A highly-enriched 244Pu reference material for nuclear safeguards and nuclear forensics measurements
A highly-enriched 244 Pu isotope dilution reference material has been prepared and characterized for metrologically traceable measurements of very small quantities of plutonium. The amount of plutonium in samples associated with nuclear safeguards and nuclear forensic measurements can be significant...
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| Veröffentlicht in: | Journal of radioanalytical and nuclear chemistry 2020, Vol.324 (1), p.257-270 |
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| container_title | Journal of radioanalytical and nuclear chemistry |
| container_volume | 324 |
| creator | Essex, Richard M. Williams, Ross W. Treinen, Kerri C. Hubert, Amélie Humphrey, Marc A. Inglis, Jeremy D. Kinman, William S. Maassen, Joel Peńkin, Maxim V. Steiner, Robert E. |
| description | A highly-enriched
244
Pu isotope dilution reference material has been prepared and characterized for metrologically traceable measurements of very small quantities of plutonium. The amount of plutonium in samples associated with nuclear safeguards and nuclear forensic measurements can be significantly less than 1 ng. Accordingly, the ability to quantify the amount and isotopic composition of plutonium from a single mass-spectrometric analysis is particularly desirable. The highly-enriched
244
Pu reference material, described here, will minimize the magnitude of spike corrections necessary to obtain accurate information on plutonium isotopic composition from isotope dilution measurements. |
| doi_str_mv | 10.1007/s10967-020-07075-y |
| format | Article |
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244
Pu isotope dilution reference material has been prepared and characterized for metrologically traceable measurements of very small quantities of plutonium. The amount of plutonium in samples associated with nuclear safeguards and nuclear forensic measurements can be significantly less than 1 ng. Accordingly, the ability to quantify the amount and isotopic composition of plutonium from a single mass-spectrometric analysis is particularly desirable. The highly-enriched
244
Pu reference material, described here, will minimize the magnitude of spike corrections necessary to obtain accurate information on plutonium isotopic composition from isotope dilution measurements.</description><identifier>ISSN: 0236-5731</identifier><identifier>EISSN: 1588-2780</identifier><identifier>DOI: 10.1007/s10967-020-07075-y</identifier><identifier>PMID: 34248241</identifier><language>eng</language><publisher>Cham: Springer International Publishing</publisher><subject>07 ISOTOPE AND RADIATION SOURCES ; Chemistry ; Chemistry and Materials Science ; Composition ; Diagnostic Radiology ; Dilution ; Enrichment ; Hadrons ; Heavy Ions ; Inorganic Chemistry ; isotope dilution mass spectrometry ; Isotopes ; nuclear 40 safeguards ; Nuclear Chemistry ; NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL PROTECTION ; nuclear forensics ; Nuclear Physics ; Nuclear safety ; Physical Chemistry ; Plutonium ; RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEAR CHEMISTRY ; reference material ; Reference materials ; Spectrometry ; traceability</subject><ispartof>Journal of radioanalytical and nuclear chemistry, 2020, Vol.324 (1), p.257-270</ispartof><rights>This is a U.S. Government work and not under copyright protection in the US; foreign copyright protection may apply 2020</rights><rights>2020© This is a U.S. Government work and not under copyright protection in the US; foreign copyright protection may apply 2020</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c323y-3ac0dd10b50d66a627c844c8aa13364dc12484d6aa9c9d355ff501a4a4cebbe63</citedby><cites>FETCH-LOGICAL-c323y-3ac0dd10b50d66a627c844c8aa13364dc12484d6aa9c9d355ff501a4a4cebbe63</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10967-020-07075-y$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10967-020-07075-y$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>230,314,780,784,885,27924,27925,41488,42557,51319</link.rule.ids><backlink>$$Uhttps://www.osti.gov/servlets/purl/1813701$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Essex, Richard M.