Photochemical tyrosine oxidation with a hydrogen-bonded proton acceptor by bidirectional proton-coupled electron transferElectronic supplementary information (ESI) available: Synthetic procedures, detailed experimental methods, kinetic analysis, fitting details, base concentration-dependent emission quenching data. See DOI: 10.1039/c2sc20113e
Amino acid radical generation and transport are fundamentally important to numerous essential biological processes to which small molecule models lend valuable mechanistic insights. Pyridyl-amino acid-methyl esters are appended to a rhenium( i ) tricarbonyl 1,10-phenanthroline core to yield rhenium-...
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