Selectivity of Per- and Polyfluoroalkyl Substance Sensors and Sorbents in Water
Per- and polyfluoroalkyl substances (PFAS) are a large group of engineered chemicals that have been widely used in industrial production. PFAS have drawn increasing attention due to their frequent occurrence in the aquatic environment and their toxicity to animals and humans. Developing effective an...
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| Veröffentlicht in: | ACS applied materials & interfaces 2021-12, Vol.13 (51), p.60789-60814 |
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| creator | Wang, Yuqin Darling, Seth B Chen, Junhong |
| description | Per- and polyfluoroalkyl substances (PFAS) are a large group of engineered chemicals that have been widely used in industrial production. PFAS have drawn increasing attention due to their frequent occurrence in the aquatic environment and their toxicity to animals and humans. Developing effective and efficient detection and remediation methods for PFAS in aquatic systems is critical to mitigate ongoing exposure and promote water reuse. Adsorption-based removal is the most common method for PFAS remediation since it avoids hazardous byproducts; in situ sensing technology is a promising approach for PFAS monitoring due to its fast response, easy operation, and portability. This review summarizes current materials and devices that have been demonstrated for PFAS adsorption and sensing. Selectivity, the key factor underlying both sensor and sorbent performance, is discussed by exploring the interactions between PFAS and various probes. Examples of selective probes will be presented and classified by fluorinated groups, cationic groups, and cavitary groups, and their synergistic effects will also be analyzed. This review aims to provide guidance and implication for future material design toward more selective and effective PFAS sensors and sorbents. |
| doi_str_mv | 10.1021/acsami.1c16517 |
| format | Article |
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(ANL), Argonne, IL (United States)</creatorcontrib><description>Per- and polyfluoroalkyl substances (PFAS) are a large group of engineered chemicals that have been widely used in industrial production. PFAS have drawn increasing attention due to their frequent occurrence in the aquatic environment and their toxicity to animals and humans. Developing effective and efficient detection and remediation methods for PFAS in aquatic systems is critical to mitigate ongoing exposure and promote water reuse. Adsorption-based removal is the most common method for PFAS remediation since it avoids hazardous byproducts; in situ sensing technology is a promising approach for PFAS monitoring due to its fast response, easy operation, and portability. This review summarizes current materials and devices that have been demonstrated for PFAS adsorption and sensing. Selectivity, the key factor underlying both sensor and sorbent performance, is discussed by exploring the interactions between PFAS and various probes. Examples of selective probes will be presented and classified by fluorinated groups, cationic groups, and cavitary groups, and their synergistic effects will also be analyzed. This review aims to provide guidance and implication for future material design toward more selective and effective PFAS sensors and sorbents.</description><identifier>ISSN: 1944-8244</identifier><identifier>EISSN: 1944-8252</identifier><identifier>DOI: 10.1021/acsami.1c16517</identifier><identifier>PMID: 34911297</identifier><language>eng</language><publisher>WASHINGTON: American Chemical Society</publisher><subject>adsorption ; detection ; fluorescence ; INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY ; Materials Science ; Materials Science, Multidisciplinary ; Nanoscience & Nanotechnology ; PFAS ; Review ; Science & Technology ; Science & Technology - Other Topics ; selectivity ; sensors ; sorbents ; Technology ; water pollution ; water treatment</subject><ispartof>ACS applied materials & interfaces, 2021-12, Vol.13 (51), p.60789-60814</ispartof><rights>2021 The Authors. Published by American Chemical Society</rights><rights>2021 The Authors. 