</creatorcontrib><creatorcontrib>Williams, Ross W.</creatorcontrib><creatorcontrib>Treinen, Kerri C.</creatorcontrib><creatorcontrib>Hubert, Amélie</creatorcontrib><creatorcontrib>Humphrey, Marc A.</creatorcontrib><creatorcontrib>Inglis, Jeremy D.</creatorcontrib><creatorcontrib>Kinman, William S.</creatorcontrib><creatorcontrib>Maassen, Joel</creatorcontrib><creatorcontrib>Peńkin, Maxim V.</creatorcontrib><creatorcontrib>Steiner, Robert E.</creatorcontrib><creatorcontrib>Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)</creatorcontrib><creatorcontrib>Los Alamos National Lab. (LANL), Los Alamos, NM (United States)</creatorcontrib><title>A highly-enriched 244Pu reference material for nuclear safeguards and nuclear forensics measurements</title><title>Journal of radioanalytical and nuclear chemistry</title><addtitle>J Radioanal Nucl Chem</addtitle><description>A highly-enriched
244
Pu isotope dilution reference material has been prepared and characterized for metrologically traceable measurements of very small quantities of plutonium. The amount of plutonium in samples associated with nuclear safeguards and nuclear forensic measurements can be significantly less than 1 ng. Accordingly, the ability to quantify the amount and isotopic composition of plutonium from a single mass-spectrometric analysis is particularly desirable. The highly-enriched
244
Pu reference material, described here, will minimize the magnitude of spike corrections necessary to obtain accurate information on plutonium isotopic composition from isotope dilution measurements.</description><subject>07 ISOTOPE AND RADIATION SOURCES</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Composition</subject><subject>Diagnostic Radiology</subject><subject>Dilution</subject><subject>Enrichment</subject><subject>Hadrons</subject><subject>Heavy Ions</subject><subject>Inorganic Chemistry</subject><subject>isotope dilution mass spectrometry</subject><subject>Isotopes</subject><subject>nuclear 40 safeguards</subject><subject>Nuclear Chemistry</subject><subject>NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL PROTECTION</subject><subject>nuclear forensics</subject><subject>Nuclear Physics</subject><subject>Nuclear safety</subject><subject>Physical Chemistry</subject><subject>Plutonium</subject><subject>RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEAR CHEMISTRY</subject><subject>reference material</subject><subject>Reference materials</subject><subject>Spectrometry</subject><subject>traceability</subject><issn>0236-5731</issn><issn>1588-2780</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><recordid>eNp9kUtv1TAQhS0EopfCH2AVwYZNYPyM7wapqnhJlWABa2uuPbnXVeIUO6mUf49LqiJYsLI0_s45ozmMveTwlgN07wqHvelaENBCB51u10dsx7W1regsPGY7ENK0upP8jD0r5RoA9tbKp-xMKqGsUHzHwkVzisfTsLaUcvQnCo1Q6tvSZOopU_LUjDhTjjg0_ZSbtPiBMDcFezoumENpMIWHcUUolehLMxKWJdNIaS7P2ZMeh0Iv7t9z9uPjh--Xn9urr5--XF5ctV4KubYSPYTA4aAhGINGdN4q5S0il9Ko4HndWgWDuPf7ILXuew0cFSpPhwMZec7eb743y2Gk4Gt2xsHd5DhiXt2E0f39k-LJHadbZ4Wxne2qwavNYCpzdMXHmfzJTymRnx23XHbAK_TmPiVPPxcqsxtj8TQMmGhaihNag5FCG13R1_-g19OSU72BE9JKy7WCu1SxUT5PpdTDP2zMwd017bamXW3a_W7arVUkN1GpcDpS_mP9H9UvXoWsCw</recordid><startdate>2020</startdate><enddate>2020</enddate><creator>Essex, Richard M.</creator><creator>Williams, Ross W.</creator><creator>Treinen, Kerri C.</creator><creator>Hubert, Amélie</creator><creator>Humphrey, Marc A.</creator><creator>Inglis, Jeremy D.</creator><creator>Kinman, William S.</creator><creator>Maassen, Joel</creator><creator>Peńkin, Maxim V.</creator><creator>Steiner, Robert E.</creator><general>Springer International Publishing</general><general>Springer Nature B.V</general><general>Springer</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>OIOZB</scope><scope>OTOTI</scope><scope>5PM</scope></search><sort><creationdate>2020</creationdate><title>A highly-enriched 244Pu reference material for nuclear safeguards and nuclear forensics measurements</title><author>Essex, Richard M. ; Williams, Ross W. ; Treinen, Kerri C. ; Hubert, Amélie ; Humphrey, Marc A. ; Inglis, Jeremy D. ; Kinman, William S. ; Maassen, Joel ; Peńkin, Maxim V. ; Steiner, Robert E.