Bottom-Up, On-Surface-Synthesized Armchair Graphene Nanoribbons for Ultra-High-Power Micro-Supercapacitors
Bottom-up-synthesized graphene nanoribbons (GNRs) with excellent electronic properties are promising materials for energy storage systems. Herein, we report bottom-up-synthesized GNR films employed as electrode materials for micro-supercapacitors (MSCs). The micro-device delivers an excellent volume...
Gespeichert in:
| Veröffentlicht in: | Journal of the American Chemical Society 2020-10, Vol.142 (42), p.17881-17886 |
|---|---|
| Hauptverfasser: | , , , , , , , , , |
| Format: | Artikel |
| Sprache: | eng |
| Schlagworte: | |
| Online-Zugang: | Volltext |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | 17886 |
|---|---|
| container_issue | 42 |
| container_start_page | 17881 |
| container_title | Journal of the American Chemical Society |
| container_volume | 142 |
| creator | Liu, Zhaoyang Chen, Zongping Wang, Can Wang, Hai I Wuttke, Michael Wang, Xiao-Ye Bonn, Mischa Chi, Lifeng Narita, Akimitsu Müllen, Klaus |
| description | Bottom-up-synthesized graphene nanoribbons (GNRs) with excellent electronic properties are promising materials for energy storage systems. Herein, we report bottom-up-synthesized GNR films employed as electrode materials for micro-supercapacitors (MSCs). The micro-device delivers an excellent volumetric capacitance and an ultra-high power density. The electrochemical performance of MSCs could be correlated with the charge carrier mobility within the differently employed GNRs, as determined by pump–probe terahertz spectroscopy studies. |
| doi_str_mv | 10.1021/jacs.0c06109 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_pubme</sourceid><recordid>TN_cdi_pubmedcentral_primary_oai_pubmedcentral_nih_gov_7582623</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2449181983</sourcerecordid><originalsourceid>FETCH-LOGICAL-a460t-642b28a423fff9459da6715c471334c26ae2c2ec6db23db797908c7f0c1955783</originalsourceid><addsrcrecordid>eNptkclKxTAUhoMoeh12PkCXLoxmapJuBBUncAK965Cmqc2lTWrSKvr09uJFEVyFk_Of7ww_APsYHWFE8PFCm3SEDOIYFWtghnOCYI4JXwczhBCBQnK6BbZTWkwhIxJvgi1Kp0ohxQwszsIwhA7O-8PswcOnMdbaWPj04YfGJvdpq-w0dqbRLmZXUfeN9Ta71z5EV5bBp6wOMZu3Q9Tw2r008DG825jdORPDBOttNLrXxg0hpl2wUes22b3VuwPmlxfP59fw9uHq5vz0FmrG0QA5IyWRmhFa13XB8qLSXODcMIEpZYZwbYkh1vCqJLQqRSEKJI2okcFFngtJd8DJN7cfy85Wxvppulb10XU6fqignfqb8a5RL-FNiVwSTugEOFgBYngdbRpU55Kxbau9DWNShLECS1zIpfTwWzrtm1K09U8bjNTSHrW0R63s-SUvPxdhjH46xP_SL5Y9kII</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2449181983</pqid></control><display><type>article</type><title>Bottom-Up, On-Surface-Synthesized Armchair Graphene Nanoribbons for Ultra-High-Power Micro-Supercapacitors</title><source>American Chemical Society Journals</source><creator>Liu, Zhaoyang ; Chen, Zongping ; Wang, Can ; Wang, Hai I ; Wuttke, Michael ; Wang, Xiao-Ye ; Bonn, Mischa ; Chi, Lifeng ; Narita, Akimitsu ; Müllen, Klaus</creator><creatorcontrib>Liu, Zhaoyang ; Chen, Zongping ; Wang, Can ; Wang, Hai I ; Wuttke, Michael ; Wang, Xiao-Ye ; Bonn, Mischa ; Chi, Lifeng ; Narita, Akimitsu ; Müllen, Klaus</creatorcontrib><description>Bottom-up-synthesized graphene nanoribbons (GNRs) with excellent electronic properties are promising materials for energy storage systems. Herein, we report bottom-up-synthesized GNR films employed as electrode materials for micro-supercapacitors (MSCs). The micro-device delivers an excellent volumetric capacitance and an ultra-high power density. The electrochemical performance of MSCs could be correlated with the charge carrier mobility within the differently employed GNRs, as determined by pump–probe terahertz spectroscopy studies.