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(ANL), Argonne, IL (United States)</creatorcontrib><title>Selectivity of Per- and Polyfluoroalkyl Substance Sensors and Sorbents in Water</title><title>ACS applied materials & interfaces</title><addtitle>ACS APPL MATER INTER</addtitle><addtitle>ACS Appl. Mater. Interfaces</addtitle><description>Per- and polyfluoroalkyl substances (PFAS) are a large group of engineered chemicals that have been widely used in industrial production. PFAS have drawn increasing attention due to their frequent occurrence in the aquatic environment and their toxicity to animals and humans. Developing effective and efficient detection and remediation methods for PFAS in aquatic systems is critical to mitigate ongoing exposure and promote water reuse. Adsorption-based removal is the most common method for PFAS remediation since it avoids hazardous byproducts; in situ sensing technology is a promising approach for PFAS monitoring due to its fast response, easy operation, and portability. This review summarizes current materials and devices that have been demonstrated for PFAS adsorption and sensing. Selectivity, the key factor underlying both sensor and sorbent performance, is discussed by exploring the interactions between PFAS and various probes. Examples of selective probes will be presented and classified by fluorinated groups, cationic groups, and cavitary groups, and their synergistic effects will also be analyzed. This review aims to provide guidance and implication for future material design toward more selective and effective PFAS sensors and sorbents.</description><subject>adsorption</subject><subject>detection</subject><subject>fluorescence</subject><subject>INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY</subject><subject>Materials Science</subject><subject>Materials Science, Multidisciplinary</subject><subject>Nanoscience & Nanotechnology</subject><subject>PFAS</subject><subject>Review</subject><subject>Science & Technology</subject><subject>Science & Technology - Other Topics</subject><subject>selectivity</subject><subject>sensors</subject><subject>sorbents</subject><subject>Technology</subject><subject>water pollution</subject><subject>water treatment</subject><issn>1944-8244</issn><issn>1944-8252</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><sourceid>HGBXW</sourceid><recordid>eNqNkc1LHTEUxYO0qLXddilDly3zzNfMJJtCedgPEBReS5chybup0XmJJBnl_fdGxz7souAqF_I7556cIPSe4AXBlJxom_XGL4glfUeGPXRIJOetoB19tZs5P0Bvcr7CuGcUd_vogHFJCJXDITpfwQi2-Ftftk10zQWkttFh3VzEcevGKaaox-vt2Kwmk4sOFpoVhBxTfqRWMRkIJTc-NL91gfQWvXZ6zPDu6TxCv76e_lx-b8_Ov_1YfjlrNe9oaRkfhJYceukcdcO6E0ZYbtZAjcEAzFiBe0c0BSuZs_VtHYNuwLqjUoDE7Ah9nn1vJrOBta0hkh7VTfIbnbYqaq_-vQn-Uv2Jt0oMRDJKq8GH2SDm4lW2voC9tDGE2oYigvWkHyq0mCGbYs4J3G4BweqhfzX3r576r4Lj57F2-N_CKyBm4A5MdHUt1Ep3GMZ4YExQweuEydIXXXwMyziFUqWfXi6t9MeZrgnVVZxSqN_xv9j3YBOyfA</recordid><startdate>20211229</startdate><enddate>20211229</enddate><creator>Wang, Yuqin</creator><creator>Darling, Seth B</creator><creator>Chen, Junhong</creator><general>American Chemical Society</general><general>Amer Chemical Soc</general><scope>BLEPL</scope><scope>DTL</scope><scope>HGBXW</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>OTOTI</scope><scope>5PM</scope><orcidid>https://orcid.org/0000-0002-5461-6965</orcidid><orcidid>https://orcid.org/0000-0003-4444-2487</orcidid><orcidid>https://orcid.org/0000-0002-2615-1347</orcidid><orcidid>https://orcid.org/0000000226151347</orcidid><orcidid>https://orcid.org/0000000254616965</orcidid><orcidid>https://orcid.org/0000000344442487</orcidid></search><sort><creationdate>20211229</creationdate><title>Selectivity of Per- and Polyfluoroalkyl Substance Sensors and Sorbents in Water</title><author>Wang, Yuqin ; Darling, Seth B ; Chen, Junhong</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a452t-3478a94e69ff2f7d58b8c4bde2bb0ee3bc806f1a2ec93fc65153e570a5298e903</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>adsorption</topic><topic>detection</topic><topic>fluorescence</topic><topic>INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY</topic><topic>Materials Science</topic><topic>Materials Science, Multidisciplinary</topic><topic>Nanoscience & Nanotechnology</topic><topic>PFAS</topic><topic>Review</topic><topic>Science & Technology</topic><topic>Science & Technology - Other Topics</topic><topic>selectivity</topic><topic>sensors</topic><topic>sorbents</topic><topic>Technology</topic><topic>water pollution</topic><topic>water treatment</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Wang, Yuqin</creatorcontrib><creatorcontrib>Darling, Seth B</creatorcontrib><creatorcontrib>Chen, Junhong</creatorcontrib><creatorcontrib>Univ. of Chicago, IL (United States)</creatorcontrib><creatorcontrib>Argonne National Lab. 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| subjects | adsorption detection fluorescence INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY Materials Science Materials Science, Multidisciplinary Nanoscience & Nanotechnology PFAS Review Science & Technology Science & Technology - Other Topics selectivity sensors sorbents Technology water pollution water treatment |
| title | Selectivity of Per- and Polyfluoroalkyl Substance Sensors and Sorbents in Water |
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