Heteroatoms Induce Localization of the Electric Field and Promote a Wide Potential‐Window Selectivity Towards CO in the CO2 Electroreduction

Carbon dioxide electroreduction (CO2RR) is a sustainable way of producing carbon‐neutral fuels. Product selectivity in CO2RR is regulated by the adsorption energy of reaction‐intermediates. Here, we employ differential phase contrast‐scanning transmission electron microscopy (DPC‐STEM) to demonstrat...

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Veröffentlicht in:	Angewandte Chemie International Edition 2022-11, Vol.61 (44), p.e202212640-n/a
Hauptverfasser:	Cai, Chao, Liu, Bao, Liu, Kang, Li, Pengcheng, Fu, Junwei, Wang, Yanqiu, Li, Wenzhang, Tian, Chen, Kang, Yicui, Stefancu, Andrei, Li, Hongmei, Kao, Cheng‐Wei, Chan, Ting‐Shan, Lin, Zhang, Chai, Liyuan, Cortés, Emiliano, Liu, Min
Format:	Artikel
Sprache:	eng
Schlagworte:	Adsorption Ag-Based Carbon dioxide Catalysts Communication Communications Electric fields Electric Filed Electrochemical CO2 Reduction Electrowinning Energy efficiency Heteroatoms Infrared reflection Infrared spectroscopy Intermediate Intermediates Localization Phase contrast Reaction intermediates Scanning transmission electron microscopy Selectivity Silver Tin Transmission electron microscopy
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