visible-light irradiation of a Ti-based metal-organic framework, MIL-125-NH
2
.</description><identifier>ISSN: 1359-7345</identifier><identifier>EISSN: 1364-548X</identifier><identifier>DOI: 10.1039/c8cc02679c</identifier><identifier>PMID: 29993052</identifier><language>eng</language><publisher>England: Royal Society of Chemistry</publisher><subject>Catalysis ; Catalytic activity ; Disproportionation ; Hydrogen peroxide ; Hydrogen production ; Light irradiation ; Metal-organic frameworks ; Nanoparticles ; Nickel oxides ; Reduction</subject><ispartof>Chemical communications (Cambridge, England), 2018, Vol.54 (67), p.927-9273</ispartof><rights>Copyright Royal Society of Chemistry 2018</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c337t-103df6e6e88f0a8e33c2e84d5da2c9ca799c8ae06a5b86b49cd95a590ff3ca393</citedby><cites>FETCH-LOGICAL-c337t-103df6e6e88f0a8e33c2e84d5da2c9ca799c8ae06a5b86b49cd95a590ff3ca393</cites><orcidid>0000-0003-1796-5776 ; 0000-0002-5867-6463 ; 0000-0003-3915-4528</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,4024,27923,27924,27925</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/29993052$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Isaka, Yusuke</creatorcontrib><creatorcontrib>Kondo, Yoshifumi</creatorcontrib><creatorcontrib>Kawase, Yudai</creatorcontrib><creatorcontrib>Kuwahara, Yasutaka</creatorcontrib><creatorcontrib>Mori, Kohsuke</creatorcontrib><creatorcontrib>Yamashita, Hiromi</creatorcontrib><title>Photocatalytic production of hydrogen peroxide through selective two-electron reduction of dioxygen utilizing amine-functionalized MIL-125 deposited with nickel oxide nanoparticles</title><title>Chemical communications (Cambridge, England)</title><addtitle>Chem Commun (Camb)</addtitle><description>Photocatalytic H
2
O
2
production
via
two-electron reduction of O
2
was realized by visible-light irradiation of a metal-organic framework, MIL-125-NH
2
, in the presence of TEOA and benzylalcohol. Deposition of NiO nanoparticles onto MIL-125-NH
2
dramatically enhanced the catalytic activity. Further studies suggested that fast disproportionation of the O
2
&z.rad;
−
intermediate to H
2
O
2
resulted in the enhancement.
Photocatalytic H
2
O
2
production
via
two-electron reduction of O
2
is realized by visible-light irradiation of a Ti-based metal-organic framework, MIL-125-NH
2
.</description><subject>Catalysis</subject><subject>Catalytic activity</subject><subject>Disproportionation</subject><subject>Hydrogen peroxide</subject><subject>Hydrogen production</subject><subject>Light irradiation</subject><subject>Metal-organic frameworks</subject><subject>Nanoparticles</subject><subject>Nickel oxides</subject><subject>Reduction</subject><issn>1359-7345</issn><issn>1364-548X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><recordid>eNpdksFu1DAQhi1ERUvhwh1kiUtVKeDEcWIfUUSh0lblABK3yDuebFyycbAd2uW5eECc3VIQvtjz-_vH9owJeZGzNznj6i1IAFZUtYJH5CTnVZmJUn59vKyFympeimPyNIQblkYu5BNyXCilOBPFCfn1qXfRgY562EULdPLOzBCtG6nraL8z3m1wpBN6d2cN0th7N296GnDAhP1Iyq3L9oFPHo__uI11d7vFPUc72J923FC9tSNm3TzuIZ1UNPTqcpXlhaAGJxdsTMqtjT0dLXzDgR7OHfXoJu3TFQcMz8hRp4eAz-_nU_Ll4v3n5mO2uv5w2bxbZcB5HbNUHNNVWKGUHdMSOYcCZWmE0QUo0LVSIDWySou1rNalAqOEFop1HQfNFT8lZ4e8qSrfZwyx3doAOAx6RDeHtmCV5CUvS5bQ1_-hN2726YULJWVV16xYqPMDBd6F4LFrJ2-32u_anLVLL9tGNs2-l02CX92nnNdbNA_on-Yl4OUB8AEedv9-Bv4bwnGpFw</recordid><startdate>2018</startdate><enddate>2018</enddate><creator>Isaka, Yusuke</creator><creator>Kondo, Yoshifumi</creator><creator>Kawase, Yudai</creator><creator>Kuwahara, Yasutaka</creator><creator>Mori, Kohsuke</creator><creator>Yamashita, Hiromi</creator><general>Royal Society of