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c323y-3ac0dd10b50d66a627c844c8aa13364dc12484d6aa9c9d355ff501a4a4cebbe63</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>07 ISOTOPE AND RADIATION SOURCES</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Composition</topic><topic>Diagnostic Radiology</topic><topic>Dilution</topic><topic>Enrichment</topic><topic>Hadrons</topic><topic>Heavy Ions</topic><topic>Inorganic Chemistry</topic><topic>isotope dilution mass spectrometry</topic><topic>Isotopes</topic><topic>nuclear 40 safeguards</topic><topic>Nuclear Chemistry</topic><topic>NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL PROTECTION</topic><topic>nuclear forensics</topic><topic>Nuclear Physics</topic><topic>Nuclear safety</topic><topic>Physical Chemistry</topic><topic>Plutonium</topic><topic>RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEAR CHEMISTRY</topic><topic>reference material</topic><topic>Reference materials</topic><topic>Spectrometry</topic><topic>traceability</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Essex, Richard M.</creatorcontrib><creatorcontrib>Williams, Ross W.</creatorcontrib><creatorcontrib>Treinen, Kerri C.</creatorcontrib><creatorcontrib>Hubert, Amélie</creatorcontrib><creatorcontrib>Humphrey, Marc A.</creatorcontrib><creatorcontrib>Inglis, Jeremy D.</creatorcontrib><creatorcontrib>Kinman, William S.</creatorcontrib><creatorcontrib>Maassen, Joel</creatorcontrib><creatorcontrib>Peńkin, Maxim V.</creatorcontrib><creatorcontrib>Steiner, Robert E.</creatorcontrib><creatorcontrib>Lawrence Livermore National Lab. 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(LANL), Los Alamos, NM (United States)</aucorp><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>A highly-enriched 244Pu reference material for nuclear safeguards and nuclear forensics measurements</atitle><jtitle>Journal of radioanalytical and nuclear chemistry</jtitle><stitle>J Radioanal Nucl Chem</stitle><date>2020</date><risdate>2020</risdate><volume>324</volume><issue>1</issue><spage>257</spage><epage>270</epage><pages>257-270</pages><issn>0236-5731</issn><eissn>1588-2780</eissn><abstract>A highly-enriched
244
Pu isotope dilution reference material has been prepared and characterized for metrologically traceable measurements of very small quantities of plutonium. The amount of plutonium in samples associated with nuclear safeguards and nuclear forensic measurements can be significantly less than 1 ng. Accordingly, the ability to quantify the amount and isotopic composition of plutonium from a single mass-spectrometric analysis is particularly desirable. The highly-enriched
244
Pu reference material, described here, will minimize the magnitude of spike corrections necessary to obtain accurate information on plutonium isotopic composition from isotope dilution measurements.</abstract><cop>Cham</cop><pub>Springer International Publishing</pub><pmid>34248241</pmid><doi>10.1007/s10967-020-07075-y</doi><tpages>14</tpages><oa>free_for_read</oa></addata></record> |
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| ispartof | Journal of radioanalytical and nuclear chemistry, 2020, Vol.324 (1), p.257-270 |
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| subjects | 07 ISOTOPE AND RADIATION SOURCES Chemistry Chemistry and Materials Science Composition Diagnostic Radiology Dilution Enrichment Hadrons Heavy Ions Inorganic Chemistry isotope dilution mass spectrometry Isotopes nuclear 40 safeguards Nuclear Chemistry NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL PROTECTION nuclear forensics Nuclear Physics Nuclear safety Physical Chemistry Plutonium RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEAR CHEMISTRY reference material Reference materials Spectrometry traceability |
| title | A highly-enriched 244Pu reference material for nuclear safeguards and nuclear forensics measurements |
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