Decoherence and revival in attosecond charge migration driven by non-adiabatic dynamics

Attosecond charge migration is a periodic evolution of the charge density at specific sites of a molecule on a timescale defined by the energy intervals between the electronic states involved. Here we report the observation of charge migration in neutral silane (SiH 4 ) in 690 as, its decoherence wi...

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Veröffentlicht in:Nature physics 2022-10, Vol.18 (10), p.1206-1213
Hauptverfasser: Matselyukh, Danylo T., Despré, Victor, Golubev, Nikolay V., Kuleff, Alexander I., Wörner, Hans Jakob
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Sprache:eng
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