</description><identifier>ISSN: 0002-7863</identifier><identifier>EISSN: 1520-5126</identifier><identifier>DOI: 10.1021/jacs.0c06109</identifier><identifier>PMID: 33021787</identifier><language>eng</language><publisher>American Chemical Society</publisher><subject>Communication</subject><ispartof>Journal of the American Chemical Society, 2020-10, Vol.142 (42), p.17881-17886</ispartof><rights>XXXX American Chemical Society</rights><rights>2020 American Chemical Society 2020 American Chemical Society</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a460t-642b28a423fff9459da6715c471334c26ae2c2ec6db23db797908c7f0c1955783</citedby><cites>FETCH-LOGICAL-a460t-642b28a423fff9459da6715c471334c26ae2c2ec6db23db797908c7f0c1955783</cites><orcidid>0000-0003-3835-2776 ; 0000-0003-0940-3984 ; 0000-0001-7972-3452 ; 0000-0003-3540-0277 ; 0000-0002-3625-522X ; 0000-0001-6630-8786 ; 0000-0001-6851-8453</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/jacs.0c06109$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/jacs.0c06109$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>230,314,780,784,885,2765,27076,27924,27925,56738,56788</link.rule.ids></links><search><creatorcontrib>Liu, Zhaoyang</creatorcontrib><creatorcontrib>Chen, Zongping</creatorcontrib><creatorcontrib>Wang, Can</creatorcontrib><creatorcontrib>Wang, Hai I</creatorcontrib><creatorcontrib>Wuttke, Michael</creatorcontrib><creatorcontrib>Wang, Xiao-Ye</creatorcontrib><creatorcontrib>Bonn, Mischa</creatorcontrib><creatorcontrib>Chi, Lifeng</creatorcontrib><creatorcontrib>Narita, Akimitsu</creatorcontrib><creatorcontrib>Müllen, Klaus</creatorcontrib><title>Bottom-Up, On-Surface-Synthesized Armchair Graphene Nanoribbons for Ultra-High-Power Micro-Supercapacitors</title><title>Journal of the American Chemical Society</title><addtitle>J. Am. Chem. Soc</addtitle><description>Bottom-up-synthesized graphene nanoribbons (GNRs) with excellent electronic properties are promising materials for energy storage systems. Herein, we report bottom-up-synthesized GNR films employed as electrode materials for micro-supercapacitors (MSCs). The micro-device delivers an excellent volumetric capacitance and an ultra-high power density. The electrochemical performance of MSCs could be correlated with the charge carrier mobility within the differently employed GNRs, as determined by pump–probe terahertz spectroscopy studies.</description><subject>Communication</subject><issn>0002-7863</issn><issn>1520-5126</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><recordid>eNptkclKxTAUhoMoeh12PkCXLoxmapJuBBUncAK965Cmqc2lTWrSKvr09uJFEVyFk_Of7ww_APsYHWFE8PFCm3SEDOIYFWtghnOCYI4JXwczhBCBQnK6BbZTWkwhIxJvgi1Kp0ohxQwszsIwhA7O-8PswcOnMdbaWPj04YfGJvdpq-w0dqbRLmZXUfeN9Ta71z5EV5bBp6wOMZu3Q9Tw2r008DG825jdORPDBOttNLrXxg0hpl2wUes22b3VuwPmlxfP59fw9uHq5vz0FmrG0QA5IyWRmhFa13XB8qLSXODcMIEpZYZwbYkh1vCqJLQqRSEKJI2okcFFngtJd8DJN7cfy85Wxvppulb10XU6fqignfqb8a5RL-FNiVwSTugEOFgBYngdbRpU55Kxbau9DWNShLECS1zIpfTwWzrtm1K09U8bjNTSHrW0R63s-SUvPxdhjH46xP_SL5Y9kII</recordid><startdate>20201021</startdate><enddate>20201021</enddate><creator>Liu, Zhaoyang</creator><creator>Chen, Zongping</creator><creator>Wang, Can</creator><creator>Wang, Hai I</creator><creator>Wuttke, Michael</creator><creator>Wang, Xiao-Ye</creator><creator>Bonn, Mischa</creator><creator>Chi, Lifeng</creator><creator>Narita, Akimitsu</creator><creator>Müllen, Klaus</creator><general>American Chemical Society</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>5PM</scope><orcidid>https://orcid.org/0000-0003-3835-2776</orcidid><orcidid>https://orcid.org/0000-0003-0940-3984</orcidid><orcidid>https://orcid.org/0000-0001-7972-3452</orcidid><orcidid>https://orcid.org/0000-0003-3540-0277</orcidid><orcidid>https://orcid.org/0000-0002-3625-522X</orcidid><orcidid>https://orcid.org/0000-0001-6630-8786</orcidid><orcidid>https://orcid.org/0000-0001-6851-8453</orcidid></search><sort><creationdate>20201021</creationdate><title>Bottom-Up, On-Surface-Synthesized Armchair Graphene Nanoribbons for Ultra-High-Power Micro-Supercapacitors</title><author>Liu, Zhaoyang ; Chen, Zongping ; Wang, Can ; Wang, Hai I ; Wuttke, Michael ; Wang, Xiao-Ye ; Bonn, Mischa ; Chi, Lifeng ; Narita, Akimitsu ; Müllen, Klaus</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a460t-642b28a423fff9459da6715c471334c26ae2c2ec6db23db797908c7f0c1955783</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>Communication</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Liu, Zhaoyang</creatorcontrib><creatorcontrib>Chen, Zongping</creatorcontrib><creatorcontrib>Wang, Can</creatorcontrib><creatorcontrib>Wang, Hai I</creatorcontrib><creatorcontrib>Wuttke, Michael</creatorcontrib><creatorcontrib>Wang, Xiao-Ye</creatorcontrib><creatorcontrib>Bonn, Mischa</creatorcontrib><creatorcontrib>Chi, Lifeng</creatorcontrib><creatorcontrib>Narita, Akimitsu</creatorcontrib><creatorcontrib>Müllen, Klaus</creatorcontrib><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>PubMed Central (Full Participant titles)</collection><jtitle>Journal of the American Chemical Society</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Liu, Zhaoyang</au><au>Chen, Zongping</au><au>Wang, Can</au><au>Wang, Hai I</au><au>Wuttke, Michael</au><au>Wang, Xiao-Ye</au><au>Bonn, Mischa</au><au>Chi, Lifeng</au><au>Narita, Akimitsu</au><au>Müllen, Klaus</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Bottom-Up, On-Surface-Synthesized Armchair Graphene Nanoribbons for Ultra-High-Power Micro-Supercapacitors</atitle><jtitle>Journal of the American Chemical Society</jtitle><addtitle>J. Am. Chem. Soc</addtitle><date>2020-10-21</date><risdate>2020</risdate><volume>142</volume><issue>42</issue><spage>17881</spage><epage>17886</epage><pages>17881-17886</pages><issn>0002-7863</issn><eissn>1520-5126</eissn><abstract>Bottom-up-synthesized graphene nanoribbons (GNRs) with excellent electronic properties are promising materials for energy storage systems. Herein, we report bottom-up-synthesized GNR films employed as electrode materials for micro-supercapacitors (MSCs). The micro-device delivers an excellent volumetric capacitance and an ultra-high power density. The electrochemical performance of MSCs could be correlated with the charge carrier mobility within the differently employed GNRs, as determined by pump–probe terahertz spectroscopy studies.</abstract><pub>American Chemical Society</pub><pmid>33021787</pmid><doi>10.1021/jacs.0c06109</doi><tpages>6</tpages><orcidid>https://orcid.org/0000-0003-3835-2776</orcidid><orcidid>https://orcid.org/0000-0003-0940-3984</orcidid><orcidid>https://orcid.org/0000-0001-7972-3452</orcidid><orcidid>https://orcid.org/0000-0003-3540-0277</orcidid><orcidid>https://orcid.org/0000-0002-3625-522X</orcidid><orcidid>https://orcid.org/0000-0001-6630-8786</orcidid><orcidid>https://orcid.org/0000-0001-6851-8453</orcidid><oa>free_for_read</oa></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0002-7863 |
| ispartof | Journal of the American Chemical Society, 2020-10, Vol.142 (42), p.17881-17886 |
| issn | 0002-7863 1520-5126 |
| language | eng |
| recordid | cdi_pubmedcentral_primary_oai_pubmedcentral_nih_gov_7582623 |
| source | American Chemical Society Journals |
| subjects | Communication |
| title | Bottom-Up, On-Surface-Synthesized Armchair Graphene Nanoribbons for Ultra-High-Power Micro-Supercapacitors |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2024-12-25T03%3A46%3A28IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_pubme&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Bottom-Up,%20On-Surface-Synthesized%20Armchair%20Graphene%20Nanoribbons%20for%20Ultra-High-Power%20Micro-Supercapacitors&rft.jtitle=Journal%20of%20the%20American%20Chemical%20Society&rft.au=Liu,%20Zhaoyang&rft.date=2020-10-21&rft.volume=142&rft.issue=42&rft.spage=17881&rft.epage=17886&rft.pages=17881-17886&rft.issn=0002-7863&rft.eissn=1520-5126&rft_id=info:doi/10.1021/jacs.0c06109&rft_dat=%3Cproquest_pubme%3E2449181983%3C/proquest_pubme%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2449181983&rft_id=info:pmid/33021787&rfr_iscdi=true |