Chemistry</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0003-1796-5776</orcidid><orcidid>https://orcid.org/0000-0002-5867-6463</orcidid><orcidid>https://orcid.org/0000-0003-3915-4528</orcidid></search><sort><creationdate>2018</creationdate><title>Photocatalytic production of hydrogen peroxide through selective two-electron reduction of dioxygen utilizing amine-functionalized MIL-125 deposited with nickel oxide nanoparticles</title><author>Isaka, Yusuke ; Kondo, Yoshifumi ; Kawase, Yudai ; Kuwahara, Yasutaka ; Mori, Kohsuke ; Yamashita, Hiromi</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c337t-103df6e6e88f0a8e33c2e84d5da2c9ca799c8ae06a5b86b49cd95a590ff3ca393</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2018</creationdate><topic>Catalysis</topic><topic>Catalytic activity</topic><topic>Disproportionation</topic><topic>Hydrogen peroxide</topic><topic>Hydrogen production</topic><topic>Light irradiation</topic><topic>Metal-organic frameworks</topic><topic>Nanoparticles</topic><topic>Nickel oxides</topic><topic>Reduction</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Isaka, Yusuke</creatorcontrib><creatorcontrib>Kondo, Yoshifumi</creatorcontrib><creatorcontrib>Kawase, Yudai</creatorcontrib><creatorcontrib>Kuwahara, Yasutaka</creatorcontrib><creatorcontrib>Mori, Kohsuke</creatorcontrib><creatorcontrib>Yamashita, Hiromi</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>Chemical communications (Cambridge, England)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Isaka, Yusuke</au><au>Kondo, Yoshifumi</au><au>Kawase, Yudai</au><au>Kuwahara, Yasutaka</au><au>Mori, Kohsuke</au><au>Yamashita, Hiromi</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Photocatalytic production of hydrogen peroxide through selective two-electron reduction of dioxygen utilizing amine-functionalized MIL-125 deposited with nickel oxide nanoparticles</atitle><jtitle>Chemical communications (Cambridge, England)</jtitle><addtitle>Chem Commun (Camb)</addtitle><date>2018</date><risdate>2018</risdate><volume>54</volume><issue>67</issue><spage>927</spage><epage>9273</epage><pages>927-9273</pages><issn>1359-7345</issn><eissn>1364-548X</eissn><abstract>Photocatalytic H
2
O
2
production
via
two-electron reduction of O
2
was realized by visible-light irradiation of a metal-organic framework, MIL-125-NH
2
, in the presence of TEOA and benzylalcohol. Deposition of NiO nanoparticles onto MIL-125-NH
2
dramatically enhanced the catalytic activity. Further studies suggested that fast disproportionation of the O
2
&z.rad;
−
intermediate to H
2
O
2
resulted in the enhancement.
Photocatalytic H
2
O
2
production
via
two-electron reduction of O
2
is realized by visible-light irradiation of a Ti-based metal-organic framework, MIL-125-NH
2
.</abstract><cop>England</cop><pub>Royal Society of Chemistry</pub><pmid>29993052</pmid><doi>10.1039/c8cc02679c</doi><tpages>4</tpages><orcidid>https://orcid.org/0000-0003-1796-5776</orcidid><orcidid>https://orcid.org/0000-0002-5867-6463</orcidid><orcidid>https://orcid.org/0000-0003-3915-4528</orcidid></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 1359-7345 |
| ispartof | Chemical communications (Cambridge, England), 2018, Vol.54 (67), p.927-9273 |
| issn | 1359-7345 1364-548X |
| language | eng |
| recordid | cdi_rsc_primary_c8cc02679c |
| source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| subjects | Catalysis Catalytic activity Disproportionation Hydrogen peroxide Hydrogen production Light irradiation Metal-organic frameworks Nanoparticles Nickel oxides Reduction |
| title | Photocatalytic production of hydrogen peroxide through selective two-electron reduction of dioxygen utilizing amine-functionalized MIL-125 deposited with nickel oxide nanoparticles |
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